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arXiv:1404.5721 · Physical Review Letters

Topological Mott Insulator in Three-Dimensional Systems with Quadratic Band Touching

Igor F. Herbut, Lukas Janssen

Published Sep 2, 2014• 147 citations
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Abstract

We argue that a three-dimensional electronic system with the Fermi level at the quadratic band touching point such as HgTe could be unstable with respect to the spontaneous formation of the (topological) Mott insulator at arbitrary weak long-range Coulomb interaction. The mechanism of the instability can be understood as the collision of Abrikosov's non-Fermi liquid fixed point with another, quantum critical, fixed point, which approaches it in the coupling space as the system's dimensionality $d\ensuremath{\rightarrow}{d}_{\text{low}}+$, with the ``lower critical dimension'' $2<{d}_{\text{low}}<4$. Arguments for the existence of the quantum critical point based on considerations in the large-$N$ limit in $d=3$, as well as close to $d=2$, are given. In the one-loop calculation we find that ${d}_{\text{low}}=3.26$, and thus above, but not far from three dimensions. This translates into a temperature or energy window (${T}_{\mathrm{c}}$, ${T}_{*}$) over which the non-Fermi liquid scaling should still be observable, before the Mott transition finally takes place at the critical temperature ${T}_{\mathrm{c}}\ensuremath{\sim}{T}_{*}\mathrm{exp}[\ensuremath{-}zC/({d}_{\text{low}}\ensuremath{-}d{)}^{1/2}]$. We estimate $C=\ensuremath{\pi}/1.1$, dynamical critical exponent $z\ensuremath{\approx}1.8$, and the temperature scale ${k}_{B}{T}_{*}\ensuremath{\approx}(4m/{m}_{\text{el}}{ϵ}^{2})13.6\text{ }\text{ }\mathrm{eV}$, with $m$ as the band mass and $ϵ$ as the dielectric constant.

DOI
10.1103/physrevlett.113.106401

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We argue that a three-dimensional electronic system with the Fermi level at the quadratic band touching point such as HgTe could be unstable with respect to the spontaneous formation of the (topological) Mott insulator at arbitrary weak long-range Coulomb interaction. The mechanism of the instability can be understood as the collision of Abrikosov's non-Fermi liquid fixed point with another, quantum critical, fixed point, which approaches it in the coupling space as the system's dimensionality d\ensuremath→dlow+d\ensuremath{\rightarrow}{d}_{\text{low}}+d\ensuremath→dlow​+, with the ``lower critical dimension'' 2<dlow<42<{d}_{\text{low}}<42<dlow​<4. Arguments for the existence of the quantum critical point based on considerations in the large-NNN limit in d=3d=3d=3, as well as close to d=2d=2d=2, are given. In the one-loop calculation we find that dlow=3.26{d}_{\text{low}}=3.26dlow​=3.26, and thus above, but not far from three dimensions. This translates into a temperature or energy window (Tc{T}_{\mathrm{c}}Tc​, T∗{T}_{*}T∗​) over which the non-Fermi liquid scaling should still be observable, before the Mott transition finally takes place at the critical temperature Tc\ensuremath∼T∗exp[\ensuremath−zC/(dlow\ensuremath−d)1/2]{T}_{\mathrm{c}}\ensuremath{\sim}{T}_{*}\mathrm{exp}[\ensuremath{-}zC/({d}_{\text{low}}\ensuremath{-}d{)}^{1/2}]Tc​\ensuremath∼T∗​exp[\ensuremath−zC/(dlow​\ensuremath−d)1/2]. We estimate C=\ensuremathπ/1.1C=\ensuremath{\pi}/1.1C=\ensuremathπ/1.1, dynamical critical exponent z\ensuremath≈1.8z\ensuremath{\approx}1.8z\ensuremath≈1.8, and the temperature scale kBT∗\ensuremath≈(4m/melϵ2)13.6  eV{k}_{B}{T}_{*}\ensuremath{\approx}(4m/{m}_{\text{el}}{ϵ}^{2})13.6\text{ }\text{ }\mathrm{eV}kB​T∗​\ensuremath≈(4m/mel​ϵ2)13.6  eV, with mmm as the band mass and ϵϵϵ as the dielectric constant.
We construct and discuss the field theory for tensorial nematic order parameter coupled to gapless four-component fermions at the quadratic band touching point in three (spatial) dimensions. Within a properly formulated epsilon-expansion this theory is found to have a quantum critical point, which describes the (presumably continuous) transition from the semimetal into a (nematic) Mott insulator. The latter phase breaks the rotational, but not the time-reversal, symmetry and may be relevant to materials such as gray tin or mercury telluride at low temperatures. The critical point represents a simple quantum analog of the familiar classical isotropic-to-nematic transition in liquid crystals. The properties and the consequences of this quantum critical point are discussed. Its existence supports the scenario of the ``fixed-point collision,'' according to which three-dimensional Fermi systems with quadratic band touching and long-range Coulomb interactions are unstable towards the gapped nematic ground state at low temperatures.
At low temperatures, isotropic two-dimensional Fermi systems with quadratic band touching are unstable with respect to a symmetry-broken ground state when interactions are taken into account. Here, the authors demonstrate that in a setup with threefold symmetry only - as realized, for instance, in bilayer graphene - interactions induce a splitting of the quadratic band touching into four Dirac cones. This shifts the instability to a finite interaction strength and leads to a quantum critical point with emergent Lorentz invariance.
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The rearrangement of the Fermi surface in a diluted two-dimensional electron gas beyond the topological quantum critical point has been examined within an approach based on the Landau theory of Fermi liquid and a nonperturbative functional method. The possibility of a transition of the first order in the coupling constant at zero temperature between the states with a three-sheet Fermi surface and a transition of the first order in temperature between these states at a fixed coupling constant has been shown. It has also been shown that a topological crossover, which is associated with the joining of two sheets of the Fermi surface and is characterized by the maxima of the density of states N(T) and ratio C(T)/T of the specific heat to the temperature, occurs at a very low temperature T ⋄ determined by the structure of a state with the three-sheet Fermi surface. A momentum region where the distribution n(p, T) depends slightly on the temperature, which is manifested in the maximum of the specific heat C(T) near T *, appears through a crossover at temperatures T ∼ T * > T ⋄. It has been shown that the flattening of the single-particle spectrum of the strongly correlated two-dimensional electron gas results in the crossover from the Fermi liquid behavior to a non-Fermi liquid one with the density of states N(T) ∝ T −α with the exponent α }~ 2/3.
We investigate the interplay of Coulomb interactions and short-range-correlated disorder in three-dimensional systems where absent disorder the noninteracting band structure hosts a quadratic band crossing. Though the clean Coulomb problem is believed to host a non-Fermi liquid phase, disorder and Coulomb interactions have the same scaling dimension in a renormalization group (RG) sense, and thus should be treated on an equal footing. We therefore implement a controlled $\ensuremath{\varepsilon}$ expansion and apply it at leading order to derive RG flow equations valid when disorder and interactions are both weak. We find that the non-Fermi liquid fixed point is unstable to disorder, and demonstrate that the problem inevitably flows to strong coupling, outside the regime of applicability of the perturbative RG. An examination of the flow to strong coupling suggests that disorder is asymptotically more important than interactions, so that the low-energy behavior of the system can be described by a noninteracting sigma model in the appropriate symmetry class (which depends on whether exact particle-hole symmetry is imposed on the problem). We close with a discussion of general principles unveiled by our analysis that dictate the interplay of disorder and Coulomb interactions in gapless semiconductors, and of connections to many-body localized systems with long-range interactions.
Understanding correlation effects in topological phases and their transitions is a cutting-edge area of research in recent condensed matter physics. We study topological quantum phase transitions (TQPTs) between double-Weyl semimetals (DWSMs) and insulators, and argue that a novel class of quantum criticality appears at the TQPT characterized by emergent anisotropic non-Fermi-liquid behaviors, in which the interplay between the Coulomb interaction and electronic critical modes induces not only anisotropic renormalization of the Coulomb interaction but also strongly correlated electronic excitation in three spatial dimensions. Using the standard renormalization group methods, large N_{f} theory, and the ε=4-d method with a fermion flavor number N_{f} and spatial dimension d, we obtain the anomalous dimensions of electrons (η_{f}=0.366/N_{f}) in large N_{f} theory and the associated anisotropic scaling relations of various physical observables. Our results may be observed in candidate materials for DWSMs such as HgCr_{2}Se_{4} or SrSi_{2} when the system undergoes a TQPT.