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arXiv:1405.5612 · Physical Review A

Nonlinear atom-photon-interaction-induced population inversion and inverted quantum phase transition of Bose-Einstein condensate in an optical cavity

Xiuqin Zhao, Ni Liu, J.-Q. Liang

Published Aug 15, 2014• 26 citations
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Abstract

In this paper we explore the rich structure of macroscopic many-particle quantum states for a Bose-Einstein condensate in an optical cavity with a tunable nonlinear atom-photon interaction [K. Baumann et al., Nature (London) 464, 1301 (2010)]. Population inversion, bistable normal phases, and the coexistence of normal-superradiant phases are revealed by adjusting the experimentally realizable interaction strength and pump-laser frequency. For the negative (effective) cavity frequency we observe, remarkably, an inverted quantum phase transition (QPT) from the superradiant to the normal phases with an increase in atom-field coupling, which is just opposite the QPT in the normal Dicke model. Bistable macroscopic states are derived analytically in terms of the spin-coherent-state variational method by taking into account both normal and inverted pseudospin states.

DOI
10.1103/physreva.90.023622

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In this paper we explore the rich structure of macroscopic many-particle quantum states for a Bose-Einstein condensate in an optical cavity with a tunable nonlinear atom-photon interaction [K. Baumann et al., Nature (London) 464, 1301 (2010)]. Population inversion, bistable normal phases, and the coexistence of normal-superradiant phases are revealed by adjusting the experimentally realizable interaction strength and pump-laser frequency. For the negative (effective) cavity frequency we observe, remarkably, an inverted quantum phase transition (QPT) from the superradiant to the normal phases with an increase in atom-field coupling, which is just opposite the QPT in the normal Dicke model. Bistable macroscopic states are derived analytically in terms of the spin-coherent-state variational method by taking into account both normal and inverted pseudospin states.
We investigate the multiple stable macroscopic quantum states of a Bose-Einstein condensate in an optomechanical cavity with pump-cavity field detuning and atom-photon interaction following the experimental realization of the quantum phase transition [Nature (London) 464, 1301 (2010)]. The spin-coherent-state variational method is useful in exploring the multistability since it has the advantage of including both normal and inverted pseudospin states. In the blue detuning regime the usual transition from normal to superradiant phases still exists, however, when the atom-field coupling increases to a certain value, called the turning point, the superradiant phase collapses due to the resonant damping of the mechanical oscillator. As a consequence, the system undergoes at this point an additional phase transition to the normal phase of the atomic population inversion state. In particular, the superradiant phase disappears completely at strong photon-phonon interaction, resulting in the direct atomic population transfer between two atomic levels. Moreover, the coupling-induced collapse and revival of the superradiant state are also found in the red detuning region.
In this paper we investigate the ground-state properties and related quantum phase transitions for the two-component Bose-Einstein condensate in a single-mode optical cavity. Apart from the usual normal and superradiant phases, multi-stable macroscopic quantum states are realized by means of the spin-coherent-state variational method. We demonstrate analytically the stimulated radiation from a collective state of atomic population inversion, which does not exist in the normal Dicke model with single-component atoms. It is also revealed that the stimulated radiation can be generated only from one component of atoms and the other remains in the ordinary superradiant state. However, the order of superradiant and stimulated-radiation states is interchangeable between two components of atoms by tuning the relative atom-field couplings and the frequency detuning as well.
A link to the Dicke-model type quantum phase transition (QPT) is established by considering a time-dependent driving of the atom-field coupling and nonlinear atom-photon interaction as well, which make a notable impact on the ground-state properties. Motivated by the recent pioneer experiment [K. Baumann, C. Guerlin, F. Brennecke, and T. Esslinger, Nature (London) 464, 1301 (2010)], in this paper we demonstrate theoretically a rich multistable structure and nonequilibrium QPTs in terms of the Floquet theory and generalized rotating wave approximation. The positive nonlinear interaction does not lead to the change of the order-parameter curve except for a slight shift of the critical point. However, an additional full atomic population of the excited state is generated by the negative interaction resulting in the coexistence region of normal and superradiant phases. When both driving and nonlinear interaction exist the single order-parameter curve of the superradiant phase spreads out and a wide area of multiple local minima emerges in addition.
We investigate in this paper the macroscopic quantum states of multiple atoms in an optical cavity with non-Hermitian coupling motivated by recent experiments. The tunable atom-photon nonlinear interaction is included to demonstrate the variety of quantum phases in the realistic realization of Dicke phase transition with cold atoms. The energies of macroscopic quantum states are obtained in terms of the spin-coherent-state variational method, in which the nonunitary operator of the similarity transformation is used to diagonalize the effective non-Hermitian Hamiltonian, which is pseudo-Hermitian below the exceptional point (EP). The superradiant phase (SP) and related quantum phase transition (QPT) disappear completely for the non-Hermitian Dicke model (DM) because of imaginary coupling, which leads to instability of states with nonzero photons. The situation is dramatically changed by including the nonlinear atom-photon interaction generated by the pump field. It is found that the second EP emerges at a higher value of coupling. The spectrum is complex between the two EPs and real otherwise. Phase diagrams are obtained for red and blue cavity pump field detunings, showing explicitly the revival of the SP and QPT, respectively. However, the QPT from the SP to the normal phase with the increase of coupling is opposite to the transition in the normal DM. The critical property of the Berry phase indicates the first-order nature of the QPT, which again is different from the DM, where the QPT is known as the second order.
Dicke model, as an important many-body model in quantum optics, describes the interaction between multiple identical two-level atoms and a quantized electromagnetic field. This spin-boson model shows collective phenomena in light-matter interaction systems and can undergo a second-order quantum phase transition from a normal phase to a superradiant phase when the coupling strength between the two-level atoms and the optical field exceeds a critical value. Dicke model embodies unique many-body quantum theories. And it has been widely studied and obtained many significant research results in quantum information, quantum process, and other quantum systems. Meanwhile, Dicke model also has wide applications in quantum optics and condensed matter physics. The extended Dicke model, describing the interaction of a Bose-Einstein condensate in an optical cavity, provides a remarkable platform for studying extraordinary quantum phase transitions in theory and experiment. Based on the recent experiment on non-Hermitian coupling between two long-lived atomic spin waves in an optical cavity, in this work we use spin-coherent-state variational method and present the macroscopic quantum-state energy of the non-Hermitian Dicke model. The spin coherent state variational method has an advantage in the theoretical research of macroscopic quantum states, especially in the normal and the inverted pseudospin states. In the variational method, optical coherent states and atomic extremum spin coherent states are used as the trial wave functions. A Hermitian transformation operator is proposed to diagonalize the non-Hermitian Hamiltonian, which is different from the ordinary quantum mechanics where the transformation operator must be unitary. Herein, the energy function is not necessarily real in the entire coupling region. Beyond an exceptional point, the spectrum becomes complex and introducing biorthogonal sets of atomic extremum states is necessary to evaluate the average quantities. The normal phase (for the zero average photon number) possesses real energy and atomic population. The non-Hermitian interaction destroys the superradiant phase (for the stable nonzero average photon number) and leads to the absence of quantum phase transition. However, the introduced atom-photon interaction, which is induced by the pump field experimentally, can change the situation, dramatically. The pump field can balance the loss by the non-Hermitian atom-photon interaction to achieve the superradiant phase. An interesting double exceptional point are observed in the energy functional. There is the real spectrum below the first exceptional point and beyond the second exceptional point, while there is a complex spectrum between these two exceptional points. The superradiant phase appears only beyond a critical value, which is related to the nonlinear interaction and the pump laser. A new and inverted quantum phase transition from the superradiant phase to the normal phase, is observed by modulating the atom-field coupling strength. The superradiant phase of the population inversion state appears for a negative effective frequency and a large atom-photon interaction. The influence of the dissipative coupling may be observed in cold atom experiment in an optical cavity. All the parameters adopted in this work are the actual experimental parameters.
In this paper we reveal the rich ground-state properties induced by the strong nonlinear atom-photon interaction which has been found in the recent experiment about a Bose-Einstein condensate coupling with a high-finesse cavity [Nature (London) 464, 1301 (2010)]. Two detuning-dependent phase diagrams are revealed by investigating the experimentally measurable atomic population. In particular, two quantum phase transitions from the superradiant phase or the normal phase to a dynamically unstable phase are predicted in the blue detuning. Moreover, the three-phase coexistence points are found. It is also demonstrated that these predicted quantum phase transitions are the intrinsic transitions governed only by the second-order derivative of the ground-state energy. Finally, we also point out that the region involving coexistence of the superradiant phase and the normal phase previously predicted cannot happen in the ground state.