Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Log inSign up
Challenges
Datasets
Workspaces
Papers
Discussions
Leaderboard
Blog
Job Board
Q3AS

© 2026 Aqora Quantum S.A.S.

TermsPrivacyLegal Notice

arXiv:1410.2440 · Physical Review B

Quantum state tomography of large nuclear spins in a semiconductor quantum well: Optimal robustness against errors as quantified by condition numbers

Adam Miranowicz, Şahin Kaya Özdemir, J. Bajer, G. Yusa, Nobuyuki Imoto, Y. Hirayama, Franco Nori

Published Aug 27, 2015• 31 citations
arXivHTMLPDF

Abstract

We discuss methods of quantum state tomography for solid-state systems with a large nuclear spin $I=3/2$ in nanometer-scale semiconductors devices based on a quantum well. Due to quadrupolar interactions, the Zeeman levels of these nuclear-spin devices become nonequidistant, forming a controllable four-level quantum system (known as quartit or ququart). The occupation of these levels can be selectively and coherently manipulated by multiphoton transitions using the techniques of nuclear magnetic resonance (NMR) [Yusa et al., Nature (London) 434, 1001 (2005)]. These methods are based on an unconventional approach to NMR, where the longitudinal magnetization ${M}_{z}$ is directly measured. This is in contrast to the standard NMR experiments and tomographic methods, where the transverse magnetization ${M}_{xy}$ is detected. The robustness against errors in the measured data is analyzed by using the condition number based on the spectral norm. We propose several methods with optimized sets of rotations yielding the highest robustness against errors, as described by the condition number equal to 1, assuming an ideal experimental detection. This robustness is only slightly deteriorated, as given by the condition number equal to 1.05, for a more realistic ``noisy'' ${M}_{z}$ detection based on the standard cyclically ordered phase sequence (CYCLOPS) method.

DOI
10.1103/physrevb.92.075312

Related papers

Characterization of quantum algorithms by quantum process tomography using quadrupolar spins in solid-state nuclear magnetic resonance

Hermann Kampermann, W. S. Veeman

NMR quantum computing with qubit systems represented by nuclear spins (I=12) in small molecules in liquids has led to the most successful experimental quantum information processors so far. We use the quadrupolar spin-32 sodium nuclei of a NaNO3 single crystal as a virtual two-qubit system. The large quadrupolar coupling in comparison with the environmental interactions and the usage of strongly modulating pulses allow us to manipulate the system fast enough and at the same time keeping the decoherence reasonably slow. The experimental challenge is to characterize the "calculation" behavior of the quantum processor by process tomography which is here adapted to the quadrupolar spin system. The results of a selection of quantum gates and algorithms are presented as well as a detailed analysis of experimental results.

The Journal of Chemical Physics•Jun 1, 2005•47 citations

Grover algorithm for large nuclear spins in semiconductors

Michael Niklaus Leuenberger, Daniel Loss

We show a possible way to implement the Grover algorithm in large nuclear spins $1/2<I<~9/2$ in semiconductors. The Grover sequence is performed by means of multiphoton transitions that distribute the spin amplitude between the nuclear spin states. They are distinguishable due to the quadrupolar splitting, which makes the nuclear spin levels nonequidistant. We introduce a generalized rotating frame for an effective Hamiltonian that governs the nonperturbative time evolution of the nuclear spin states for arbitrary spin lengths I. The larger the quadrupolar splitting, the better the agreement between our approximative method using the generalized rotating frame and exact numerical calculations.

arXiv:cond-mat/0304674•Physical review. B, Condensed matter•Oct 16, 2003•47 citations

Quantum information processing by nuclear magnetic resonance on quadrupolar nuclei

B Y J Oão, T Eles, E Duardo +6 more

Nuclear magnetic resonance is viewed as an important technique for the implementation of many quantum information algorithms and protocols. Although the most straightforward approach is to use the two-level system composed of spin 1 nuclei as qubits, quadrupolar nuclei, which possess a spin greater than 1 , are being used as an alternative. In this study, we show some unique features of quadrupolar systems for quantum information processing, with an emphasis on the ability to execute efficient quantum state tomography (QST) using only global rotations of the spin system, whose performance is shown in detail. By preparing suitable states and implementing logical operations by numerically optimized pulses together with the QST method, we follow the stepwise execution of Grover’s algorithm. We also review some work in the literature concerning the relaxation of pseudo-pure states in spin 3 systems as well as its modelling in both the Redfield and Kraus formalisms. These data are used to discuss differences in the behaviour of the quantum correlations observed for two-qubit systems implemented by spin 1 and quadrupolar spin 3 systems, also presented in the literature. The possibilities and advantages of using nuclear quadrupole resonance experiments for quantum information processing are also discussed.

•Jan 1, 2015•2 citations

Quantum information processing by nuclear magnetic resonance on quadrupolar nuclei

J. Teles, Eduardo Ribeiro DeAzevedo, Jair C. C. Freitas +3 more

Nuclear magnetic resonance is viewed as an important technique for the implementation of many quantum information algorithms and protocols. Although the most straightforward approach is to use the two-level system composed of spin 1/2 nuclei as qubits, quadrupolar nuclei, which possess a spin greater than 1/2, are being used as an alternative. In this study, we show some unique features of quadrupolar systems for quantum information processing, with an emphasis on the ability to execute efficient quantum state tomography (QST) using only global rotations of the spin system, whose performance is shown in detail. By preparing suitable states and implementing logical operations by numerically optimized pulses together with the QST method, we follow the stepwise execution of Grover's algorithm. We also review some work in the literature concerning the relaxation of pseudo-pure states in spin 3/2 systems as well as its modelling in both the Redfield and Kraus formalisms. These data are used to discuss differences in the behaviour of the quantum correlations observed for two-qubit systems implemented by spin 1/2 and quadrupolar spin 3/2 systems, also presented in the literature. The possibilities and advantages of using nuclear quadrupole resonance experiments for quantum information processing are also discussed.

Philosophical Transactions of the Royal Society A Mathematical Physical and Engineering Sciences•Sep 3, 2012•15 citations

Quantum Sensing via Large Spin-Clusters in Solid-State NMR: Optimal coherence order for practical sensing

Conan Alexander, T S Mahesh

Quantum entanglement has long been recognized as an important resource for quantum sensing. In this work, we demonstrate the use of multiple-quantum solid-state NMR for quantum sensing by creating, manipulating, and detecting large clusters of correlated nuclear spins. We show that such clusters can sensitively detect pulse-width jitters in radio-frequency control fields at the level of tens of nanoseconds. By analyzing the response of high-order quantum coherences to these control-field jitters, we investigate the critical interplay between the enhanced sensitivity offered by large coherence orders, their relative distributions, and their varying susceptibility to decoherence. We further demonstrate that, even within a non-uniform distribution of coherence orders, there exists an optimal maximum coherence order that maximizes sensing efficiency. To support our interpretation, we supplement the experimental results with a simplified numerical model that estimates the corresponding quantum Fisher information. These results support the solid-state NMR platform as a valuable testbed for investigating many-body quantum metrology protocols.

quant-pharXiv:2512.00494•Physical Review A•Dec 2, 2025•0 citations

Quantum tomography for solid state qubits

Yu-xi Liu, L. F. Wei, Franco Nori

PACS. 03.65.Ta – Foundations of quantum mechanics; measurement theory. PACS. 03.65.Wj – State reconstruction, quantum tomography. Abstract. – We propose a method for the tomographic reconstruction of qubit states for a general class of solid-state systems in which the Hamiltonians are represented by spin operators, e.g., with Heisenberg-, XXZ-, or XY-type exchange interactions. We analyze the implementation of the projective operator measurements, or spin measurements, on qubit states. All the qubit states for the spin Hamiltonians can be reconstructed by using experimental data. Quantum information processing requires the effective measurement of quantum states. However, a single quantum measurement can only obtain partial information of a quantum state. The reconstruction of a quantum state requires measuring a complete set of observables on an ensemble of identically prepared copies of the system. This method called quantum state tomography [1], is very important because any unknown state can be ascertained by tomographic measurements. Moreover, the full description of qubit states can increase the accuracy of quantum operations. Tomographic measurements have been experimentally implemented for, e.g., the nuclear spin state of an NMR system [2], the electromagnetic field and photon

•Jan 1, 2004•19 citations
We discuss methods of quantum state tomography for solid-state systems with a large nuclear spin I=3/2I=3/2I=3/2 in nanometer-scale semiconductors devices based on a quantum well. Due to quadrupolar interactions, the Zeeman levels of these nuclear-spin devices become nonequidistant, forming a controllable four-level quantum system (known as quartit or ququart). The occupation of these levels can be selectively and coherently manipulated by multiphoton transitions using the techniques of nuclear magnetic resonance (NMR) [Yusa et al., Nature (London) 434, 1001 (2005)]. These methods are based on an unconventional approach to NMR, where the longitudinal magnetization Mz{M}_{z}Mz​ is directly measured. This is in contrast to the standard NMR experiments and tomographic methods, where the transverse magnetization Mxy{M}_{xy}Mxy​ is detected. The robustness against errors in the measured data is analyzed by using the condition number based on the spectral norm. We propose several methods with optimized sets of rotations yielding the highest robustness against errors, as described by the condition number equal to 1, assuming an ideal experimental detection. This robustness is only slightly deteriorated, as given by the condition number equal to 1.05, for a more realistic ``noisy'' Mz{M}_{z}Mz​ detection based on the standard cyclically ordered phase sequence (CYCLOPS) method.
NMR quantum computing with qubit systems represented by nuclear spins (I=12) in small molecules in liquids has led to the most successful experimental quantum information processors so far. We use the quadrupolar spin-32 sodium nuclei of a NaNO3 single crystal as a virtual two-qubit system. The large quadrupolar coupling in comparison with the environmental interactions and the usage of strongly modulating pulses allow us to manipulate the system fast enough and at the same time keeping the decoherence reasonably slow. The experimental challenge is to characterize the "calculation" behavior of the quantum processor by process tomography which is here adapted to the quadrupolar spin system. The results of a selection of quantum gates and algorithms are presented as well as a detailed analysis of experimental results.
We show a possible way to implement the Grover algorithm in large nuclear spins 1/2<I< 9/21/2<I<~9/21/2<I< 9/2 in semiconductors. The Grover sequence is performed by means of multiphoton transitions that distribute the spin amplitude between the nuclear spin states. They are distinguishable due to the quadrupolar splitting, which makes the nuclear spin levels nonequidistant. We introduce a generalized rotating frame for an effective Hamiltonian that governs the nonperturbative time evolution of the nuclear spin states for arbitrary spin lengths I. The larger the quadrupolar splitting, the better the agreement between our approximative method using the generalized rotating frame and exact numerical calculations.
Nuclear magnetic resonance is viewed as an important technique for the implementation of many quantum information algorithms and protocols. Although the most straightforward approach is to use the two-level system composed of spin 1 nuclei as qubits, quadrupolar nuclei, which possess a spin greater than 1 , are being used as an alternative. In this study, we show some unique features of quadrupolar systems for quantum information processing, with an emphasis on the ability to execute efficient quantum state tomography (QST) using only global rotations of the spin system, whose performance is shown in detail. By preparing suitable states and implementing logical operations by numerically optimized pulses together with the QST method, we follow the stepwise execution of Grover’s algorithm. We also review some work in the literature concerning the relaxation of pseudo-pure states in spin 3 systems as well as its modelling in both the Redfield and Kraus formalisms. These data are used to discuss differences in the behaviour of the quantum correlations observed for two-qubit systems implemented by spin 1 and quadrupolar spin 3 systems, also presented in the literature. The possibilities and advantages of using nuclear quadrupole resonance experiments for quantum information processing are also discussed.
Nuclear magnetic resonance is viewed as an important technique for the implementation of many quantum information algorithms and protocols. Although the most straightforward approach is to use the two-level system composed of spin 1/2 nuclei as qubits, quadrupolar nuclei, which possess a spin greater than 1/2, are being used as an alternative. In this study, we show some unique features of quadrupolar systems for quantum information processing, with an emphasis on the ability to execute efficient quantum state tomography (QST) using only global rotations of the spin system, whose performance is shown in detail. By preparing suitable states and implementing logical operations by numerically optimized pulses together with the QST method, we follow the stepwise execution of Grover's algorithm. We also review some work in the literature concerning the relaxation of pseudo-pure states in spin 3/2 systems as well as its modelling in both the Redfield and Kraus formalisms. These data are used to discuss differences in the behaviour of the quantum correlations observed for two-qubit systems implemented by spin 1/2 and quadrupolar spin 3/2 systems, also presented in the literature. The possibilities and advantages of using nuclear quadrupole resonance experiments for quantum information processing are also discussed.
Quantum entanglement has long been recognized as an important resource for quantum sensing. In this work, we demonstrate the use of multiple-quantum solid-state NMR for quantum sensing by creating, manipulating, and detecting large clusters of correlated nuclear spins. We show that such clusters can sensitively detect pulse-width jitters in radio-frequency control fields at the level of tens of nanoseconds. By analyzing the response of high-order quantum coherences to these control-field jitters, we investigate the critical interplay between the enhanced sensitivity offered by large coherence orders, their relative distributions, and their varying susceptibility to decoherence. We further demonstrate that, even within a non-uniform distribution of coherence orders, there exists an optimal maximum coherence order that maximizes sensing efficiency. To support our interpretation, we supplement the experimental results with a simplified numerical model that estimates the corresponding quantum Fisher information. These results support the solid-state NMR platform as a valuable testbed for investigating many-body quantum metrology protocols.
PACS. 03.65.Ta – Foundations of quantum mechanics; measurement theory. PACS. 03.65.Wj – State reconstruction, quantum tomography. Abstract. – We propose a method for the tomographic reconstruction of qubit states for a general class of solid-state systems in which the Hamiltonians are represented by spin operators, e.g., with Heisenberg-, XXZ-, or XY-type exchange interactions. We analyze the implementation of the projective operator measurements, or spin measurements, on qubit states. All the qubit states for the spin Hamiltonians can be reconstructed by using experimental data. Quantum information processing requires the effective measurement of quantum states. However, a single quantum measurement can only obtain partial information of a quantum state. The reconstruction of a quantum state requires measuring a complete set of observables on an ensemble of identically prepared copies of the system. This method called quantum state tomography [1], is very important because any unknown state can be ascertained by tomographic measurements. Moreover, the full description of qubit states can increase the accuracy of quantum operations. Tomographic measurements have been experimentally implemented for, e.g., the nuclear spin state of an NMR system [2], the electromagnetic field and photon