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arXiv:1403.2495 · Europhysics Letters (EPL)

Field-assisted doublon manipulation in the Hubbard model: A quantum doublon ratchet

Karsten Balzer, Martin Eckstein

Published Sep 1, 2014• 3 citations
arXivHTMLPDF

Abstract

For the fermionic Hubbard model at strong coupling, we demonstrate that directional transport of localized doublons (repulsively bound pairs of two particles occupying the same site of the crystal lattice) can be achieved by applying an unbiased ac field of time-asymmetric (sawtooth-like) shape. The mechanism involves a transition to intermediate states of virtually zero double occupation which are reached by splitting the doublon by fields of the order of the Hubbard interaction. The process is discussed on the basis of numerically exact calculations for small clusters, and we apply it to more complex states to manipulate the charge order pattern of one-dimensional systems.

DOI
10.1209/0295-5075/107/57012

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For the fermionic Hubbard model at strong coupling, we demonstrate that directional transport of localized doublons (repulsively bound pairs of two particles occupying the same site of the crystal lattice) can be achieved by applying an unbiased ac field of time-asymmetric (sawtooth-like) shape. The mechanism involves a transition to intermediate states of virtually zero double occupation which are reached by splitting the doublon by fields of the order of the Hubbard interaction. The process is discussed on the basis of numerically exact calculations for small clusters, and we apply it to more complex states to manipulate the charge order pattern of one-dimensional systems.
The hopping dynamics of two fermionic species with different effective masses in the one-dimensional Hubbard model driven by an external field are theoretically investigated. A multiple-time-scale asymptotic analysis of the driven asymmetric Hubbard model shows that a high-frequency bichromatic external field can sustain a low-energy particle bound state (a doublon) in which two fermions of different species occupy nearest-neighbor sites and cotunnel along the lattice. The predictions of the asymptotic analysis are confirmed by direct numerical simulations of the two-particle Hubbard Hamiltonian.
Two fermions occupying the same site of a lattice model with strongly repulsive Hubbard-type interaction UUU form a doublon, a long-living excitation, the decay of which is suppressed because of energy conservation. By means of an exact-diagonalization approach based on the Krylov-space technique, we study the dynamics of a single doublon, of two doublons, and of a doublon in the presence of two additional fermions prepared locally in the initial state of the extended Hubbard model. The time dependence of the expectation value of the double occupancy at the different sites of a large one-dimensional lattice is analyzed by perturbative arguments. In this way the spatiotemporal evolution of the doublon can be understood. The initial decay takes place on a short time scale 1/U1/U1/U, and the long-time average of the decayed fraction of the total double occupancy scales as 1/U21/{U}^{2}1/U2. We demonstrate how the dynamics of a doublon in the initial state is related to the spectrum of two-fermion excitations obtained from linear-response theory, we work out the difference between doublons composed of fermions vs doublons composed of bosons, and we show that despite the increase of phase space for inelastic decay processes, the stability of a doublon is enhanced by the presence of additional fermions on an intermediate time scale.
We investigate the possibility to control dynamically the interactions between repulsively bound pairs of fermions (doublons) in correlated systems with off-resonant ac fields. We introduce an effective Hamiltonian that describes the physics of doublons up to second order in the high-frequency limit. It unveils that the doublon interaction, which is attractive in equilibrium, can be completely suppressed and then switched to repulsive by varying the power of the ac field. We show that the signature of the dynamical repulsion between doublons can be found in the single-fermion density of states averaged in time. Our results are further supported by nonequilibrium dynamical mean-field theory simulations for the half-filled Fermi-Hubbard model.
Periodically driven systems can lead to a directed motion of particles. We investigate this ratchet effect for a bosonic Mott insulator where both a staggered hopping and a staggered local potential vary periodically in time. If driving frequencies are smaller than the interaction strength and the density of excitations is small, one obtains effectively a one-particle quantum ratchet describing the motion of doubly occupied sites (doublons) and empty sites (holes). Such a simple quantum machine can be used to manipulate the excitations of the Mott insulator. For suitably chosen parameters, for example, holes and doublons move in opposite directions. To investigate whether the periodic driving can be used to move particles ``uphill,'' i.e., against an external force, we study the influence of a linear potential $\ensuremath{-}gx$. For long times, transport is only possible when the driving frequency $\ensuremath{\omega}$ and the external force ggg are commensurate, ${n}_{0}g={m}_{0}\ensuremath{\omega}$, with $\frac{{n}_{0}}{2},{m}_{0}\ensuremath{\in}\mathbb{Z}$.
Dynamical formation of doublons or on-site repulsively bound pairs of particles on a lattice is a highly nontrivial phenomenon. In this work, we show the signatures of doublon formation in a quantum computer by simulating the continuous time quantum walk in the framework of the one-dimensional extended Fermi-Hubbard model. By considering two up-component and one down-component particles initially created at the three neighboring sites at the middle of the lattice and allowing intra- (inter-)component nearest-neighbor (on-site) interactions, we show the formation of a stable on-site doublon in the quantum walk. The probability of such doublon formation is more (less) if the hopping strength of the down particle is weaker (stronger) compared to the up particle. On the contrary, for an initial doublon along with a free up particle, the stability of the doublon is more prominent than the doublon dissociation in the dynamics irrespective of the hopping asymmetry between the two components. We first numerically obtain the signatures of the stable doublon formation in the dynamics and then observe them using noisy intermediate-scale quantum (NISQ) devices.
The fate of a local two-hole doublon excitation in the one-dimensional Fermi-Hubbard model is systematically studied for strong Hubbard interaction UUU in the entire filling range using the density-matrix renormalization group (DMRG) and the Bethe ansatz. For strong UUU, two holes at the same site form a compound object whose decay is impeded by the lack of phase space. Still, a partial decay is possible on an extremely short time scale where phase-space arguments do not yet apply. We argue that the initial decay and the resulting intermediate state are relevant for experiments performed with ultracold atoms loaded into an optical lattice as well as for (time-resolved) CVV Auger-electron spectroscopy. The detailed discussion comprises the mixed ballistic-diffusive real-time propagation of the doublon through the lattice, its partial decay on the short time scale as a function of filling and interaction strength, as well as the analysis of the decay products, which are metastable on the intermediate time scale that is numerically accessible and which show up in the two-hole excitation (Auger) spectrum. The ambivalent role of singly occupied sites is key to understanding the doublon physics; for high fillings, ground-state configurations with single occupancies are recognized to strongly relax the kinematic constraints and to open up decay channels. For fillings close to half-filling, however, their presence actually blocks the doublon decay. Finally, the analysis of the continua in the two-hole spectrum excludes a picture where the doublon decays into unbound electron holes for generic fillings, different from the limiting case of the completely filled band. We demonstrate that the decay products as well as the doublon propagation should rather be understood in terms of Bethe ansatz eigenstates.