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arXiv:1404.5124 · International Journal of Modern Physics B

Generic model for Cooper pair splitting

Henning Soller

Published May 30, 2014• 3 citations
arXivHTMLPDF

Abstract

A superconductor connected to normal leads allows to generate Einstein–Podolsky–Rosen pairs by Cooper pair splitting (CPS). It has been realized with quantum dots either defined in carbon nanotubes or InAs nanowires. After establishing the presence of CPS in such devices new works have investigated the effects of a finite potential difference between the quantum dots to improve and characterize the efficiency of CPS. In this paper, we present a generic model for CPS and develop two minimal models specifically for the two experimental realizations and compare them to the experimental data. In addition, we also explore the relation of nonlocal charge transfer to positive current cross-correlation of currents and discuss the temperature dependence of CPS.

DOI
10.1142/s0217979214501379

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A superconductor connected to normal leads allows to generate Einstein–Podolsky–Rosen pairs by Cooper pair splitting (CPS). It has been realized with quantum dots either defined in carbon nanotubes or InAs nanowires. After establishing the presence of CPS in such devices new works have investigated the effects of a finite potential difference between the quantum dots to improve and characterize the efficiency of CPS. In this paper, we present a generic model for CPS and develop two minimal models specifically for the two experimental realizations and compare them to the experimental data. In addition, we also explore the relation of nonlocal charge transfer to positive current cross-correlation of currents and discuss the temperature dependence of CPS.
In a device with a superconductor coupled to two parallel quantum dots (QDs) the electrical tunability of the QD levels can be used to exploit nonclassical current correlations due to the splitting of Cooper pairs. We experimentally investigate the effect of a finite potential difference across one quantum dot on the conductance through the other completely grounded QD in a Cooper pair splitter fabricated on an InAs nanowire. We demonstrate that the nonlocal electrical transport through the device can be tuned by electrical means and that the energy dependence of the effective density of states in the QDs is relevant for the rates of Cooper pair splitting (CPS) and elastic cotunneling. Such experimental tools are necessary to understand and develop CPS-based sources of entangled electrons in solid-state devices.
The two electrons of a Cooper pair in a conventional superconductor form a spin singlet and therefore a maximally entangled state. Recently, it was demonstrated that the two particles can be extracted from the superconductor into two spatially separated contacts via two quantum dots in a process called Cooper pair splitting (CPS). Competing transport processes, however, limit the efficiency of this process. Here we demonstrate efficiencies up to 90%, significantly larger than required to demonstrate interaction-dominated CPS, and on the right order to test Bell's inequality with electrons. We compare the CPS currents through both quantum dots, for which large apparent discrepancies are possible. The latter we explain intuitively and in a semiclassical master equation model. Large efficiencies are required to detect electron entanglement and for prospective electronics-based quantum information technologies.
Entanglement, being at the heart of the Einstein-Podolsky-Rosen (EPR) paradox, is a necessary ingredient in processing quantum information. Cooper pairs in superconductors - being composites of two fully entangled electrons - can be split adiabatically, thus forming entangled electrons. We fabricated such electron splitter by contacting an aluminum superconductor strip at the center of a suspended InAs nanowire; terminated at both ends with two normal metallic drains. Intercepting each half of the nanowire by gate - induced Coulomb blockaded quantum dot strongly impeded the flow of Cooper pairs due to large charging energy, while still permitting passage of single electrons. Here, we provide conclusive evidence of extremely high efficiency Cooper pairs splitting via observing positive average (conductance) and time (shot noise) correlations of the split electrons in the two opposite drains of the nanowire. Moreover, The actual charge of the injected quasiparticles was verified by shot noise measurements.
A Cooper pair splitter consists of two quantum dots side-coupled to a conventional superconductor. Usually, the quantum dots are assumed to have a large charging energy compared to the superconducting gap, in order to suppress processes other than the coherent splitting of Cooper pairs. In this work, in contrast, we investigate the limit in which the charging energy is smaller than the superconducting gap. This allows us, in particular, to study the effect of a Zeeman field comparable to the charging energy. We find analytically that in this parameter regime the superconductor mediates an interdot tunneling term with a spin symmetry determined by the Zeeman field. Together with electrostatically tunable quantum dots, we show that this makes it possible to engineer a spin triplet state shared between the quantum dots. Compared to previous works, we thus extend the capabilities of the Cooper pair splitter to create entangled nonlocal electron pairs.
A split Cooper pair is a natural source for entangled electrons which is a basic ingredient for quantum information in the solid state. We report an experiment on a superconductor-graphene double quantum dot (QD) system, in which we observe Cooper pair splitting (CPS) up to a CPS efficiency of ∼10%. With bias on both QDs, we are able to detect a positive conductance correlation across the two distinctly decoupled QDs. Furthermore, with bias only on one QD, CPS and elastic cotunneling can be distinguished by tuning the energy levels of the QDs to be asymmetric or symmetric with respect to the Fermi level in the superconductor.
Abstract Entanglement of electrons is studied by means of current–current correlations in two Cooper pair splitter devices: with one and two proximized quantum dots (1QD and 2QD), in presence of intra- and inter-dot Coulomb interactions, and weakly coupled with metallic electrodes. The 1QD system, where Cooper pairs can be transmitted to the same or split to different normal electrodes, is contrasted with the 2QD device, where double occupancy of a single quantum dot is forbidden and transport is only through an inter-dot singlet due to non-local crossed Andreev reflection processes deep in the superconducting energy gap. Separating the current correlation function into components for partial currents of electrons and holes through various Andreev bound states, one can see bunching and antibunching of split particles: inter-level components between electron and hole currents flowing to different electrodes are positive, while intra-level electron–electron or hole–hole components are negative, respectively. Spectral decomposition of the frequency-dependent current cross-correlation is performed to get better insight into mechanisms of entanglement and dynamics of split Cooper pairs, and to extract various charge fluctuation processes with different relaxation times, related to electron and hole currents flowing through the Andreev bound states. Only low frequency polarization fluctuations are seen in the current cross-correlations, while various negative and positive high frequency (charge fluctuations) components compensate each other in the symmetric system.