We have prepared two ultracold fermionic atoms in an isolated double-well potential and obtained full control over the quantum state of this system. In particular, we can independently control the interaction strength between the particles, their tunneling rate between the wells and the tilt of the potential. By introducing repulsive (attractive) interparticle interactions we have realized the two-particle analog of a Mott-insulating (charge-density-wave) state. We have also spectroscopically observed how second-order tunneling affects the energy of the system. This work realizes the first step of a bottom-up approach to deterministically create a single-site addressable realization of a ground-state Fermi-Hubbard system.
We have prepared two ultracold fermionic atoms in an isolated double-well potential and obtained full control over the quantum state of this system. In particular, we can independently control the interaction strength between the particles, their tunneling rate between the wells and the tilt of the potential. By introducing repulsive (attractive) interparticle interactions we have realized the two-particle analog of a Mott-insulating (charge-density-wave) state. We have also spectroscopically observed how second-order tunneling affects the energy of the system. This work realizes the first step of a bottom-up approach to deterministically create a single-site addressable realization of a ground-state Fermi-Hubbard system.
In this thesis, I report on the deterministic preparation and the observation of strongly correlated few-fermion systems in single and double-well potentials. In a first experiment, we studied a system of one impurity interacting with a number of majority atoms which we prepared in a single potential well in the one-dimensional limit. With increasing number of majority particles, we observed a decrease in the quasi-particle residue which is in agreement with expectations from the Anderson orthogonality catastrophe. In a second experiment, we prepared two fermions in a double-well potential which represents the fundamental building block of the Fermi-Hubbard model. By increasing the repulsion between the two fermions, we observed the crossover into the antiferromagnetic Mott-insulator regime. Furthermore, I describe a new imaging technique, which allows spin-resolved single-atom detection both in in-situ and in time-of-flight. We use this technique to investigate the emergence of momentum correlations of two repulsive fermions in the ground state of the double well. With the methods developed in this thesis, we have established a framework for quantum simulation of strongly correlated many-body systems in tunable potentials.
"Bottom-up" approaches to the many-body physics of fermions have recently demonstrated precise number and site-resolved preparations with tunability of interparticle interactions in single-well, SW, and double-well, DW, nanoscale confinements created by manipulating ultracold fermionic atoms with optical tweezers. These experiments emulate an analogue-simulator mapping onto the requisite microscopic Hamiltonian, approaching realization of Feynmans' vision of quantum simulators that "will do exactly the same as nature". Here we report on exact benchmark configuration-interaction computational microscopy solutions of the Hamiltonian, uncovering the spectral evolution, wave function anatomy, and entanglement properties of the interacting fermions in the entire parameter range, including crossover from an SW to a DW confinement and a controllable energy imbalance between the wells. We demonstrate attractive pairing and formation of repulsive, highly correlated, ultracold Wigner molecules, well-described in the natural orbital representation. The agreement with the measurements affirms the henceforth gained deep insights into ultracold molecules and opens access to the size-dependent evolution of nanoclustered and condensed-matter phases and ultracold-atoms quantum information.
Identification and understanding of the evolution of interference patterns in two-particle momentum correlations as a function of the strength of interatomic interactions are important in explorations of the nature of quantum states of trapped particles. Together with the analysis of two-particle spatial correlations, they offer the prospect of uncovering fundamental symmetries and structure of correlated many-body states, as well as opening vistas into potential control and utilization of correlated quantum states as quantum information resources. With the use of the two-particle density matrix constructed via configuration-interaction (CI) exact diagonalization of the microscopic Hamiltonian, we explored here the systematic evolution of characteristic, damped, interference patterns in the two-particle momentum and spatial correlation maps of two ultracold fermionic atoms trapped in a double-well potential, over the entire range of variation of the contact repulsive interatomic interaction strength. For the singlet ground state the two-particle momentum maps were found to transform from a square-plaid pattern for non-interacting particles, to a system of striped interference fringes, with the most intense fringe lying along the main diagonal indicating bunching. Two-particle momentum correlation maps for low-lying excited states were also analyzed, with the triplet excited state found to exhibit antibunching. A modified Hubbard-type effective model is shown to reproduce well the microscopic CI results. This led to uncovering of analytic expressions capturing the full evolution of the two-particle momentum correlation maps over the entire range of interparticle interactions, from the independent particle limit with a substantial site-double-occupancy fraction, to the Mott insulating regime.
Identification and understanding of the evolution of interference patterns in two-particle momentum correlations as a function of the strength of interatomic interactions are important in explorations of the nature of quantum states of trapped particles. Together with the analysis of two-particle spatial correlations, they offer the prospect of uncovering fundamental symmetries and structure of correlated many-body states, as well as opening vistas into potential control and utilization of correlated quantum states as quantum-information resources. With the use of the second-order density matrix constructed via exact diagonalization of the microscopic Hamiltonian, and an analytic Hubbard-type model, we explore here the systematic evolution of characteristic interference patterns in the two-body momentum and spatial correlation maps of two entangled ultracold fermionic atoms in a double well, for the entire attractive- and repulsive-interaction range. We uncover quantum-statistics-governed bunching and antibunching, as well as interaction-dependent interference patterns, in the ground and excited states, and interpret our results in light of the Hong-Ou-Mandel interference physics, widely exploited in photon indistinguishability testing and quantum-information science.
Abstract In a recent work, Murmann et al (2015 Phys. Rev. Lett. 114 080402) have experimentally prepared and manipulated a double-well optical potential containing a pair of Fermi atoms as a possible building block of Hubbard model. Here, we carry out a detailed theoretical study on the properties of both fermionic and bosonic two-site Hubbard models with a pair of interacting atoms in a trap with a double-well structure along z -axis and a 2D harmonic confinement along the transverse directions. We consider fermions as of two-component type and bosons as of spinless as well as of two spin components. We first calculate Hubbard parameters using the finite-range interaction potentials of Jost and Kohn. In general, a finite range of interaction leads to on-site, inter-site, exchange and partial-exchange terms We show that, given the same input parameters for both bosonic and fermionic two-site Hubbard models, many of the statistical properties such as the single- and double-occupancy of a site, and the probabilities for the single-particle and pair tunneling are similar in both fermionic and bosonic cases. But, quantum entanglement and quantum fluctuations are found to be markedly different for the two cases. We discuss atom-atom entanglement in two spatial modes corresponding to the two sites of the double-well. Our results show that the entanglement of a pair of spin-half fermions is always greater than that of spinless bosons; and when the fermions are maximally entangled the fluctuation in the two-mode phase difference is largely squeezed. In contrast, spinless bosons never exhibit phase squeezing, but shows squeezing in two-mode population imbalance depending on the system parameters.
This thesis reports on the deterministic preparation of magnetically ordered states in systems of few fermionic atoms. We follow the concept of quantum simulation and use 6Li atoms in two different hyperfine states to mimic the behavior of electrons in a solidstate system. In a first experiment, we simulate the two-site Hubbard model by using two atoms in an isolated double-well potential. We prepare the two-particle ground state of this model with a fidelity exceeding 90%. By introducing strong repulsive interactions, we are able to realize a pure spin model and describe the energy spectrum with a two-site Heisenberg Hamiltonian. In a second experiment, we realize Heisenberg spin chains of up to four atoms in a single strongly-elongated trapping potential. Here, the atoms self-align along the potential axis due to strong repulsive interactions. We introduce two novel measurement techniques to identify the state of the spin chains and thereby confirm that we can deterministically prepare antiferromagnetic ground-state systems. This constitutes the first observation of quantum magnetism with fermionic atoms that exceeds nearest-neighbor correlations. Both the double-well system and the spin chains can be seen as building blocks of larger ground-state spin systems. Their deterministic preparation therefore opens up a new bottom-up approach to the experimental realization of quantum many-body systems with ultracold atoms.