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arXiv:1409.1945 · Proceedings of the National Academy of Sciences

Dynamical phase transition in the open Dicke model

Jens Klinder, Hans Keßler, Matthias Wolke, Ludwig Mathey, Andreas Hemmerich

Published Mar 2, 2015• 343 citations
arXivHTMLPDF

Abstract

The Dicke model with a weak dissipation channel is realized by coupling a Bose-Einstein condensate to an optical cavity with ultranarrow bandwidth. We explore the dynamical critical properties of the Hepp-Lieb-Dicke phase transition by performing quenches across the phase boundary. We observe hysteresis in the transition between a homogeneous phase and a self-organized collective phase with an enclosed loop area showing power-law scaling with respect to the quench time, which suggests an interpretation within a general framework introduced by Kibble and Zurek. The observed hysteretic dynamics is well reproduced by numerically solving the mean-field equation derived from a generalized Dicke Hamiltonian. Our work promotes the understanding of nonequilibrium physics in open many-body systems with infinite range interactions.

DOI
10.1073/pnas.1417132112

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The Dicke model with a weak dissipation channel is realized by coupling a Bose-Einstein condensate to an optical cavity with ultranarrow bandwidth. We explore the dynamical critical properties of the Hepp-Lieb-Dicke phase transition by performing quenches across the phase boundary. We observe hysteresis in the transition between a homogeneous phase and a self-organized collective phase with an enclosed loop area showing power-law scaling with respect to the quench time, which suggests an interpretation within a general framework introduced by Kibble and Zurek. The observed hysteretic dynamics is well reproduced by numerically solving the mean-field equation derived from a generalized Dicke Hamiltonian. Our work promotes the understanding of nonequilibrium physics in open many-body systems with infinite range interactions.
A phase transition describes the sudden change of state in a physical system, such as the transition between a fluid and a solid. Quantum gases provide the opportunity to establish a direct link between experiment and generic models which capture the underlying physics. A fundamental concept to describe the collective matter-light interaction is the Dicke model which has been predicted to show an intriguing quantum phase transition. Here we realize the Dicke quantum phase transition in an open system formed by a Bose-Einstein condensate coupled to an optical cavity, and observe the emergence of a self-organized supersolid phase. The phase transition is driven by infinitely long-ranged interactions between the condensed atoms. These are induced by two-photon processes involving the cavity mode and a pump field. We show that the phase transition is described by the Dicke Hamiltonian, including counter-rotating coupling terms, and that the supersolid phase is associated with a spontaneously broken spatial symmetry. The boundary of the phase transition is mapped out in quantitative agreement with the Dicke model. The work opens the field of quantum gases with long-ranged interactions, and provides access to novel quantum phases.
Approaching phase boundaries in many-body systems can give rise to intriguing signatures in their excitation spectra. Here, we explore the excitation spectrum of a Bose-Einstein condensate strongly coupled to an optical cavity and pumped by an optical standing wave, which simulates the famous Dicke-Hepp-Lieb phase transition of the open Dicke model with dissipation arising due to photon leakage from the cavity. For weak dissipation, the excitation spectrum displays two strongly polaritonic modes. Close to the phase boundary, we observe an intriguing regime where the lower energetic of these modes, instead of showing the expected roton-type mode softening, is found to approach and persist at zero energy, well before the critical pump strength for the Dicke-Hepp-Lieb transition boundary is reached. Hence, a peculiar situation arises, where an excitation is possible at zero energy cost, but nevertheless no instability of the system is created.
We report on the first experimental realization of the Dicke quantum phase transition realized in the quantum motion of a Bose–Einstein condensate coupled to an optical cavity. Conceptually, the transition is driven by cavity-mediated long-range interactions, giving rise to the emergence of a self-organized supersolid phase. The Dicke phase transition, predicted in 1973, has not been demonstrated experimentally before this work, both due to fundamental and technological reasons. These challenges have been overcome in the present thesis by employing atomic momentum states of a Bose-Einstein condensate, which are coupled via two-photon Raman transitions involving a cavity photon and a free-space pump photon. This open-system implementation of the Dicke model allows to tune all relevant parameters and offers a unique detection scheme to monitor the manybody system in real time. We demonstrate that the phase transition is accompanied by a macroscopically occupied cavity field and a striking change in the atomic momentum distribution, due to spontaneous self-organization of the atomic density on a checkerboard lattice. The boundary of the transition is mapped out by scanning two parameters of the Dicke model, to reveal a phase diagram in close agreement with the model description. Two different ordered configurations are allowed in the superradiant phase, giving rise to the concept of spontaneous symmetry breaking at the phase transition. We experimentally distinguish the symmetry-broken states and study the origin of the symmetry-breaking process. The finite spatial extension of our system induces a small symmetry-breaking field which changes randomly on each experimental realization. The influence of this field is studied and shown to diminish upon dynamically crossing the transition point with increasing transition rates.
The Dicke model is a paradigmatic setting for collective light-matter physics and the superradiant phase transition. Yet extracting the critical exponents is challenging at experimentally accessible mesoscopic sizes, due to the slow divergence of the correlation time under all-to-all coupling and a photon-loss-driven crossover to a distinct dissipative universality class. Here, we perform a large-NNN analysis that identifies distinct coherent and dissipative fixed points for the closed and open Dicke models. We then develop a unified mesoscopic scaling framework that incorporates the leading irrelevant correction and, going beyond static and spectral probes, brings ramping dynamics under the same scaling description. It recovers the corresponding exponents, verifies Kibble-Zurek scaling, and clarifies how finite size, dissipation, and speed compete in the ramping dynamics. Our work thus establishes a unified framework for resolving static and dynamical critical scaling in closed and open quantum systems, with broader applicability to mesoscopic systems with long-range interactions.
The quantum phase transition of the Dicke model has been observed recently in a system formed by motional excitations of a laser-driven Bose-Einstein condensate coupled to an optical cavity [Baumann et al., Nature (London) 464, 1301 (2010)]. The cavity-based system is intrinsically open: photons leak out of the cavity where they are detected. Even at zero temperature, the continuous weak measurement of the photon number leads to an irreversible dynamics toward a steady state. In the framework of a generalized Bogoliubov theory, we show that the steady state exhibits a dynamical quantum phase transition. We find that the critical point and the mean field are only slightly modified with respect to the phase transition in the ground state. However, the critical exponents of the singular quantum correlations are significantly different in the two cases. There is also a drastic modification of the atom-field entanglement, since the divergence of the logarithmic negativity of the ground state at the critical point is suppressed and a finite entanglement is found in the steady state.