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arXiv:1402.1930 · Optics Express

Quantum theory of a spaser-based nanolaser

Vladimir Parfenyev, S. S. Vergeles

Published May 29, 2014• 25 citations
arXivHTMLPDF

Abstract

We present a quantum theory of a spaser-based nanolaser, under the bad-cavity approximation. We find first- and second-order correlation functions g(1)(τ) and g(2)(τ) below and above the generation threshold, and obtain the average number of plasmons in the cavity. The latter is shown to be of the order of unity near the generation threshold, where the spectral line narrows considerably. In this case the coherence is preserved in a state of active atoms in contradiction to the good-cavity lasers, where the coherence is preserved in a state of photons. The damped oscillations in g(2)(τ) above the generation threshold indicate the unusual character of amplitude fluctuations of polarization and population, which become interconnected in this case. Obtained results allow to understand the fundamental principles of operation of nanolasers.

DOI
10.1364/oe.22.013671

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We present a quantum theory of a spaser-based nanolaser, under the bad-cavity approximation. We find first- and second-order correlation functions g(1)(τ) and g(2)(τ) below and above the generation threshold, and obtain the average number of plasmons in the cavity. The latter is shown to be of the order of unity near the generation threshold, where the spectral line narrows considerably. In this case the coherence is preserved in a state of active atoms in contradiction to the good-cavity lasers, where the coherence is preserved in a state of photons. The damped oscillations in g(2)(τ) above the generation threshold indicate the unusual character of amplitude fluctuations of polarization and population, which become interconnected in this case. Obtained results allow to understand the fundamental principles of operation of nanolasers.
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We investigate the dynamics of the spaser-based nanolaser in the strong incoherent pumping regime in the quantum limit when the photon number is the order of unity. We consider the situation where the newly irradiated photon finds itself in the cloud of earlier irradiated photons that are not thermalized. As the result the entanglement of nanoparticle with quantum dot degrees of freedom in the nanolaser and the lasing intensity increases several times. In fact, the nonthermal bath effectively makes the nanolaser ``more quantum'' and the master equation for the nanolaser density matrix nonlinear and self-consistent.
The Siegert relation connects the first- and second-order coherence properties of light. Although strictly valid only in the thermal regime and in the absence of correlations, this relation is routinely extended to the partially coherent regime in the study of high-β nanolasers, where it aids in the identification of the lasing threshold. We re-evaluate the use of a generalized Siegert relation in different device regimes. A full two-time quantum-optical theory is derived as a reference for obtaining first- and second-order correlation functions g(1)(τ) and g(2)(τ) in the steady state. We find that even in the partially coherent regime, the generalized Siegert relation is well suited as an approximation to g(2)(τ) as long as emitter correlations are negligible but does not apply well in the quantum regime of few-emitter nanolasers or to devices featuring sub- and super-radiant emission.
We detail the derivation of nanolaser models that include coherent and incoherent variables and predict the existence of a laser threshold, irrespective of cavity size and emitter number, for both single- and multielectron systems. The growth in photon number in the lasing mode is driven by an increase in correlation between absorption and emission processes, leading to the onset of self-sustained stimulated emission (laser threshold), followed in turn by a correlation decrease and ending with the dominance of coherent emission. The first-order coherence g(1){g}^{(1)}g(1) steadily increases, as the pump grows towards the laser threshold value, and reaches unity at or beyond threshold. The transition toward coherent emission becomes increasingly sharp as the numbers of emitters and coupled electromagnetic cavity modes increase, continuously connecting, in the thermodynamic limit, the physics of nano- and macroscopic lasers at threshold. Our predictions are in remarkable agreement with experiments whose first-order coherence measurements have so far been explained only phenomenologically. A consistent evaluation of different threshold indicators provides a tool for a correct interpretation of experimental measurements at the onset of laser action.
The laser has evolved from table size apparatuses to truly nano sized devices, in much the same way that computer chips have been continuously minimized. The few-emitter nanolaser represents an extreme in terms of size. The emitters can be either atoms or quantum dots, and they are coupled to a high-Q optical cavity. This system has previously been studied for the one and two emitters case, see e.g. [1, 2]. The emitters and cavity are modelled as two-level systems and a harmonic oscillator, respectively. The coupled system is modelled using the Jaynes-Cummings Hamiltonian and the two-level systems are pumped incoherently by a rate P. Solutions are found using the corresponding master equation. However, with cavity populations exceeding 100 and several emitters, the dimension of the Hilbert space of the system becomes too large to handle efficiently on a conventional computer. E.g. for four emitters and 100 photon states the density matrix has more than 2.5 × 106 elements. We have been able to simplify the problem significantly by adiabatically eliminating the photon-assisted polarizations and the correlations between emitters and cavity [3]. This results in a set of rate equations for the population of the cavity, na, and the occupation of the emitters. Fig. 1a) shows na for up to 4 emitters coupled to a cavity, as a function of the pumping rate P. The figure also shows results from a full master equation solution, and the correspondence is very good for large values of P. In Fig. 1b) the second order correlation functions g(2)(0) are shown, as obtained using the full model. The second order correlation functions become 1 for sufficiently large values of P signifying the onset of lasing. However, for larger values of P the laser quenches and the emission becomes chaotic (g(2)(0) = 2). This quenching effect is well-known in two-level models [3], but might not be realistic for semiconductor quantum dots. A proposed application for these nanolasers is in on-chip optical interconnects. In this application the modulation bandwidth is important. We have calculated the modulation bandwidth using a small-signal analysis of the rate equations, which has the advantage compared the full model of yielding a semianalytical result. The results are shown in Fig. 1c). The nanolaser has a high bandwidth, which is mostly limited by the cavity lifetime (/ 1/), but shows a prominent drop during the lasing regime. The modulation bandwidth again becomes limited by as the output becomes chaotic.
A numerically exact solution to the many emitter--cavity problem as an open many body system is presented. The solution gives access to the full, nonperturbative density matrix and thus the full quantum statistics and quantum correlations. The numerical effort scales with the third power in the number of emitters. Notably the solution requires none of the common approximations such as good/bad cavity limit. As a first application the recently discussed concept of coherent surface plasmon amplification---spaser---is addressed: A spaser consists of a plasmonic nanostructure that is driven by a set of quantum emitters. In the context of laser theory it is a laser in the (very) bad cavity limit with an extremely high light matter interaction strength. The method allows us to answer the question of spasing with a fully quantized theory.