arXiv:1404.3967

On-chip resonantly-driven quantum emitter with enhanced coherence

M. N. Makhonin, J. Dixon, R. J. Coles, Benjamin Royall, Edmund Clarke, Maurice S. Skolnick, A. M. Fox

Published Apr 15, 2014• 2 citations

Abstract

Advances in nanotechnology provide techniques for the realisation of integrated quantum-optical circuits for on-chip quantum information processing(QIP). The indistinguishable single photons, required for such devices can be generated by parametric down-conversion, or from quantum emitters such as colour centres and quantum dots(QDs). Among these, semiconductor QDs offer distinctive capabilities including on-demand operation, coherent control, frequency tuning and compatibility with semiconductor nanotechnology. Moreover, the coherence of QD photons can be significantly enhanced in resonance fluorescence(RF) approaching at its best the coherence of the excitation laser. However, the implementation of QD RF in scalable on-chip geometries remains challenging due to the need to suppress stray laser photons. Here we report on-chip QD RF coupled into a single-mode waveguide with negligible resonant laser background and show that the coherence is enhanced compared to off-resonant excitation. The results pave the way to a novel class of integrated quantum-optical devices for on-chip QIP with embedded resonantly-driven quantum emitters.

DOI: 10.48550/arxiv.1404.3967

Related papers

Waveguide Coupled Resonance Fluorescence from On-Chip Quantum Emitter

M. N. Makhonin, J. Dixon, R. J. Coles +6 more

Resonantly driven quantum emitters offer a very promising route to obtain highly coherent sources of single photons required for applications in quantum information processing (QIP). Realizing this for on-chip scalable devices would be important for scientific advances and practical applications in the field of integrated quantum optics. Here we report on-chip quantum dot (QD) resonance fluorescence (RF) efficiently coupled into a single-mode waveguide, a key component of a photonic integrated circuit, with a negligible resonant laser background and show that the QD coherence is enhanced by more than a factor of 4 compared to off-resonant excitation. Single-photon behavior is confirmed under resonant excitation, and fast fluctuating charge dynamics are revealed in autocorrelation g((2)) measurements. The potential for triggered operation is verified in pulsed RF. These results pave the way to a novel class of integrated quantum-optical devices for on-chip quantum information processing with embedded resonantly driven quantum emitters.

Nano LettersNov 10, 201495 citations

Enhanced indistinguishability of in-plane single photons by resonance fluorescence on an integrated quantum dot

Sokratis Kalliakos, Yarden Brody, Anthony J. Bennett +6 more

Integrated quantum light sources in photonic circuits are envisaged as the building blocks of future on-chip architectures for quantum logic operations. While semiconductor quantum dots have been proven to be the highly efficient emitters of quantum light, their interaction with the host material induces spectral decoherence, which decreases the indistinguishability of the emitted photons and limits their functionality. Here, we show that the indistinguishability of in-plane photons can be greatly enhanced by performing resonance fluorescence on a quantum dot coupled to a photonic crystal waveguide. We find that the resonant optical excitation of an exciton state induces an increase in the emitted single-photon coherence by a factor of 15. Two-photon interference experiments reveal a visibility of 0.80 ± 0.03, which is in good agreement with our theoretical model. Combined with the high in-plane light-injection efficiency of photonic crystal waveguides, our results pave the way for the use of this system for the on-chip generation and transmission of highly indistinguishable photons.

Applied Physics LettersOct 10, 201621 citations

Purcell-Enhanced and Indistinguishable Single-Photon Generation from Quantum Dots Coupled to On-Chip Integrated Ring Resonators

Łukasz Dusanowski, Dominik Köck, Eunso Shin +3 more

Integrated photonic circuits provide a versatile toolbox of functionalities for advanced quantum optics applications. Here, we demonstrate an essential component of such a system in the form of a Purcell-enhanced single-photon source based on a quantum dot coupled to a robust on-chip integrated resonator. For that, we develop GaAs monolithic ring cavities based on distributed Bragg reflector ridge waveguides. Under resonant excitation conditions, we observe an over 2-fold spontaneous emission rate enhancement using Purcell effect and gain a full coherent optical control of a QD-two-level system via Rabi oscillations. Furthermore, we demonstrate an on-demand single-photon generation with strongly suppressed multiphoton emission probability as low as 1% and two-photon interference with visibility up to 95%. This integrated single-photon source can be readily scaled up, promising a realistic pathway for scalable on-chip linear optical quantum simulation, quantum computation, and quantum networks.

arXiv:2007.12920Nano LettersJul 24, 202067 citations

The resonance fluorescence of single semiconductor quantum dots for the generation of indistinguishable photons.

Carole Diederichs

Single semiconductor quantum dots, which are considered as two-level systems in the artificial atom model, are promising structures for the realization of integrated devices such as single photon sources for quantum information applications. However, contrary to genuine atoms, they are condensed matter systems which suffer from the coupling to their solid environment, leading to a degradation of the coherence of the emitted photons. One possibility to avoid this coupling, thereby improving the coherence of the photons until the one imposed by the radiative limit T2 = 2T1, is to perform strictly resonant excitation of a quantum dot at low temperature. Using an experimental setup that spatially decouples the excitation and detection paths, we showed that a fine control of the electrostatic environment related to the nanostructures residual doping remains a major challenge to answer the widely encountered problem of the inhibition of the resonance fluorescence of a quantum dot. Meanwhile, thanks to quantum optics experiments and high resolution optical spectroscopy, we demonstrated that the resonant Rayleigh scattering regime where quantum dots emit single photons with the laser coherence time, paves the way to the development of "ultra-coherent" sources of single photons with high degrees of indistinguishability. In this regime where the laser tailors the coherence of the photons and where the radiative limit becomes a secondary requirement, two photons emitted successively by the same quantum dot are indistinguishable on time scales never obtained before for a solid nano-emitter (up to ten nanoseconds, comparing to the carriers lifetime and decoherence time of about a hundred of picoseconds).

Dec 7, 20162 citations

A programmable quantum photonic platform integrating coherent emitters

Hanna Salamon, Mikkel T. Mikkelsen, Zhe Liu +4 more

Photonic quantum technologies require the integration of high-quality quantum light sources with programmable photonic circuitry to enable on-chip quantum information processing. Semiconductor quantum dots have emerged as a leading platform for quantum light generation, yet their monolithic integration with cryogenic-compatible, programmable photonic circuitry remains challenging. Here we demonstrate a programmable quantum photonic platform that enables simultaneous control of highly coherent quantum dot-based single photon emitters and reconfigurable optical elements at cryogenic temperatures. System-level integration enables individual electrical and optical addressing of active components on a single chip, allowing their concurrent operation while preserving coherent non-classical light emission. We demonstrate multiple quantum-photonic functionalities, including pure single-photon generation, two-photon interference, and resonant transmission and reflection measurements of integrated emitters. These results mark a step from isolated quantum-optical devices towards programmable quantum-photonic hardware platforms capable of combining coherent quantum emitters with large-scale photonic functionality.

quant-pharXiv:2610.06451Oct 6, 20260 citations

Photonic-circuited resonance fluorescence of single molecules with an ultrastable lifetime-limited transition

Penglong Ren, Shangming Wei, Weixi Liu +6 more

Resonance fluorescence as the emission of a resonantly-excited two-level quantum system promises indistinguishable single photons and coherent high-fidelity quantum-state manipulation of the matter qubit, which underpin many quantum information processing protocols. Real applications of the protocols demand high degrees of scalability and stability of the experimental platform, and thus favor quantum systems integrated on one chip. However, the on-chip solution confronts several formidable challenges compromising the scalability prospect, such as the randomness, spectral wandering and scattering background of the integrated quantum systems near heterogeneous and nanofabricated material interfaces. Here we report an organic-inorganic hybrid integrated quantum photonic platform that circuits background-free resonance fluorescence of single molecules with an ultrastable lifetime-limited transition. Our platform allows a collective alignment of the dipole orientations of many isolated molecules with the photonic waveguide. We demonstrate on-chip generation, beam splitting and routing of resonance-fluorescence single photons with a signal-to-background ratio over 3000 in the waveguide at the weak excitation limit. Crucially, we show the photonic-circuited single molecules possess a lifetime-limited-linewidth transition and exhibit inhomogeneous spectral broadenings of only about 5% over hours' measurements. These findings and the versatility of our platform pave the way for scalable quantum photonic networks.

Nature CommunicationsJul 9, 202223 citations