How to understand the order of Floquet stationary states in the presence of external bath coupling and their statistical mechanics is challenging; the answers are important for preparation and control of those Floquet states. Here, we propose a scheme to classify the statistical distribution of Floquet states for time-periodic systems which couple to an external heat bath. If an effective Hamiltonian and a system-bath coupling operator, which are all time independent, can be simultaneously obtained via a time-periodic unitary transformation, the statistical mechanics of the Floquet states is equivalent to the equilibrium statistical mechanics of the effective Hamiltonian. In the large driving frequency cases, we also show that the conditions of this theorem can be weakened to the following: The time-period part in the system Hamiltonian commutes with the system-bath coupling operator. A Floquet-Markov approach is applied to numerically compute the Floquet state occupation distribution of a bosonic chain, and the results agree with the theoretical predictions.
How to understand the order of Floquet stationary states in the presence of external bath coupling and their statistical mechanics is challenging; the answers are important for preparation and control of those Floquet states. Here, we propose a scheme to classify the statistical distribution of Floquet states for time-periodic systems which couple to an external heat bath. If an effective Hamiltonian and a system-bath coupling operator, which are all time independent, can be simultaneously obtained via a time-periodic unitary transformation, the statistical mechanics of the Floquet states is equivalent to the equilibrium statistical mechanics of the effective Hamiltonian. In the large driving frequency cases, we also show that the conditions of this theorem can be weakened to the following: The time-period part in the system Hamiltonian commutes with the system-bath coupling operator. A Floquet-Markov approach is applied to numerically compute the Floquet state occupation distribution of a bosonic chain, and the results agree with the theoretical predictions.
Although the statistical mechanics of periodically driven ("Floquet") systems in contact with a heat bath has some formal analogy with the traditional statistical mechanics of undriven systems, closer examination reveals radical differences. In Floquet systems all quasienergies epsilon_{j} can be placed in a finite frequency interval 0< or =epsilon_{j}<omega (with omega the driving frequency and variant Planck's over 2pi=1 ). Therefore, if we describe a Floquet system approximately by restricting its available state space to be spanned by a finite number N of basis states, then the number of near degeneracies ( |epsilon_{j}-epsilon_{k}|< or =delta for arbitrarily small fixed delta ) in this interval grows without limit as N is increased. As we noted in a previous paper, this leads to pathologies, including drastic changes in Floquet states, as N tends to infinity. In earlier work on Floquet systems in contact with a heat bath these difficulties were often put aside by fixing N while taking the coupling to the bath to be smaller than any quasienergy difference. This led to a simple explicit theory for the reduced density matrix, with some major differences from the usual time-independent statistical mechanics. We show that, for weak but finite coupling between system and heat bath, the accuracy of a calculation within the truncated space spanned by the N lowest energy eigenstates of the undriven system is limited, as N increases indefinitely, only by the usual Born-Markov approximation, which neglects bath memory effects. As we seek higher accuracy by increasing N , we inevitably encounter quasienergy differences smaller than the system-bath coupling. We therefore derive here the equations for the steady-state reduced density matrix without restriction on the size of quasienergy splittings. In general, this matrix is no longer diagonal in the Floquet states. We analyze, in particular, the behavior near a weakly avoided crossing, where near degeneracies of quasienergies appear. In spite of the Floquet state pathologies, the explicit form of our results for the density matrix gives a consistent prescription for the statistical mechanics of periodically driven systems in the limit as N approaches infinity.
In Floquet engineering, periodic driving is used to realize novel phases of matter that are inaccessible in thermal equilibrium. For this purpose, the Floquet theory provides us a recipe for obtaining a static effective Hamiltonian. Although many existing works have treated closed systems, it is important to consider the effect of dissipation, which is ubiquitous in nature. Understanding the interplay of periodic driving and dissipation is a fundamental problem of nonequilibrium statistical physics that is receiving growing interest because of the fact that experimental advances have allowed us to engineer dissipation in a controllable manner. In this review, we give a detailed exposition on the formalism of quantum master equations for open Floquet systems and highlight recent work investigating whether equilibrium statistical mechanics applies to Floquet states.
A periodically driven quantum system, when coupled to a heat bath, relaxes to a non-equilibrium asymptotic state. In the general situation, the retrieval of this asymptotic state presents a rather non-trivial task. It was recently shown that in the limit of an infinitesimal coupling, using the so-called rotating wave approximation (RWA), and under strict conditions imposed on the time-dependent system Hamiltonian, the asymptotic state can attain the Gibbs form. A Floquet–Gibbs state is characterized by a density matrix which is diagonal in the Floquet basis of the system Hamiltonian with the diagonal elements obeying a Gibbs distribution, being parametrized by the corresponding Floquet quasi-energies. Addressing the non-adiabatic driving regime, upon using the Magnus expansion, we employ the concept of a corresponding effective Floquet Hamiltonian. In doing so we go beyond the conventionally used RWA and demonstrate that the idea of Floquet–Gibbs states can be extended to the realistic case of a weak, although finite system-bath coupling, herein termed effective Floquet–Gibbs states.
We study probability distribution of a steady state of a periodically driven system coupled to a thermal bath by using a quantum master equation in the weak-coupling limit. It is proved that, even when the external field is strong, the probability distribution is independent of the detailed nature of the thermal bath under the following conditions: (i) the Hamiltonian of the relevant system is bounded and the period of the driving field is short, (ii) the Hamiltonians for the driving field at different times commute, and (iii) the Hamiltonians of the driving field and of the interaction between the relevant system and the thermal bath commute. It is shown that the steady state is described by the Gibbs distribution of the Floquet states of the relevant system at the temperature of the thermal bath.
For a periodically driven open quantum system, the Floquet theorem states that the time evolution operator Λ(t,0) of the system can be factorized as Λ(t,0)=D(t)eLefft with micro-motion operator D(t) possessing the same period as the external driving, and time-independent operator Leff. In this work, we extend this theorem to open systems that follow a modulated periodic evolution, in which the fast part is periodic while the slow part breaks the periodicity. We derive a factorization for the time evolution operator that separates the long time dynamics and the micro-motion for the open quantum system. High-frequency expansions for the effective evolution operator control the long time dynamics, and the micro-motion operator is also given and discussed. It may find applications in quantum engineering with open systems following modulated periodic evolution.
Time-periodic quantum systems are present all over science and technology. They have been successfully studied using Floquet theory, and a broad diversity of interesting phenomena such as coherent destruction of tunnelling, dynamical localization and creation of new phases of matter have been discovered. Furthermore, periodic driving has also been introduced as a tool for engineering novel quantum systems that have no static analogue. Besides these remarkable achievements for isolated systems, in reality, systems always interact with their surroundings. Taking the effect of the environment into account, time-periodic quantum systems have been mainly described using the Floquet-Markov approach, which consists in deriving a weak coupling master equation in the Floquet basis. In this thesis, we focus on how to overcome these standard approximations in the description of driven open quantum systems. We start by providing a general review on the topics of isolated driven systems, open quantum systems and the Floquet-Markov approach, before presenting the main results of this work. Under the effect of high-frequency driving, we provide an analytic solution to a large class of open quantum systems. Our method relies on discrete symmetries of the system-bath Hamiltonian and grants access to the time evolution operator of the full system, including bath degrees of freedom. The solution can be interpreted as the stroboscopic evolution of a family of observables under the influence of an effective static Hamiltonian. This provides a flexible simulation procedure of nontrivial Hamiltonians. The results are exemplified with the driven spin-boson model, where a coherent control of dissipation is observed. By a novel combination of Floquet theory, full counting statistics and a Markovian embedding strategy (reaction coordinate mapping), more intricate scenarios with additional driven system-environment interactions are addressed. Hereby, we can access the dynamics and thermodynamics of a periodically driven thermal machine. For the particular case where the working medium is a two-level system, we identify four different operating regimes, including a heat engine and a refrigerator. As the coupling strength is increased, their efficiency and coefficient of performance decrease and the refrigerator regime disappears. Notably, our model reproduces the setup of laser cooling of trapped ions in a specific parameter limit. Following the same combination of methods, we investigate electron pumping through a single quantum dot with periodically modulated energy and tunnelling amplitudes. In the high-frequency regime, the direction of the current can be controlled with the driving phase and a rectification effect that is exclusive to the non-Markovian character of the model is observed. In the low-frequency regime, we apply an additional transformation to view the model as three independent transport channels and observe that the coupling strength also controls the current direction. Studying charge fluctuations we validate that our model behaves as a single-electron source.