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arXiv:1401.7674

Quantum quenches and competing orders: I. Time-dependent Hartree-Fock+BCS theory

Wenbo Fu, Ling-Yan Hung, Subir Sachdev A

Published Jan 29, 2014• 0 citations
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Abstract

We study the non-equlibrium dynamics of an electronic model of competing bond density wave order and $d$-wave superconductivity. In a time-dependent Hartree-Fock+BCS approximation, the dynamics reduces to the equations of motion of operators realizing the generators of SU(4) at each pair of momenta, $(\boldsymbol{k}, -\boldsymbol{k})$, in the Brillouin zone. We compare the results of numerical studies of our model with recent picosecond optical experiments.

DOI
10.48550/arxiv.1401.7674

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We study the non-equlibrium dynamics of an electronic model of competing bond density wave order and ddd-wave superconductivity. In a time-dependent Hartree-Fock+BCS approximation, the dynamics reduces to the equations of motion of operators realizing the generators of SU(4) at each pair of momenta, (k,−k)(\boldsymbol{k}, -\boldsymbol{k})(k,−k), in the Brillouin zone. We compare the results of numerical studies of our model with recent picosecond optical experiments.
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We analyze the effect of pairing on particle transport in time-dependent theories based on the Hartree-Fock-Bogoliubov (HFB) or BCS approximations. The equations of motion for the HFB density matrices are unique and the theory respects the usual conservation laws defined by commutators of the conserved quantity with the Hamiltonian. In contrast, the theories based on the BCS approximation are more problematic. In the usual formulation of time-dependent Hartree-Fock (TDHF)+BCS(\mathrm{TDHF})+\mathrm{BCS}(TDHF)+BCS, the equation of continuity is violated and one sees unphysical oscillations in particle densities. This can be ameliorated by freezing the occupation numbers during the evolution in TDHF+BCS\mathrm{TDHF}+\mathrm{BCS}TDHF+BCS, but there are other problems with the BCS approximation that make it doubtful for reaction dynamics. We also compare different numerical implementations of the time-dependent HFB equations. The equations of motion for the UUU and VVV Bogoliubov transformations are not unique, but it appears that the usual formulation is also the most efficient. Finally, we compare the time-dependent HFB solutions with numerically exact solutions of the two-particle Schr\"odinger equation. Depending on the treatment of the initial state, the HFB dynamics produces a particle emission rate at short times similar to that of the Schr\"odinger equation. At long times, the total particle emission can be quite different, due to inherent mean-field approximation of the HFB theory.
We study the non-equilibrium dynamics of a quantum generalization of a O(6) non-linear sigma model of competing orders in the underdoped cuprates (Hayward {\em et al.}, arXiv:1309.6639). We obtain results, in the large NNN limit of a O(NNN) model, on the time-dependence of correlation functions following a pulse disturbance. We find that the oscillatory responses share various qualitative features with recent optical experiments.
Non-equilibrium aspects of the BCS model have fascinated physicists for decades, from the seminal works of Eliashberg to modern realizations in cold atom experiments. The latter scenarios have lead to a great deal of interest in the quench dynamics of fermions with pairing interactions. The recently introduced notion of a dynamical quantum phase transition is an attempt to classify the myriad of possible phenomena which can result in such far from equilibrium systems. These are defined as non-analytic points of the logarithm of the Loschmidt echo and are linked to oscillations in the dynamics a systems order parameter. In this work we analytically investigate the relation between DQPTs and oscillation of the superconducting order parameter in quenches of the BCS model. We find that each oscillation of the order parameter is accompanied by a DQPT which is first order in nature. We show this for a variety of initial states and furthermore find that when the order parameter attains a constant steady state then no DQPTS occur.
The phase diagrams and superconducting properties of the extended Hubbard model with pair hopping interaction, i.e., the Penson-Kolb-Hubbard model are studied. The analysis of the model is performed for d-dimensional hypercubic lattices, including d=1d=1d=1 and $d=\ensuremath{\infty},$ by means of the (broken symmetry) Hartree-Fock approximations and, for $d=\ensuremath{\infty},$ by the slave-boson mean-field method. For d=1,d=1,d=1, at half filling the phase diagram is shown to consist of nine different phases including two superconducting states with center-of-mass momentum q=0q=0q=0 and q=Qq=Qq=Q $(\ensuremath{\eta}$ pairing), site and bond-located antiferromagnetic and charge-density wave states as well as three mixed phases with coexisting site and bond orderings. The stability range of the bond-type orderings shrinks with increasing lattice dimensionality d and for $d=\ensuremath{\infty}$ the corresponding diagram consists of four phases only, involving exclusively site-located orderings. Comparing the pair hopping model with the attractive Hubbard model we found in both cases gradual evolution from the BCS-like limit to the tightly bound pairs regime and a monotonic increase of the gap in the excitation spectrum with increasing coupling. However, the dynamics of electron pairs in both models is qualitatively different, which results in different dependences of condensation energies and critical temperatures on interaction parameters as well as in different electrodynamic properties, especially in a strong coupling regime.