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arXiv:1405.5413 · Physical Review Letters

Cooperative Emission of a Coherent Superflash of Light

Chang Chi Kwong, Tao Yang, Mysore Srinivas Pramod, Kanhaiya Pandey, Dominique Delande, Romain Pierrat, David Wilkowski

Published Nov 26, 2014• 73 citations
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Abstract

We investigate the transient coherent transmission of light through an optically thick cold strontium gas. We observe a coherent superflash just after an abrupt probe extinction, with peak intensity more than three times the incident one. We show that this coherent superflash is a direct signature of the cooperative forward emission of the atoms. By engineering fast transient phenomena on the incident field, we give a clear and simple picture of the physical mechanisms at play.

DOI
10.1103/physrevlett.113.223601

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We investigate the transient coherent transmission of light through an optically thick cold strontium gas. We observe a coherent superflash just after an abrupt probe extinction, with peak intensity more than three times the incident one. We show that this coherent superflash is a direct signature of the cooperative forward emission of the atoms. By engineering fast transient phenomena on the incident field, we give a clear and simple picture of the physical mechanisms at play.
We study the coherent transmission of light through cold strontium atomic clouds, using the narrow intercombination line. In the first part of the thesis, the cooperative emission in the coherent transmission is studied experimentally. By applying fast changes to the incident probe field, flashes of light are observed in the forward direction. The peak intensity of the flashes can be much larger than the incident intensity. These flashes are called superflashes. Due to cooperative effect, the time scale of the flashes are shortened with respect to the single scatterer lifetime. By packing these flashes, we generate a pulse train with short repetition time, where the dynamics can almost be fully governed by cooperative effect. The effect of atomic density on the coherent transmission of light is also studied theoretically and numerically. The effective refractive index of the cloud is calculated up to the second order in atomic density. It is eventually validated with a numerical simulation of the coherent light transmission. The second part of the thesis focuses on the effect of magnetic field on the coherent transmission of light. The strontium intercombination line has a sensitivity in the milligauss regime, which is the typical value of stray magnetic field in the lab. An active magnetic field control system is implemented to cancel the low frequency and AC 50~Hz stray magnetic field. Using this control system, we study the nonlinear magneto-optical rotation (NMOR) effect due to a high intensity light field transmitting through a dilute and thin cloud of strontium atom. Interestingly, at sufficiently high cloud temperature, the NMOR effect can have a higher sensitivity to the magnetic field, compared to its linear counterpart at the same cloud temperature.
An optically thick cold atomic cloud emits a coherent flash of light in the forward direction when the phase of an incident probe field is abruptly changed. Because of cooperativity, the duration of this phenomena can be much shorter than the excited lifetime of a single atom. Repeating periodically the abrupt phase jump, we generate a train of pulses with short repetition time, high intensity contrast, and high efficiency. In this regime, the emission is fully governed by cooperativity even if the cloud is dilute.
We present a theoretical and experimental analysis of transient optical properties of a dense cold atomic gas. After the rapid extinction of a weak coherent driving field (mean photon number ∼1.5\sim 1.5∼1.5), a transient `flash' is observed. Surprisingly the decay of the `flash' is faster than the decay of the fastest superradiant mode of the system. We show that this `faster than superradiance decay' is expected due to the interference between collective eigenmodes that exhibit a range of frequency shifts away from the bare atomic transition. Experimental results confirm that the initial decay rate of the superradiant flash increases with optical depth, in agreement with the numerical simulations for the experimental conditions.
We use coherent backscattering of light by cold strontium atoms to study phase-breaking mechanisms in the multiple-scattering regime. As the probe light intensity is increased, the atomic optical transition starts to be saturated. Nonlinearities and inelastic scattering then occur. The latter induces a characteristic phase-breaking time that reduces the wave coherence. In our experiment, this leads to a strong reduction of the enhancement factor of the coherent backscattering cone. The results at different probe detuning are also presented.