Faithful storage and coherent manipulation of quantum optical pulses are key for long distance quantum communications and quantum computing. Combining these functions in a light–matter interface that can be integrated on-chip with other photonic quantum technologies, e.g. sources of entangled photons, is an important step towards these applications. To date there have only been a few demonstrations of coherent pulse manipulation utilizing optical storage devices compatible with quantum states, and that only in atomic gas media (making integration difficult) and with limited capabilities. Here we describe how a broadband waveguide quantum memory based on the atomic frequency comb (AFC) protocol can be used as a programmable processor for essentially arbitrary spectral and temporal manipulations of individual quantum optical pulses. Using weak coherent optical pulses at the few photon level, we experimentally demonstrate sequencing, time-to-frequency multiplexing and demultiplexing, splitting, interfering, temporal and spectral filtering, compressing and stretching as well as selective delaying. Our integrated light–matter interface offers high-rate, robust and easily configurable manipulation of quantum optical pulses and brings fully practical optical quantum devices one step closer to reality. Furthermore, as the AFC protocol is suitable for storage of intense light pulses, our processor may also find applications in classical communications.
Faithful storage and coherent manipulation of quantum optical pulses are key for long distance quantum communications and quantum computing. Combining these functions in a light–matter interface that can be integrated on-chip with other photonic quantum technologies, e.g. sources of entangled photons, is an important step towards these applications. To date there have only been a few demonstrations of coherent pulse manipulation utilizing optical storage devices compatible with quantum states, and that only in atomic gas media (making integration difficult) and with limited capabilities. Here we describe how a broadband waveguide quantum memory based on the atomic frequency comb (AFC) protocol can be used as a programmable processor for essentially arbitrary spectral and temporal manipulations of individual quantum optical pulses. Using weak coherent optical pulses at the few photon level, we experimentally demonstrate sequencing, time-to-frequency multiplexing and demultiplexing, splitting, interfering, temporal and spectral filtering, compressing and stretching as well as selective delaying. Our integrated light–matter interface offers high-rate, robust and easily configurable manipulation of quantum optical pulses and brings fully practical optical quantum devices one step closer to reality. Furthermore, as the AFC protocol is suitable for storage of intense light pulses, our processor may also find applications in classical communications.
Processing and distributing quantum information using photons through fibre-optic or free-space links are essential for building future quantum networks. The scalability needed for such networks can be achieved by employing photonic quantum states that are multiplexed into time and/or frequency, and light-matter interfaces that are able to store and process such states with large time-bandwidth product and multimode capacities. Despite important progress in developing such devices, the demonstration of these capabilities using non-classical light remains challenging. Here, employing the atomic frequency comb quantum memory protocol in a cryogenically cooled erbium-doped optical fibre, we report the quantum storage of heralded single photons at a telecom-wavelength (1.53 μm) with a time-bandwidth product approaching 800. Furthermore, we demonstrate frequency-multimode storage and memory-based spectral-temporal photon manipulation. Notably, our demonstrations rely on fully integrated quantum technologies operating at telecommunication wavelengths. With improved storage efficiency, our light-matter interface may become a useful tool in future quantum networks.
The light–matter interface is an important building block for long-distance quantum networks. Towards a scalable quantum network with high-rate quantum information processing, it requires to develop integrated light–matter interfaces with broadband and multiplexing capacities. Here we demonstrate a light–matter interface at the telecom band in an integrated system. A five-spectral-channel atomic-frequency-comb photonic memory is prepared on a laser-written Er3+:LiNbO3 chip. The bandwidth of each channel is 4 GHz with a channel spacing of 15 GHz. The signal photons from time-bin entangled photon pairs at the telecom band are sent into the on-chip memory and recalled after a storage time of 152 ns. The entanglement-preserving nature of our integrated quantum interface is assessed by an input/output fidelity of >92% for all five spectral channels. Our light–matter interfaces constitute a notable step forward toward a high-rate quantum network involving integrated devices.
Quantum communication founds on the possibility to encode quantum states into photons and allows, for instance, the provable secure distribution of encryption keys. Despite a lot of progress during the past two decades, quantum communication still faces a distance barrier, which can be overcome by quantum repeaters whose currently most challenging ingredient is a memory for quantum states of light. In addition to robustness and ease of use, the requirements for such a quantum memory include high fidelity quantum state storage and the preservation of entanglement, sufficiently long storage time with on-demand recall, high efficiency, large bandwidth, and high multimode capacity. Six years ago, some of these properties had already been demonstrated using atomic vapor. However, practical solid-state memories were virtually unexplored in view of quantum state storage. The main goal of this thesis was to realize a solid-state quantum memory for light with emphasis on meeting requirements for long distance quantum communication. First, we identified a potential material candidate, a thulium doped lithium niobate waveguide, and conducted spectroscopic investigations to assess its suitability for quantum state storage using a photon-echo type approach. Next, we demonstrated that our storage device is suitable for high fidelity quantum state storage and for the storage of photonic entanglement, and that its large spectral multimode capacity allows for on-demand selective recall in conjunction with standard spectral filters and frequency shifters. In addition, by performing two-photon interference experiments and Bell-State measurements, we found that our memory preserves not only quantum information, but, more generally, the entire photonic wave function, which further confirms its suitability for quantum repeaters as well as for linear optics quantum computers. Finally, we showed that our integrated device also allows for general temporal and spectral manipulation of individual quantum optical pulses, which paves the way towards on-chip quantum optical processors. While more work remains to be done, in particular to improve memory efficiency and storage time, the large number of achievements, together with known ways to overcome the remaining obstacles, makes us confident that a quantum memory suitable for quantum repeaters will soon be built.
(English) Future networks for quantum communication will require a new form of technology in order to operate over long distances. The no-cloning theorem precludes the use of amplification, so quantum repeater schemes have been proposed to achieve long-distance quantum communication through the distribution of entanglement. A key device for this setup is a quantum memory, which is required in order to store entanglement and synchronise its distribution. Among the many physical systems than can be used as a quantum memory, rare-earth ion-doped crystals stand out due to their long coherence times and potential for multiplexing and integration. This thesis reports the use of one such system, Pr3+:Y2SiO5, as a quantum memory using the atomic frequency comb (AFC) protocol. Building on previous work, we improved the performance of the memory to be able to demonstrate light-matter entanglement with a telecommunications wavelength photon and the quantum memory, for both a bulk memory and an integrated version. To measure light-matter entanglement, we use photon pairs generated through cavity-enhanced spontaneous parametric down conversion, where one photon (the signal) is stored in the memory and the other (the idler) is at a telecommunications wavelength. These photon pairs exhibit energy-time entanglement, which we analyse in the time basis using fibre- and AFC-based Mach-Zehnder interferometers. In the first experiment, we demonstrate light-matter entanglement where the bulk quantum memory is used with on-demand retrieval via storage in a spin-wave. We measure interference fringes with average visibilities of 89(2)% for AFC storage, and 70(3)% for spin-wave storage, sufficient to demonstrate entanglement. This is the first such demonstration using an on-demand multimode solid-state memory and telecom photon. We show that entanglement is maintained for up to 47.7 µs of storage. These results were made possible through improvements in the AFC efficiency and the noise filtering. Furthermore, we perform on-demand storage and retrieval of up to 30 temporal modes. We take the next step towards implementing our system in a real world scenario by measuring entanglement over a distance. To do so, we send the idler photons through both optical fibre spools and deployed fibre in the metropolitan area of Barcelona, Spain, while the photon detection still occurs in the same lab. The resulting visibilities (80% or higher) demonstrate that the photonic qubit does not decohere during transmission through the optical fibre. We then decouple the photon creation and detection by measuring non-classical correlations between signal photons detected in the lab, and idler photons detected 16 km away (44 km in fibre) in a different location. The final experiment uses a fibre-integrated memory for light-matter entanglement. We use a Pr3+:Y2SiO5 crystal containing a Type I laser-written waveguide, interfaced directly with optical fibre. The fibre-integration allows for improved transmission and AFC efficiency compared to a free-space coupled waveguide memory. To analyse the performance of the memory, we demonstrate non-classical correlations for storage times up to 28 µs. We perform qubit tomography in the time basis for storage times of 3 and 10 µs, measuring two-qubit fidelities of 86(2)% and 86(4)%, respectively, demonstrating storage of entanglement. These experiments demonstrate the potential of our system for use as part of a quantum repeater, with many opportunities for further improvement to the storage time, efficiency, and multiplexing capability.
For advanced applications in quantum information and communication the reversible transfer of quantum information between light and matter is essential. A key property of such a light-matter quantum interface is the faithful mapping of entanglement. We report the reversible transfer of photon-photon entanglement into entanglement between a photon and a collective atomic excitation in a thulium-doped lithium niobate waveguide. We use an Atomic Frequency Comb (AFC) memory protocol yielding a 5 GHz acceptance bandwidth of our memory. We reconstruct the bi-photon quantum state before and after the reversible transfer and asses the entanglement-preserving nature of our memory. We demonstrate a near perfect mapping of the entangled state. Additionally, we measure a violation of the CHSH Bell inequality before and after storage, thus directly verifying the sufficiency of the entanglement for quantum communication.
Advanced applications of quantum information science, such as long-distance quantum communication based on quantum repeaters, require photons to be interfaced with different devices. These devices, such as single photon detectors, quantum memories, quantum signal processors, and linear optical elements, may be integrated on a single chip to enable efficient, robust and scalable implementations. With aim of constructing a quantum repeater, and towards realizing integrated optical quantum memories and signal processors in general, we experimentally develop quantum light-matter interfaces using a cryogenically-cooled rare-earth-ion-doped waveguide, namely thulium-doped lithium niobate (Tm3+:LiNbO3). As the basis for our work, we describe a quantum repeater architecture that uses spectral multiplexing and quantum memories that operate with a fixed storage time. Our repeater architecture promises efficient operation, is compatible with the properties of cryogenically-cooled rare-earth-ion-doped crystals, and simplifies the demands of quantum memories compared to other architectures. To demonstrate the feasibility of our repeater design, we utilize our light-matter interface as a quantum memory to perform several experimental demonstrations. These include high-fidelity storage and retrieval of 26 spectrally-multiplexed quantum bits encoded into single-photon-level laser pulses, high-fidelity storage and retrieval of single and entangled photons derived from a photon-pair source, and high-visibility two-photon interference between weak laser pulses that are stored in one or two, separate, quantum memories. The unique properties of our light-matter interface allow us to demonstrate additional protocols that further highlight its promise for integrated quantum signal processing. By combining our Tm3+:LiNbO3 waveguide with a LiNbO3 waveguide phase modulator, we demonstrate operations such as sequencing, filtering, interference, and compression of laser pulses attenuated to the single-photon level. In another experiment, we measure the cross-phase modulation between strong pulses, by which we demonstrate photon-photon interactions that point towards non-destructive measurements of quantum bits. Since the performance of all aforementioned protocols, and future light-matter applications, hinge on the basic spectroscopic properties of our waveguide, we measure these properties at temperatures as low as 800 millikelvin. Our findings, discussed over several attached publications, usher the development of integrated quantum memories and processors for multi-component optical quantum information applications such as repeaters and networks.