We provide an introduction to the experimental physics of quantum gases. At the low densities of ultracold quantum gases, confinement can be understood from single-particle physics, and interactions can be understood from two-body physics. The structure of atoms provides resonances both in the optical domain and in the radio-frequency domain. Atomic structure data is given for the 27 atomic isotopes that had been brought to quantum degeneracy at the time this chapter was written. We discuss the motivations behind choosing among these species. We review how static and oscillatory fields are treated mathematically. An electric dipole moment can be induced in a neutral atom, and is the basis for optical manipulation as well as short-range interactions. Many atoms have permanent magnetic dipole moments, which can be used for trapping or long-range interactions. The Toronto $^{40}$K/$^{87}$Rb lattice experiment provides an illustration of how these tools are combined to create an ultracold, quantum-degenerate gas.
We provide an introduction to the experimental physics of quantum gases. At the low densities of ultracold quantum gases, confinement can be understood from single-particle physics, and interactions can be understood from two-body physics. The structure of atoms provides resonances both in the optical domain and in the radio-frequency domain. Atomic structure data is given for the 27 atomic isotopes that had been brought to quantum degeneracy at the time this chapter was written. We discuss the motivations behind choosing among these species. We review how static and oscillatory fields are treated mathematically. An electric dipole moment can be induced in a neutral atom, and is the basis for optical manipulation as well as short-range interactions. Many atoms have permanent magnetic dipole moments, which can be used for trapping or long-range interactions. The Toronto 40K/87Rb lattice experiment provides an illustration of how these tools are combined to create an ultracold, quantum-degenerate gas.
Since the achievement of quantum degeneracy in gases of chromium atoms in 2004, the experimental investigation of ultracold gases made of highly magnetic atoms has blossomed. The field has yielded the observation of many unprecedented phenomena, in particular those in which long-range and anisotropic dipole-dipole interactions (DDIs) play a crucial role. In this review, we aim to present the aspects of the magnetic quantum-gas platform that make it unique for exploring ultracold and quantum physics as well as to give a thorough overview of experimental achievements. Highly magnetic atoms distinguish themselves by the fact that their electronic ground-state configuration possesses a large electronic total angular momentum. This results in a large magnetic moment and a rich electronic transition spectrum. Such transitions are useful for cooling, trapping, and manipulating these atoms. The complex atomic structure and large dipolar moments of these atoms also lead to a dense spectrum of resonances in their two-body scattering behaviour. These resonances can be used to control the interatomic interactions and, in particular, the relative importance of contact over dipolar interactions. These features provide exquisite control knobs for exploring the few- and many-body physics of dipolar quantum gases. The study of dipolar effects in magnetic quantum gases has covered various few-body phenomena that are based on elastic and inelastic anisotropic scattering. Various many-body effects have also been demonstrated. These affect both the shape, stability, dynamics, and excitations of fully polarised repulsive Bose or Fermi gases. Beyond the mean-field instability, strong dipolar interactions competing with slightly weaker contact interactions between magnetic bosons yield new quantum-stabilised states, among which are self-bound droplets, droplet assemblies, and supersolids. Dipolar interactions also deeply affect the physics of atomic gases with an internal degree of freedom as these interactions intrinsically couple spin and atomic motion. Finally, long-range dipolar interactions can stabilise strongly correlated excited states of 1D gases and also impact the physics of lattice-confined systems, both at the spin-polarised level (Hubbard models with off-site interactions) and at the spinful level (XYZ models). In the present manuscript, we aim to provide an extensive overview of the various related experimental achievements up to the present.
Ultracold quantum gases are versatile model systems for exploring quantum physics or for the simulation of solid state materials. Meanwhile, they have been created from various atomic species - from alkali metals over alkaline earths to rare earth elements. The latest addition are quantum gases of different kinds of polar molecules. Expectations for quantum gases of heteronuclear molecules are high: Due to their large electric dipole moments, these molecules can interact with each other via long-range interactions - not just via contact interactions as is the case for most atoms. Additionally, they have vibrational and rotational degrees of freedom, with open up new possibilities for quantum simulation. But the same degrees of freedom also pose some challenges. For example, they make the preparation of the quantum gas more difficult, which is typically produced with a combination of laser cooling and evaporative cooling in the atomic case. Molecules mostly lack closed transitions in their spectra, which are required for laser cooling. Therefore, we create our molecular quantum gas from a mixture of two atomic quantum gases. In this work, such an experimental method was developed for fermionic NaK molecules, which is based on the two-photon process Stimulated Raman Adiabatic Passage (STIRAP). Within STIRAP, the hyperfine structure of the chosen intermediate state plays an important role. Experimentally, and with the help of a theoretical model describing the whole process, we find that we produce the most molecules when we use a large one-photon detuning, if the hyperfine structure of the intermediate state is unresolved. In another project, we explored the rotational level structure of the molecular ground state populated by STIRAP. Rotation is closely linked to the electric dipole moment. The superposition of the ground state with the first excited rotational state, for example, has a transition dipole moment of almost 60% of the permanent electric dipole moment. Unfortunately, coherence times of such superpositions are typically short, as the different polarizabilities of the rotational states lead to dephasing in optical traps. However, using a special polarization angle and a small, dc electric field, we can compensate these differences and realize a spin-decoupled magic trap. With this new technique we obtain record coherence times, at least for small molecular densities. For larger densities we observe first indications for dipolar interactions in a bulk gas of polar molecules, which we also model using the moving-average cluster expansion (MACE).
Physics of ultra cold atoms and molecules is one of the most rapidly developing areas of the modern atomic, molecular, optical physics and quantum optics.This area covers several sub-areas of diverse importance, but definitely two trends can be easily identifies: i) fundamental research on properties of ultra cold atoms and molecules, and in particular atomic and molecular condensates trapped and lattice gases; here the fundamental questions of nature and form of phase transitions in degenerate systems are being posed and studied; ii) more applications oriented research on ultracold atoms and molecules, involving in particular applications in precision measurements, atomic clocks, frequency standards, atom and molecule interferometry, quantum information, quantum engineering, "super" chemistry etc.This thesis concerns both of these major trends.The applications, or more specifically quantum engineering aspect are discussed in the first four chapters of the thesis, which deal with optical manipulations of ultra cold gases, in particular optical generation of vortices in Bose condensates, quasi-solitons in Fermi gases, and retarded dipole-dipole interactions in Bose, or Fermi gases.This thesis consists of four main chapters.Chapter 2, "Optical generation of vortices in Bose Einstein Condensates".In this chapter we study theoretically the generation of vortices by phase imprinting in trapped Bose-Einstein condensates.Phase imprinting is achieved by passing a short off-resonance laser pulse through an appropriately designed absorption plate, and impinging it on a condensate.We answer the fundamental question of how the circulation and the vortex are introduced into the system, and discuss the creation of vortex arrays.We discuss vortex dynamics and interactions in such configurations.Various methods of vortex detection based on interference combined with Bragg scattering are also analyzed.In Chapter 3, "Fermionic 'Solitons'" we investigate in detail the concept of low energy excitations of ultra cold Fermi gases.This excitations are generated using the same idea of phase imprinting as that employed in the generation of vortices in BEC.We address in this chapter some questions concerning the generation (via phase imprinting) of soliton-like solutions in a single-component Fermi gas of neutral atoms at zero and finite temperatures.By using both numerical and analytical calculations, we find the conditions under which it is possible to find in non-interacting Fermi gases, quasisolitons which resemble the properties of solitons in non-linear integrable equations.We present the results for both spatially homogeneous and trapped cases, and emphasize the importance of Fermi statistics and the absence of interactions for the existence of such solutions.In Chapter 4, "Generating Dipole Condensate" we keep studying the possibilities of optical manipulations of ultracold gases.In particular, we study two different ways to laser-induce dipole-dipole interactions in trapped Bose-Einstein condensates.The first one employs the fact that those atoms in high Rydberg states posses a large dipolar moment.We first analyze the idea of imposing the dipole moment as a time average over short stroboscopic pulses.These pulses are coherently transporting the atoms from the ground atomic state to some high Rydberg state and back.The second idea is based on the observation that in strong static or oscillatory electric fields, atoms polarize and acquire dipole moment.We analyze the possibilities and limitations of inducing such a high electric field using lasers of low frequency.In Chapter 5, "Dipolar BCS", we continue our study of trapped fermionic gases, with the analysis of the BCS transition in trapped dipolar fermionic gases.We find that the critical strength of the dipole-dipole interaction to achieve BCS pairing, depends on the trap geometry.We find the particular form of this dependence, and present the solutions for the order parameter.This first chapter is meant as a general introduction to the thesis.This introduction is by no means exhaustive, and should be rather treated as a collection of basic facts concerning ultra cold gases, without rigorous derivations.The last subsection of the introductory chapter, discusses very briefly the most important achievements and trends in the field and the current state of the art.
This thesis discusses two important topics in ultracold atomic gases: strong interactions in quantum gases, and quantum Hall physics in neutral atoms.First we give a brief introduction on basic scattering models in atomic physics, and an approach to adjust the interactions between atoms.We also include a list of experimental probes in cold atom physics.After these introductions, in Chapter 3, we report a few interesting problems in strongly interacting quantum gases.We introduce the BCS-BEC crossover model and relevant many-body techniques at the beginning, and discuss the details of several specific systems.We find the Fermi gases across narrow Feshbach resonances are strongly interacting at low temperature even when the magnetic field is several widths away from the resonance.We also discuss an approach to describe the metastable repulsive branch of Bose and Fermi gases across the resonance, and find a stable region of repulsive Bose gas close to unitarity.Some studies in two dimensional Fermi gases with spin imbalance are also included, and they are closely related to a number of recent experiments.In Chapter 4, we discuss quantum Hall physics in the context of neutral atomic gases.After illustrating how the Berry phase experienced by neutral atoms is equivalent to the magnetic field in electrons, we introduce the newly developed synthetic gauge field scheme in which a gauge potential is coupled to the neutral atoms.We give a detail introduction to this Raman coupling scheme developed by NIST group, and derive the theoretical model of the system.Then we make some predictions on the evolution of quantum Hall states when an extra anisotropy is applied from the external trap.Finally, we propose some experiments to verify our predictions.4.9 Phase diagram of the cloud in rotating anisotropic traps: two phases of the BEC and QH are identified. . . . . . . . . . . . . . . . . . . . . . . . . . . .4.10 Distortion and transition in vortex lattices of a rapidly rotating BEC in an anisotropic trap. . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . .4.11 Density profiles at cut x = 0 and y = 0 of the Laughlin wavefunctions at different positions in figure 4.9. . . . . . . . . . . . . . . . . . . . . . . . . .4.12 Distribution of zeros in the relative coordinate of the ground state of two body problem in rotating anisotropic traps. . . . . . . . . . . . . . . . . . .4.13 Variation in the distance of splitting zeros as a function of inverse interaction strength, for fixed anisotropy α = 0.96. . . . . . . . . . . . . . . . . . . . . .4.14 Density profiles after TOF expansion of the gas in a rotating isotropic trap.4.15 Density profiles after TOF expansion of anisotropy α = 0.94. . . . . . . . .4.16 Second order correlation in equation 4.64, in a rotating isotropic (left) and anisotropic (right) trap. . . . . . . . . . . . . . . . . . . . . . . . . . . . . .4.17 A sketch of high-resolution in situ imaging technique in neutral atoms. . . .4.18 In situ images of the quantity |ψ(r/2, -r/2)| for an anisotropy α = 0.96. .x
This tutorial is a theoretical work, in which we study the physics of ultra-cold dipolar bosonic gases in optical lattices. Such gases consist of bosonic atoms or molecules that interact via dipolar forces, and that are cooled below the quantum degeneracy temperature, typically in the nK range. When such a degenerate quantum gas is loaded into an optical lattice produced by standing waves of laser light, new kinds of physical phenomena occur. These systems realize then extended Hubbard-type models, and can be brought to a strongly correlated regime. The physical properties of such gases, dominated by the long-range, anisotropic dipole-dipole interactions, are discussed using the mean-field approximations, and exact Quantum Monte Carlo techniques (the Worm algorithm).
Interactions between particles play an important role in quantum degenerate gases.\nIn fact, the system’s behavior is usually largely determined by the strength, range, and\nsymmetry of the interactions, even if very weak. For more than two decades after the\nfirst experimental realization of a Bose-Einstein condensate (BEC) in 1995, investigations of ultracold atomic gases have mainly considered contact-type interactions, which\nmodel the short-range van der Waals interactions between the atoms in terms of a single\nparameter, the s-wave scattering length. However, some atomic or molecules species\npossess a magnetic or electric dipole moment and additionally interact among each\nother via the dipole-dipole interaction (DDI), which is long-ranged and anisotropic.\nSignatures of the DDI have been first observed in a BEC of chromium atoms in 2005.\nIn the last several years, a new class of atoms from the lanthanide series, e.g., dysprosium and erbium, with stronger dipolar properties, have come into play. This permits\na more full-fledged study of dipolar effects in BECs. Furthermore, ultracold molecules\nand highly excited Rydberg atoms are other promising examples for futures studies of\nsystems where dipolar interaction will be even more dominant, but they still need experimental efforts to achieve the desired quantum regime. Whereas the weak DDI in a\nchromium BEC is well described with the Gross-Pitaevskii equation, stronger dipolar\ninteractions certainly necessitate a beyond-mean-field description within a Bogoliubov\ntheory.\nIn parallel to research on bosons, cold fermions also trigger great interest because\nthey are actually often found in nature, e.g., within the electron gas of metals, as\nneutrons of heavy stars, or as quarks in plasmas as constituent elements of composite particles. Contrary to Bose systems, quantum degeneracy in experiments is much\nmore difficult to achieve in Fermi systems, since s-wave scattering is absent between\nidentical fermions, due to the Pauli exclusion principle. It was first achieved in 1999\nfor alkali atoms using a technique based on the sympathetic cooling with a second spin\nstate, another species, or a different isotope. For highly magnetic atoms, quantum degeneracy was achieved for dysprosium in 2012 using the standard sympathetic cooling\ntechnique, while in 2014 erbium was cooled deep into the degenerate regime using a\ndirect evaporative cooling mediated by dipolar collisions. This direct cooling scheme\nivallows producing very dense Fermi gas down to 10% of the Fermi temperature.\nFurthermore, a novel kind of strongly dipolar quantum gases became available in\nthe last several years. These are weakly bound polar molecules produced from atoms\nwith large magnetic dipole moments, such as erbium. Only very recently a quantum\ndegenerate dipolar Fermi gas of potassium-rubidium molecules has been experimentally realized. Unlike previously considered magnetic systems, heteronuclear molecules\nsuch as potassium-rubidium possess large electric dipole moments. The next natural\nstep is to polarize this system in a preferential direction by an external electric field,\nsuch that the DDI dominates the behavior of the system, which would open up the\nrealm for experimental investigation of strong dipolar Fermi gases...