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arXiv:1410.2791 · Bulletin of the American Physical Society

Measurement of the Berry Phase in a Single Solid-State Spin Qubit

Kai Zhang, Naufer Nusran, Bradley R. Slezak, Dutt, M. V. Gurudev

Published Oct 9, 2014• 4 citations
arXivHTMLPDF

Abstract

We present measurements of the Berry Phase in a single solid-state spin qubit associated with the nitrogen-vacancy center in diamond. Our results demonstrate the remarkable degree of coherent control achievable in the presence of a highly complex solid-state environment. We manipulate the spin qubit geometrically by careful application of microwave radiation that creates an effective rotating magnetic field, and observe the resulting phase via spin-echo interferometry. We find good agreement with Berry's predictions within experimental errors. We also investigated the role of the environment on the geometric phase, and observed that unlike other solid-state qubit systems, the dephasing was primarily dominated by fast radial fluctuations in the path.

DOI
10.48550/arxiv.1410.2791

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We present measurements of the Berry Phase in a single solid-state spin qubit associated with the nitrogen-vacancy center in diamond. Our results demonstrate the remarkable degree of coherent control achievable in the presence of a highly complex solid-state environment. We manipulate the spin qubit geometrically by careful application of microwave radiation that creates an effective rotating magnetic field, and observe the resulting phase via spin-echo interferometry. We find good agreement with Berry's predictions within experimental errors. We also investigated the role of the environment on the geometric phase, and observed that unlike other solid-state qubit systems, the dephasing was primarily dominated by fast radial fluctuations in the path.
In quantum information science, the phase of a wave function plays an important role in encoding information. Although most experiments in this field rely on dynamic effects to manipulate this information, an alternative approach is to use geometric phase, which has been argued to have potential fault tolerance. We demonstrated the controlled accumulation of a geometric phase, Berry's phase, in a superconducting qubit; we manipulated the qubit geometrically by means of microwave radiation and observed the accumulated phase in an interference experiment. We found excellent agreement with Berry's predictions and also observed a geometry-dependent contribution to dephasing.
While it is often thought that the geometric phase is less sensitive to fluctuations in the control fields, a very general feature of adiabatic Hamiltonians is the unavoidable dynamic phase that accompanies the geometric phase. The effect of control field noise during adiabatic geometric quantum gate operations has not been probed experimentally, especially in the canonical spin qubit system that is of interest for quantum information. We present measurement of the Berry phase and carry out adiabatic geometric phase gate in a single solid-state spin qubit associated with the nitrogen-vacancy center in diamond. We manipulate the spin qubit geometrically by careful application of microwave radiation that creates an effective rotating magnetic field, and observe the resulting Berry phase signal via spin echo interferometry. Our results show that control field noise at frequencies higher than the spin echo clock frequency causes decay of the quantum phase, and degrades the fidelity of the geometric phase gate to the classical threshold after a few (∼10) operations. This occurs inspite of the geometric nature of the state preparation, due to unavoidable dynamic contributions. We have carried out systematic analysis and numerical simulations to study the effects of the control field noise and imperfect driving waveforms on the quantum phase gate.
A controlled qubit in a rotating frame opens new opportunities to probe fundamental quantum physics, such as geometric phases in physically rotating frames, and can potentially enhance detection of magnetic fields. Realising a single qubit that can be measured and controlled during physical rotation is experimentally challenging. In this work, we demonstrate quantum control of a single nitrogen-vacancy (NV) centre within a diamond rotated at 200,000rpm, a rotational period comparable to the NV spin coherence time T2T_2T2​. We stroboscopically image individual NV centres that execute rapid circular motion in addition to rotation, and demonstrate preparation, control and readout of the qubit quantum state with lasers and microwaves. Using spin-echo interferometry of the rotating qubit, we are able to detect modulation of the NV Zeeman shift arising from the rotating NV axis and an external DC magnetic field. Our work establishes single NV qubits in diamond as quantum sensors in the physically rotating frame, and paves the way for the realisation of single-qubit diamond-based rotation sensors.
The theory of angular momentum connects physical rotations and quantum spins together at a fundamental level. Physical rotation of a quantum system will therefore affect fundamental quantum operations, such as spin rotations in projective Hilbert space, but these effects are subtle and experimentally challenging to observe due to the fragility of quantum coherence. We report on a measurement of a single-electron-spin phase shift arising directly from physical rotation, without transduction through magnetic fields or ancillary spins. This phase shift is observed by measuring the phase difference between a microwave driving field and a rotating two-level electron spin system, and it can accumulate nonlinearly in time. We detect the nonlinear phase using spin-echo interferometry of a single nitrogen-vacancy qubit in a diamond rotating at 200 000 rpm. Our measurements demonstrate the fundamental connections between spin, physical rotation, and quantum phase, and they will be applicable in schemes where the rotational degree of freedom of a quantum system is not fixed, such as spin-based rotation sensors and trapped nanoparticles containing spins.
The Nitrogen-Vacancy(NV) center has recently emerged as a powerful quantum system, combining the good coherence properties and control techniques of atomic systems with the small size and fabrication capabilities of solid-state devices. We report on a measurement of a single electron-spin phase shift arising directly from physical rotation. This phase shift is observed by measuring the phase difference in a distortion microwave frequency of 2880 MHz, and it can accumulate nonlinearly in time. Carrier rotation information can be obtained by measuring the quantum geometric phase accumulation. We demonstrate quantum control of a NV center within a specific rotation system and a rotational period comparable to the NV spin coherence time T2*. These characteristics contribute as well to make this quantum system a sensitive and compact rotation sensor.
The coherent control of spin qubits forms the basis of many applications in quantum information processing and nanoscale sensing, imaging, and spectroscopy. Such control is conventionally achieved by direct driving of the qubit transition with a resonant global field, typically at microwave frequencies. Here we introduce an approach that relies on the resonant driving of nearby environment spins, whose localized magnetic field in turn drives the qubit when the environmental spin Rabi frequency matches the qubit resonance. This concept of environmentally mediated resonance (EMR) is explored experimentally using a qubit based on a single nitrogen-vacancy (NV) center in diamond, with nearby electronic spins serving as the environmental mediators. We demonstrate EMR driven coherent control of the NV spin state, including the observation of Rabi oscillations, free induction decay, and spin echo. This technique also provides a way to probe the nanoscale environment of spin qubits, which we illustrate by acquisition of electron spin resonance spectra from single NV centers in various settings.