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arXiv:1404.2859 · Physical Review B

Ubiquity of linear resistivity at intermediate temperature in bad metals

G. R. Boyd, V. Zlatić, James K. Freericks

Published Feb 20, 2015• 3 citations
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Abstract

Bad metals display transport behavior that differs from what is commonly seen in ordinary metals. One of the most significant differences is a resistivity that is linear in temperature and rises to well above the Ioffe-Regel limit (where the mean-free path is equal to the lattice spacing). Using an exact Kubo formula, we show that a linear resistivity naturally occurs for many systems when they are in an incoherent intermediate-temperature state. First, we provide a simple analytic model to give intuition for this phenomenology. Then, we verify the analytic arguments with numerical calculations for a simplified version of the Hubbard model which is solved with dynamical mean-field theory. Similar features have also been seen in Hubbard models, where they can begin at even lower temperatures due to the formation of resilient quasiparticles.

DOI
10.1103/physrevb.91.075118

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Bad metals display transport behavior that differs from what is commonly seen in ordinary metals. One of the most significant differences is a resistivity that is linear in temperature and rises to well above the Ioffe-Regel limit (where the mean-free path is equal to the lattice spacing). Using an exact Kubo formula, we show that a linear resistivity naturally occurs for many systems when they are in an incoherent intermediate-temperature state. First, we provide a simple analytic model to give intuition for this phenomenology. Then, we verify the analytic arguments with numerical calculations for a simplified version of the Hubbard model which is solved with dynamical mean-field theory. Similar features have also been seen in Hubbard models, where they can begin at even lower temperatures due to the formation of resilient quasiparticles.
Bad metals exhibit approximately TTT-linear dc resistivity beyond the Ioffe--Regel limit. That this behavior occurs in systems with radically different ground states suggests it is a generic manifestation of strong local correlations. We test this hypothesis in the infinite-UUU Hubbard model with small hole densities using exact diagonalization to compute thermodynamic and transport properties of finite clusters. Upon cooling, we find an intermediate temperature range, an electronic analogue of the ``semi-quantum regime'' of liquid helium, in which quantum effects produce a roughly TTT-independent compressibility, yet the resistivity is TTT-linear and exceeds the Ioffe--Regel limit. Entry into this regime is accompanied by the formation of quasi-local ferromagnetic ``spin cages'' around doped holes, regions that facilitate local quantum motion embedded in a fluctuating spin background, analogous to the transient crystalline cages thought to control incoherent transport in semi-quantum liquid helium. Remarkably, despite the simplicity of the model, the bad metal behavior found here resembles that seen in various material platforms.
Strongly correlated metals often display anomalous transport, including T-linear resistivity above the Mott-Ioffe-Regel limit. We introduce a tractable microscopic model for bad metals, by restoring in the well-known Hubbard model-with hopping t and on-site repulsion U-a "screened Coulomb" interaction between charge densities that decays exponentially with spatial separation. This interaction lifts the extensive degeneracy in the spectrum of the t=0 Hubbard model, allowing us to fully characterize the small t electric, thermal, and thermoelectric transport in our strongly correlated model. Throughout the phase diagram we observe T-linear resistivity above the Mott-Ioffe-Regel limit, together with strong violation of the Wiedemann-Franz law and a large thermopower that can undergo sign change.
We report the discovery of phenomena consistent with bad-metal relaxation dynamics in the metallic regime of an optical-lattice Hubbard model. The transport lifetime induced by inter-particle scattering for a mass current of atoms excited by stimulated Raman transitions is measured, and the corresponding analog of resistivity is inferred. By exploring a range of temperature, we demonstrate incompatibility with weak-scattering theory and a key characteristic of bad metals: anomalous resistivity scaling consistent with TTT-linear behavior. We also observe the onset of two behaviors---incoherent transport and the approach to the Mott-Ioffe-Regel limit---associated with bad metals. The interaction and temperature scaling of resistivity are verified to be consistent with dynamic mean-field theory (DMFT) predictions of a bad metal, which is associated with the reduction of quasiparticle weight by strong interactions.
Strange or bad metallic transport, defined by incompatibility with the conventional quasiparticle picture, is a theme common to many strongly correlated materials, including high-temperature superconductors. The Hubbard model represents a minimal starting point for modeling strongly correlated systems. Here we demonstrate strange metallic transport in the doped two-dimensional Hubbard model using determinantal quantum Monte Carlo calculations. Over a wide range of doping, we observe resistivities exceeding the Mott-Ioffe-Regel limit with linear temperature dependence. The temperatures of our calculations extend to as low as 1/40 of the noninteracting bandwidth, placing our findings in the degenerate regime relevant to experimental observations of strange metallicity. Our results provide a foundation for connecting theories of strange metals to models of strongly correlated materials.
Quantum simulations are quickly becoming an indispensable tool for studying particle transport in correlated lattice models. One of the central topics in the study of transport is bad-metal behavior, characterized by the direct-current resistivity linear in temperature. In the fermionic Hubbard model, optical conductivity has been studied extensively, and a recent optical lattice experiment demonstrated bad-metal behavior in qualitative agreement with theory. Far less is known about transport in the bosonic Hubbard model. We investigate the conductivity in the Bose-Hubbard model and focus on the regime of strong interactions and high temperatures. We use numerically exact calculations for small lattice sizes. At weak tunneling, we find multiple peaks in the optical conductivity that stem from the Hubbard bands present in the many-body spectrum. This feature slowly washes out as the tunneling rate gets stronger. At high temperature, we identify a regime of TTT-linear resistivity, as expected. When the interactions are very strong, the leading inverse-temperature coefficient in conductivity is proportional to the tunneling amplitude. As the tunneling becomes stronger, this dependence takes quadratic form. At very strong coupling and half filling, we identify a separate linear resistivity regime at lower temperature, corresponding to the hard-core boson regime. Additionally, we unexpectedly observe that at half filling, in a big part of the phase diagram, conductivity is an increasing function of the coupling constant before it saturates at the hard-core-boson result. We explain this feature based on the analysis of the many-body energy spectrum and the contributions to conductivity of individual eigenstates of the system.
Using determinant quantum Monte Carlo simulations, we compare charge transport in the two-dimensional attractive and repulsive Hubbard models at strong coupling, ∣U∣/t=6|U|/t=6∣U∣/t=6. Although the interaction with opposite signs generates qualitatively different low-energy spin, charge, and pairing correlations, both exhibit approximately linear-in-temperature resistivity over a broad intermediate- and high-temperature regime. At asymptotically high temperature this common behavior follows from the moment expansion of the conductivity, whose leading contribution is even in UUU. More strikingly, the similarity persists to temperatures well below ∣U∣|U|∣U∣, where strong interaction-dependent correlations have already developed, and also irrespective of whether resistivity crosses the MIR limit. Using the Nernst--Einstein relation, we find that the common linear-in-temperature resistivity is primarily associated with an approximately Curie-like charge compressibility and weakly temperature-dependent diffusivity. The two models separate only at lower temperatures, where the attractive model develops a pronounced feature in the charge diffusivity correlated with signatures of pair formation. These results show that linear-in-temperature incoherent transport in the Hubbard model can be remarkably insensitive to the microscopic nature of the low-energy correlations. Our results suggest that transport in the incoherent regime appears insensitive to what the system will ultimately become at low temperature; the distinction between competing low-energy states becomes visible only when their characteristic correlations acquire sufficiently long spatial or temporal coherence.