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arXiv:1402.4587 · Physical Review A

Unconventional photon blockade in doubly resonant microcavities with second-order nonlinearity

Dario Gerace, Vincenzo Savona

Published Mar 20, 2014• 172 citations
arXivHTMLPDF

Abstract

It is shown that noncentrosymmetric materials with bulk second-order nonlinear susceptibility can be used to generate strongly antibunched radiation at an arbitrary wavelength, solely determined by the resonant behavior of suitably engineered coupled microcavities. The proposed scheme exploits the unconventional photon blockade of a coherent driving field at the input of a coupled cavity system, where one of the two cavities is engineered to resonate at both fundamental and second harmonic frequencies, respectively. Remarkably, the unconventional blockade mechanism occurs with reasonably low quality factors at both harmonics, and does not require a sharp doubly resonant condition for the second cavity, thus proving its feasibility with current semiconductor technology.

DOI
10.1103/physreva.89.031803

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It is shown that noncentrosymmetric materials with bulk second-order nonlinear susceptibility can be used to generate strongly antibunched radiation at an arbitrary wavelength, solely determined by the resonant behavior of suitably engineered coupled microcavities. The proposed scheme exploits the unconventional photon blockade of a coherent driving field at the input of a coupled cavity system, where one of the two cavities is engineered to resonate at both fundamental and second harmonic frequencies, respectively. Remarkably, the unconventional blockade mechanism occurs with reasonably low quality factors at both harmonics, and does not require a sharp doubly resonant condition for the second cavity, thus proving its feasibility with current semiconductor technology.
Abstract We propose an unconventional photon blockade scheme in coupled semiconductor microcavities embedded in a nonlinear Kerr medium in the presence of photon leakage and bimodal driving on two cavity modes, which consists of two spatially overlapping single-mode semiconductor cavities with cross-Kerr nonlinearity and two-photon tunneling. A detailed analysis is derived for the exact optimal conditions for strong photon antibunching with weak Kerr nonlinearities. It is very important to find the transition of the structures of the solution for the optimal detuning from the quartic equation to the cubic equation when changing the two complex driving fields appropriately. The transition originates from the second driving field that compensates the numbers of interference paths reaching a two-photon state. This unconventional photon blockade can be realized by coupled photonic crystal cavities filled with a nonlinear Kerr medium. This implies that nonlinear Kerr medium systems can be used to generate tunable single-photon sources by tuning the strength and relative phase of two complex driving fields under weak Kerr nonlinearity.
We propose the use of nanostructured photonic nanocavities made of ${\ensuremath{\chi}}^{(2)}$ nonlinear materials as prospective passive devices to generate strongly sub-Poissonian light via single-photon blockade of an input coherent field. The simplest scheme is based on the requirement that the nanocavity be doubly resonant, i.e., possess cavity modes with good spatial overlap at both the fundamental and second-harmonic frequencies. We discuss the feasibility of this scheme with state-of-the art nanofabrication technology and the possibility to use it as a passive single-photon source on demand.
The single‐photon blockade effect arising in a cavity containing a quantum well and interacting with squeezed light, resulting from a down‐conversion process through a nonlinear medium, is investigated. Optical parametric oscillator (OPO) materials with positive and negative second‐order susceptibilities are considered. By solving the master equation analytically in the weak‐driving limit and calculating the second‐order equal‐time correlation function, it is found that strong photon antibunching can be achieved in this system with weak excitonic nonlinearity or squeezed light via a destructive quantum interference mechanism. The optimal conditions for the photon blockade are derived analytically and discussed in details. Unlike the excitonic nonlinearity, a strong photon blockade occurs with the squeezed light at total or quasitotal resonance, even in the weak coupling regime, using an OPO material with negative second‐order nonlinear susceptibility. By acting on the driving coherent pump frequency, the control of the cavity output is achieved and the scheme can serve as a tunable single‐photon emission source.
The photon blockade based on weak nonlinearities is called the unconventional photon blockade. The study of the unconventional photon blockade in recent decades has mainly focused on the ${\ensuremath{\chi}}^{(3)}$ Kerr nonlinearity. In this paper, we study the photon blockade in two weakly coupled nonlinear cavities via ${\ensuremath{\chi}}^{(2)}$ nonlinearity, where ${\ensuremath{\chi}}^{(2)}$ mediates the conversion of a single photon in the cavity with high frequency into two photons with low frequency in another cavity. When the two cavity modes are driven simultaneously, our calculations show that the strong photon antibunching can be obtained in the cavity. The optimal condition for strong antibunching is found by analytic calculations and numerical simulations, and discussions of the optimal condition are presented. The differences between the present scheme and that with ${\ensuremath{\chi}}^{(3)}$ nonlinearity are discussed. This scheme is not sensitive to the change of decay rates, which makes the experimental realization easy.
In the recent publications [Phys. Rev. A 92,023838 (2015)], the unconventional photon blockade are studied in a two-mode-second-order-nonlinear system with nonlinear coupling between the low frequency and high frequency modes. In this paper, we study the unconventional photon blockade in a three-mode system with weakly coupled nonlinear cavities via χ(2)χ^{(2)}χ(2) nonlinearity. By solving the master equation in the steady-state limit and calculating the zero-delay time second-order correlation function, we obtain the conditions of strong photon antibunching in the low frequency mode. The numerical result are compared with the analytical results, the results show that they are in complete agreement. By the analysis of numerical solutions, we find that this scheme is not sensitive to the change of decay rates and the reservoir temperature, and the three-mode drives make the system have more adjustable parameters, both of which increases the possibility of experimental implementation.
We propose a scheme of photon blockade in a system comprising of coupled cavities embedded in Kerr nonlinear material, where two cavities are driven and dissipated. We analytically derive the exact optimal conditions for strong photon antibunching, which are in good agreement with those obtained by numerical simulations. We find that conventional and unconventional photon blockades have controllable flexibilities by tuning the strength ratio and relative phase between two complex driving fields. Such unconventional photon-blockade effects are ascribed to the quantum interference effect to avoid two-photon excitation of the coupled cavities. We also discuss the statistical properties of the photons under given optimal conditions. Our results provide a promising platform for the coherent manipulation of photon blockade, which has potential applications for quantum information processing and quantum optical devices.