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arXiv:1402.4339 · Proceedings of the National Academy of Sciences

A new type of half-quantum circulation in a macroscopic polariton spinor ring condensate

Gangqiang Liu, David W. Snoke, Andrew J. Daley, Loren N. Pfeiffer, K. W. West

Published Feb 17, 2015• 68 citations
arXivHTMLPDF

Abstract

We report the observation of coherent circulation in a macroscopic Bose-Einstein condensate of polaritons in a ring geometry. Because they are spinor condensates, half-quanta are allowed in where there is a phase rotation of π in connection with a polarization vector rotation of π around a closed path. This half-quantum behavior is clearly seen in the experimental observations of the polarization rotation around the ring. In our ring geometry, the half-quantum state that we see is one in which the handedness of the spin flips from one side of the ring to the other side in addition to the rotation of the linear polarization component; such a state is allowed in a ring geometry but will not occur in a simply connected geometry. This state is lower in energy than a half-quantum state with no change of the spin direction and corresponds to a superposition of two different elementary half-quantum states. The direction of circulation of the flow around the ring fluctuates randomly between clockwise and counterclockwise from one shot to the next; this fluctuation corresponds to spontaneous breaking of time-reversal symmetry in the system. This type of macroscopic polariton ring condensate allows for the possibility of direct control of the circulation to excite higher quantized states and the creation of Josephson junction tunneling barriers.

DOI
10.1073/pnas.1424549112

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We report the observation of coherent circulation in a macroscopic Bose-Einstein condensate of polaritons in a ring geometry. Because they are spinor condensates, half-quanta are allowed in where there is a phase rotation of π in connection with a polarization vector rotation of π around a closed path. This half-quantum behavior is clearly seen in the experimental observations of the polarization rotation around the ring. In our ring geometry, the half-quantum state that we see is one in which the handedness of the spin flips from one side of the ring to the other side in addition to the rotation of the linear polarization component; such a state is allowed in a ring geometry but will not occur in a simply connected geometry. This state is lower in energy than a half-quantum state with no change of the spin direction and corresponds to a superposition of two different elementary half-quantum states. The direction of circulation of the flow around the ring fluctuates randomly between clockwise and counterclockwise from one shot to the next; this fluctuation corresponds to spontaneous breaking of time-reversal symmetry in the system. This type of macroscopic polariton ring condensate allows for the possibility of direct control of the circulation to excite higher quantized states and the creation of Josephson junction tunneling barriers.
We predict the spontaneous symmetry breaking in a spinor Bose-Einstein condensate of exciton-polaritons (polaritons) caused by the coupling of its spin and orbital degrees of freedom. We study a polariton condensate trapped in a ring-shaped effective potential with a broken rotational symmetry. We propose a realistic scheme of generating controllable spinor azimuthal persistent currents of polaritons in the trap under the continuous wave optical pump. We propose a new type of half-quantum circulating states in a spinor system characterized by azimuthal currents in both circular polarizations and a vortex in only one of the polarizations. The spontaneous symmetry breaking in the spinor polariton condensate that consists in the switching from co-winding to opposite-winding currents in opposite spin states is revealed. It is characterized by the change of the average orbital angular momentum of the condensate from zero to non-zero values. The radial displacement of the pump spot and the polarization of the pump act as the control parameters. The considered system exhibits a fundamental similarity to a superconducting flux qubit, which makes it highly promising for applications in quantum computing.
Bosonic condensates of spinless noninteracting particles confined on a ring cannot propagate circular periodic currents once rotation symmetry of the system is broken. However, a persistent current may appear due to interparticle interactions exceeding some critical strength. In this up-critical regime breaking of the symmetry between the clockwise and anticlockwise rotations takes place. We consider this symmetry-breaking scenario in the case of a spinor condensate of exciton polaritons trapped on a ring split by a potential barrier. Due to the intrinsic symmetry of the effective spin-orbit interaction, which stems from the linear splitting between transverse-electric and transverse-magnetic microcavity modes, the potential barrier blocks the circulating current and imposes linear polarization patterns. On the other hand, circularly polarized polaritons form circular currents propagating in opposite directions with equal absolute values of angular momentum. In the presence of interparticle interactions, the symmetry of clockwise and anticlockwise currents can be broken spontaneously. We describe several symmetry-breaking scenarios, which imply either restoration of the global condensate rotation or the onset of the circular polarization in the symmetry-broken state.
Spinorial or multi-component Bose-Einstein condensates may sustain fractional quanta of circulation, vorticant topological excitations with half integer windings of phase and polarization. Matter-light quantum fluids, such as microcavity polaritons, represent a unique test bed for realising strongly interacting and out-of-equilibrium condensates. The direct access to the phase of their wavefunction enables us to pursue the quest of whether half vortices ---rather than full integer vortices--- are the fundamental topological excitations of a spinor polariton fluid. Here, we are able to directly generate by resonant pulsed excitations, a polariton fluid carrying either the half or full vortex states as initial condition, and to follow their coherent evolution using ultrafast holography. Surprisingly we observe a rich phenomenology that shows a stable evolution of a phase singularity in a single component as well as in the full vortex state, spiraling, splitting and branching of the initial cores under different regimes and the proliferation of many vortex anti-vortex pairs in self generated circular ripples. This allows us to devise the interplay of nonlinearity and sample disorder in shaping the fluid and driving the phase singularities dynamics
Persistent circulation is a canonical effect of superfluidity. In previous experiments, quantized circulation has been observed in polariton condensates, usually far from equilibrium, but persistent current in the absence of any stirring has not been seen. We report here the direct observation of persistent circulation of a polariton condensate with no driving force and with no observable change in time. We can cause the condensate to circulate in either direction on demand using a short laser pulse, after which the condensate continues to circulate for dozens to hundreds of rotations around a ring trap without any further stimulation. Our theoretical model successfully shows how the pulse, despite not carrying any angular momentum, causes circulation.
Motivated by a recent experiment [Beattie, Moulder, Fletcher, and Hadzibabic, Phys. Rev. Lett. 110, 025301 (2013)], we study the superflow of atomic spinor Bose-Einstein condensates optically trapped in a ring-shaped geometry. Within a dissipative mean-field approach we simulate a two-component condensate in conditions adapted to the experiment. In qualitative agreement with the experimental findings, we observe stable superflow if the spin-population imbalance is above some well-defined threshold value. Below the stability threshold the persistent currents with higher-order circulation decay in quantized steps, and the vortex lines escape from the center of the ring through dynamically created ``weak links'' in the condensate annulus. These regions with reduced density of one spin component are filled by atoms of the other component. The vortices then leave the ring-shaped high-density region of the condensate and finally decay into elementary excitations.
We present a scheme for creating macroscopic superpositions of the direction of superfluid flow around a loop. Using the Bose–Hubbard model, we study an array of Bose–Einstein condensates (BECs) trapped in optical potentials and coupled to one another to form a ring. By rotating the ring so that each particle acquires on average half a quantum of superfluid flow, it is possible to create a multiparticle superposition of all the particles rotating and all the particles stationary. Under certain conditions it is possible to scale up the number of particles to form a macroscopic superposition. The simplicity of the model has allowed us to study macroscopic superpositions at an atomic level for different variables. Here, we concentrate on the tunnelling strength between the potentials. Further investigation remains important, because it could lead us to making an ultra-precise quantum-limited gyroscope.