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arXiv:1404.1437 · Physical Review A

Jaynes-Cummings dynamics in mesoscopic ensembles of Rydberg-blockaded atoms

Ilya I. Beterov, Tomas Andrijauskas, Denis B. Tretyakov, Vasily M. Entin, Elena A. Yakshina, I. I. Ryabtsev, S. Bergamini

Published Oct 20, 2014• 10 citations
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Abstract

We show that Jaynes-Cummings dynamics can be observed in mesoscopic atomic ensembles interacting with a classical electromagnetic field in the regime of a Rydberg blockade where the time dynamics of the average number of Rydberg excitations in mesoscopic ensembles displays collapses and revivals typical of this model. As the frequency of Rabi oscillations between collective states of Rydberg-blockaded ensembles depends on the number of interacting atoms, for randomly loaded optical dipole traps, we predict collapses and revivals of Rabi oscillations. We have studied the effects of finite interaction strengths and a finite laser linewidth on the visibility of the revivals. We have shown that observation of collapses and revivals of Rabi oscillations can be used as a signature of the Rydberg blockade without the need to measure the exact number of Rydberg atoms.

DOI
10.1103/physreva.90.043413

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•Apr 1, 2008•15 citations
We show that Jaynes-Cummings dynamics can be observed in mesoscopic atomic ensembles interacting with a classical electromagnetic field in the regime of a Rydberg blockade where the time dynamics of the average number of Rydberg excitations in mesoscopic ensembles displays collapses and revivals typical of this model. As the frequency of Rabi oscillations between collective states of Rydberg-blockaded ensembles depends on the number of interacting atoms, for randomly loaded optical dipole traps, we predict collapses and revivals of Rabi oscillations. We have studied the effects of finite interaction strengths and a finite laser linewidth on the visibility of the revivals. We have shown that observation of collapses and revivals of Rabi oscillations can be used as a signature of the Rydberg blockade without the need to measure the exact number of Rydberg atoms.
The interaction between atoms and a quantized radiation field is fundamentally important in quantum optics and quantum information science. Due to their unusual properties, Rydberg atoms are promising building blocks for two-qubit gates and atom-light quantum interfaces, exploiting the Rydberg blockade interaction which prevents two atoms at close distance ( < 10 μ m ) from being simultaneously excited to Rydberg states. Recently, this effect was used to engineer quantum processors based on arrays of interacting Rydberg atoms illuminated by Raman lasers. Motivated by these experiments, we extend the Jaynes–Cummings model to study the interaction between two Rydberg atoms interacting by the Rydberg blockade and a quantized radiation field. We consider both number (Fock) states of the field and single-mode quantum coherent states. In particular, we discuss different types of entanglements between various components of the total system consisting of the two Rydberg-interacting atoms and coherent states of the field, and show that the behavior is significantly different compared to a system with non-interacting atoms corresponding to the two-atom Tavis-Cummings model. Our results are relevant in view of atom-light quantum interfaces as components for future long-distance quantum communication.
We demonstrate the coherent excitation of a mesoscopic ensemble of about 100 ultracold atoms to Rydberg states by driving Rabi oscillations from the atomic ground state. We employ a dedicated beam shaping and optical pumping scheme to compensate for the small transition matrix element. We study the excitation in a weakly interacting regime and in the regime of strong interactions. When increasing the interaction strength by pair state resonances, we observe an increased excitation rate through coupling to high angular momentum states. This effect is in contrast to the proposed and previously observed interaction-induced suppression of excitation, the so-called dipole blockade.
Abstract The temporal dynamics of three-photon 5S1/2 → 5P3/2 → 6S1/2 → 39P3/2 laser excitation of mesoscopic ensembles of cold Rb atoms to Rydberg states in a magneto-optical trap is studied using cw single-frequency lasers at each stage. The ensembles comprise N = 1 – 5 atoms and are detected by the method of selective field ionisation with postselection with respect to the number of atoms. The dependence of the excitation probability on the duration of the exciting laser pulses and the number of detected Rydberg atoms is investigated. At short interaction times, a linear increase in probabilities is observed, and at large times, the probabilities reach saturation, while each number of atoms has its own characteristic features. The experimental dependences are compared with the results of numerical calculations in the framework of a four-level model, and their good agreement is obtained. The conditions necessary for observing Rabi population oscillations are determined. The obtained results are important for the application of Rydberg atoms in quantum information.
The realization of a Jaynes-Cummings model in the optical domain is proposed for an atomic ensemble. The scheme exploits the collective coupling of the atoms to a quantized cavity mode and the nonlinearity introduced by coupling to high-lying Rydberg states. A two-photon transition resonantly couples the single-atom ground state $|g\ensuremath{\rangle}$ to a Rydberg state $|e\ensuremath{\rangle}$ via a nonresonant intermediate state $|i\ensuremath{\rangle}$, but due to the interaction between Rydberg atoms only a single atom can be resonantly excited in the ensemble. This restricts the state space of the ensemble to the collective ground state $|G\ensuremath{\rangle}$ and the collectively excited state $|E\ensuremath{\rangle}$ with a single Rydberg excitation distributed evenly on all atoms. The collectively enhanced coupling of all atoms to the cavity field with coherent coupling strengths which are much larger than the decay rates in the system leads to the strong coupling regime of the resulting effective Jaynes-Cummings model. We use numerical simulations to show that the cavity transmission can be used to reveal detailed properties of the Jaynes-Cummings ladder of excited states and that the atomic nonlinearity gives rise to highly nontrivial photon emission from the cavity. Finally, we suggest that the absence of interactions between remote Rydberg atoms may, due to a combinatorial effect, induce a cavity-assisted excitation blockade whose range is larger than the typical Rydberg dipole-dipole interaction length.
Rydberg interactions of trapped alkali-metal atoms are used widely to facilitate quantum gate operations in quantum processors and repeaters. In most laboratory realizations using this protocol, the Rydberg states are repelled by the trapping laser fields, requiring that the fields be turned off during gate operations. Here we create a quasi-two-level system in a regime of Rydberg excitation blockade for a mesoscopic Rb ensemble of several hundred atoms confined in a magic-wavelength optical lattice. We observe many-body Rabi oscillations between the ground and collective Rydberg state. In addition we use Ramsey interference techniques to obtain the light shifts of both the lower and upper states of the collective qubit. Whereas the coupling producing the Rabi oscillations is enhanced by a factor of sqrt[N], there is no corresponding enhancement for the light shifts. We derive an effective two-level model which is in good agreement with our observations. Trapped Rydberg qubits and an effective two-level description are expected to have broad applicability for studies of quantum simulation and networking using collective encoding in ensembles of neutral atoms.
We present a detailed analysis of our recent observation of synchronous Rabi oscillations between the electronic ground state and Rydberg states in a mesoscopic ensemble containing roughly 100 ultracold atoms (Reetz-Lamour et al submitted, Preprint 0711.4321). The mesoscopic cloud is selected out of a sample of laser-cooled Rb atoms by optical pumping. The atoms are coupled to a Rydberg state with principal quantum number around 30 by a two-photon scheme employing flat-top laser beams. The influence of residual spatial intensity fluctuations as well as sources of decoherence such as redistribution to other states, radiative lifetime and laser bandwidth are analysed. The results open up new possibilities for the investigation of coherent many-body phenomena in dipolar Rydberg gases. As an example we demonstrate the van der Waals blockade, a variant of the dipole blockade, for a mesoscopic atom sample.