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arXiv:1405.6251 · Light Science & Applications

Complete temporal characterization of a single photon

Zhongzhong Qin, Adarsh S Prasad, Travis Brannan, Andrew MacRae, A. Lezama, Alexander I. Lvovsky

Published Jun 5, 2015• 70 citations
arXivHTMLPDF

Abstract

Precise information about the temporal mode of optical states is crucial for optimizing their interaction efficiency between themselves and/or with matter in various quantum communication devices. Here we propose and experimentally demonstrate a method of determining both the real and imaginary components of a single photon's temporal density matrix by measuring the autocorrelation function of the photocurrent from a balanced homodyne detector at multiple local oscillator frequencies. We test our method on single photons heralded from biphotons generated via four-wave mixing in an atomic vapor and obtain excellent agreement with theoretical predictions for several settings. A convenient scheme for characterizing the temporal properties of a single photon looks set to aid experiments in quantum optics. An international team of scientists from Canada, China, USA, Uruguay and Russia says that this approach can be used to determine the complete mode structure of a photon, in particular, the real and imaginary parts of its temporal density matrix. This information is important for quantum communication experiments for which it is often critical to match photon modes. The characterization scheme, which the researchers term polychromatic optical heterodyne tomography, works by collecting autocorrelation data of homodyne photocurrent at multiple local oscillator frequencies. The team says that tests of the technique with single photons generated by four-wave mixing in an atomic vapour agree well with theoretical predictions.

DOI
10.1038/lsa.2015.71

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Precise information about the temporal mode of optical states is crucial for optimizing their interaction efficiency between themselves and/or with matter in various quantum communication devices. Here we propose and experimentally demonstrate a method of determining both the real and imaginary components of a single photon's temporal density matrix by measuring the autocorrelation function of the photocurrent from a balanced homodyne detector at multiple local oscillator frequencies. We test our method on single photons heralded from biphotons generated via four-wave mixing in an atomic vapor and obtain excellent agreement with theoretical predictions for several settings. A convenient scheme for characterizing the temporal properties of a single photon looks set to aid experiments in quantum optics. An international team of scientists from Canada, China, USA, Uruguay and Russia says that this approach can be used to determine the complete mode structure of a photon, in particular, the real and imaginary parts of its temporal density matrix. This information is important for quantum communication experiments for which it is often critical to match photon modes. The characterization scheme, which the researchers term polychromatic optical heterodyne tomography, works by collecting autocorrelation data of homodyne photocurrent at multiple local oscillator frequencies. The team says that tests of the technique with single photons generated by four-wave mixing in an atomic vapour agree well with theoretical predictions.
This thesis reports the realization and applications of a versatile wideband balanced homodyne detector operating in the time domain and intended for Quantum Optical Tomography. The detector can work with high repetition rate lasers used for the production and measurement of the electric field quadratures of quantum states of light. Full characterization of the detector by shot-noise measurements and by verifying its capability to reconstruct the density matrix and Wigner function of various states of interest is given. By overcoming photodiodes response mismatch, high frequency electronics issues and by choosing an appropriate optical set-up, a high level of common mode suppression (52.4dB) and a low electronic noise gave a shot-to-electronic noise ratio of I3dB for a Local Oscillator with 6.2 x 108 photons-per-pulse on a ~ 100MHz bandwidth. Results for the characterization of a single-photon Fock state are presented. An average efficiency of 56% was obtained for the generation/detection of the state.
Quantum light is considered to be one of the key resources of the coming second quantum revolution expected to give rise to groundbreaking technologies and applications. If the spatio-temporal and polarization structure of modes is known, the properties of quantum light are well understood. This information provides the basis for contemporary quantum optics and its applications in quantum communication and metrology. However, thinking about quantum light at the most fundamental timescale, namely the oscillation cycle of a mode or the inverse frequency of an involved photon, we realize that the corresponding picture has been missing until now. For instance, how to comprehend and characterize a single photon at this timescale? To fill this gap, we demonstrate theoretically how local quantum measurements allow to reconstruct and visualize a quantum field under study at subcycle scales, even when its temporal mode structure is a priori unknown. In particular, generation and tomography of ultrabroadband squeezed states as well as photon-subtracted states derived from them are described, incorporating also single-photon states. Our results set a cornerstone in the emerging chapter of quantum physics termed time-domain quantum optics. We expect this development to elicit new spectroscopic concepts for approaching e.g. fundamental correlations and entanglement in the dynamics of quantum matter, overcoming the temporal limitation set by the oscillation cycles of both light and elementary excitations.
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We have developed a technique for dual-temporal-mode, ultrafast, time-domain, balanced homodyne detection. We have tested it by performing homodyne measurements on pairs of picosecond-duration temporal modes (or “time bins”) carrying a delocalized single photon. The experimental homodyne data have been used to reconstruct both the density matrix and the two-mode Wigner function of the delocalized state, thus showing the correlations existing between the pair of temporal modes carrying the single photon.
A single-photon Fock state has been generated by means of conditional preparation from a two-photon state emitted in the process of spontaneous parametric down-conversion. A recently developed high-frequency homodyne tomography technique has been used to completely characterize the Fock state by means of a pulse-to-pulse analysis of the detectors' difference photocurrent. The density matrix elements of the generated state have been retrieved with a final detection efficiency of about 57%. A comparison has been performed between the phase-averaged tomographic reconstructions of the Wigner function as obtained from the measured density-matrix elements and from a direct Abel transform of the homodyne data. The ability of our system to work at the full repetition rate of the pulsed laser (82MHz)(82\phantom{\rule{0.3em}{0ex}}\mathrm{MHz})(82MHz) substantially simplifies the detection scheme, allowing for more ``exotic'' quantum states to be generated and analyzed.
Ultimately the properties of all optical fields are contained in the density matrix that specifies their quantum mechanical state. It has only recently been demonstrated that it is possible to actually reconstruct this density matrix from measured data, and to do so with temporal resolution of a few hundred femtoseconds.[1] This technique, known as Optical Homodyne Tomography (OHT), is unfortunately restricted to the measurement of only single mode radiation. In fact it selects out from the test field only those components which overlap temporally with the local oscillator pulse mode.