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arXiv:1402.0381 · New Journal of Physics

Infrared-dressed entanglement of cold open-shell polar molecules for universal matchgate quantum computing

Felipe Herrera, Yudong Cao, Sabre Kais, K. Birgitta Whaley

Published Jul 4, 2014• 54 citations
arXivHTMLPDF

Abstract

Implementing a scalable quantum information processor using polar molecules in optical lattices requires precise control over the long-range dipole-dipole interaction between molecules in selected lattice sites.We present here a scheme using trapped open-shell Σ 2 polar molecules that allows dipolar exchange processes between nearest and next-nearest neighbors to be controlled in order to construct a generalized transverse Ising spin Hamiltonian with tunable XX, YY and XY couplings in the rotating frame of the driving lasers.The scheme requires a moderately strong bias magnetic field together with near-infrared light to provide local tuning of the qubit energy gap, and mid-infrared pulses to perform rotational state transfer via stimulated Raman adiabatic passage.No interaction between qubits occurs in the absence of the infrared driving.We analyze the fidelity of the resulting two-qubit matchgate, and demonstrate its robustness as a function of the driving parameters.We discuss a realistic application of the system for universal matchgate quantum computing in optical lattices.

DOI
10.1088/1367-2630/16/7/075001

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Implementing a scalable quantum information processor using polar molecules in optical lattices requires precise control over the long-range dipole-dipole interaction between molecules in selected lattice sites.We present here a scheme using trapped open-shell Σ 2 polar molecules that allows dipolar exchange processes between nearest and next-nearest neighbors to be controlled in order to construct a generalized transverse Ising spin Hamiltonian with tunable XX, YY and XY couplings in the rotating frame of the driving lasers.The scheme requires a moderately strong bias magnetic field together with near-infrared light to provide local tuning of the qubit energy gap, and mid-infrared pulses to perform rotational state transfer via stimulated Raman adiabatic passage.No interaction between qubits occurs in the absence of the infrared driving.We analyze the fidelity of the resulting two-qubit matchgate, and demonstrate its robustness as a function of the driving parameters.We discuss a realistic application of the system for universal matchgate quantum computing in optical lattices.
Ultracold polar molecules in optical lattices or tweezer arrays offer a promising platform for quantum information processing and simulation, thanks to their rich internal structure and long-range dipolar interactions. Recent experimental advances now allow precise control over individual molecules, enabling two-qubit gates based on the iSWAP gate. A key challenge is however the sensitivity to variations of the dipole-dipole interaction strength - stemming from motion of the molecules and uncertainty on the precise positioning of external confining potentials - that limits current gate fidelities. To address this, we develop a quantum optimal control framework, based on a perturbative approach, to design gates that are robust with respect to quasi-static deviations of Hamiltonian parameters, and provide criteria to evaluate a priori whether a gate can be made robust for a given control Hamiltonian. By applying these criteria to exchange-coupled qubits, as polar molecules, we demonstrate that robustness cannot be achieved with global controls only, but can be attained by breaking the exchange symmetry through local controls, such as a local detuning. We determine the robust time-optimal solution for realizing an iSWAP gate, show that the control pulses can be designed to be smooth functions, and achieve theoretical gate fidelities compatible with error correction under realistic parameters. Additionally, we show that certain entangled state preparations, such as Bell states, can be made robust even with global controls only. We demonstrate that, under the adiabatic approximation - where molecular motion occurs on timescales faster than that of the exchange interaction - the noise arising from thermal motion can be effectively treated as quasi-static variations of Hamiltonian parameters. This allows us to extend our treatment to the concrete experimental case of polar molecules.
We propose a scalable qudit-based quantum processor using rotational states of polar molecules. Previously, molecular internal states were used to enlarge Hilbert space, whereas our approach uses optical tweezer arrays to achieve scalable architectures with exponential state-space growth without increasing qudit dimensionality d . Entangling gates are implemented by adiabatically bringing traps together to activate dipole-dipole interactions. We develop encoding schemes mapping single qubits into qudits with 2 ≤ d ≤ 5 and pairs of qubits into d = 4 , 5 qudits, enabling universal set of quantum gates. Additional levels in d = 3 and d = 5 qudits simplify multiqubit gate decompositions. We analyze experimental parameters for SrF and NaCs molecules. This approach provides a promising route to scalable quantum information processing with multilevel systems using existing experimental platforms.
Polar molecules are an emerging platform for quantum technologies based on their long-range electric dipole--dipole interactions, which open new possibilities for quantum information processing and the quantum simulation of strongly correlated systems. Here, we use magnetic and microwave fields to design a fast entangling gate with >0.999>0.999>0.999 fidelity and which is robust with respect to fluctuations in the trapping and control fields and to small thermal excitations. These results establish the feasibility to build a scalable quantum processor with a broad range of molecular species in optical-lattice and optical-tweezers setups.
Ultracold polar molecules are promising candidate qubits for quantum computing and quantum simulations. Their long-lived molecular rotational states form robust qubits, and the long-range dipolar interaction between molecules provides quantum entanglement. In this work, we demonstrate dipolar spin-exchange interactions between single calcium monofluoride (CaF) molecules trapped in an optical tweezer array. We realized the spin-[Formula: see text] quantum XY model by encoding an effective spin-[Formula: see text] system into the rotational states of the molecules and used it to generate a Bell state through an iSWAP operation. Conditioned on the verified existence of molecules in both tweezers at the end of the measurement, we obtained a Bell state fidelity of 0.89(6). Using interleaved tweezer arrays, we demonstrate single-site molecular addressability.
There is growing interest to investigate states of matter with topological order, which support excitations in the form of anyons, and which underly topological quantum computing. Examples of such systems include lattice spin models in two dimensions. Here we show that relevant Hamiltonians can be systematically engineered with polar molecules stored in optical lattices, where the spin is represented by a single electron outside a closed shell of a heteronuclear molecule in its rotational ground state. Combining microwave excitation with the dipole-dipole interactions and spin-rotation couplings allows us to build a complete toolbox for effective two-spin interactions with designable range and spatial anisotropy, and with coupling strengths significantly larger than relevant decoherence rates. As an illustration we discuss two models: a 2D square lattice with an energy gap providing for protected quantum memory, and another on stacked triangular lattices leading to topological quantum computing.
Abstract Ultracold polar molecules combine a rich structure of long-lived internal states with access to controllable long-range anisotropic dipole–dipole interactions. In particular, the rotational states of polar molecules confined in optical tweezers or optical lattices may be used to encode interacting qubits for quantum computation or pseudo-spins for simulating quantum magnetism. As with all quantum platforms, the engineering of robust coherent superpositions of states is vital. However, for optically trapped molecules, the coherence time between rotational states is typically limited by inhomogeneous differential light shifts. Here we demonstrate a rotationally magic optical trap for 87 Rb 133 Cs molecules that supports a Ramsey coherence time of 0.78(4) s in the absence of dipole–dipole interactions. This is estimated to extend to >1.4 s at the 95% confidence level using a single spin-echo pulse. In our trap, dipolar interactions become the dominant mechanism by which Ramsey contrast is lost for superpositions that generate oscillating dipoles. By changing the states forming the superposition, we tune the effective dipole moment and show that the coherence time is inversely proportional to the strength of the dipolar interaction. Our work unlocks the full potential of the rotational degree of freedom in molecules for quantum computation and quantum simulation.