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arXiv:1401.0520 · Physical Review A

Bose-Einstein condensation of light in a cavity

Alexander Kruchkov

Published Mar 31, 2014• 24 citations
arXivHTMLPDF

Abstract

The paper considers Bose-Einstein condensation (BEC) of light in a cavity with a medium. In the framework of a two-level model we show the effect of gaseous medium on the critical temperature of light condensation in the system. Transition of the system to the state with released light condensate is illustrated in consequent stages. Analytical expressions for a typical spatial extent of the condensed cloud of photons, as well for spectral characteristics of the condensate peak are derived. Energy and heat capacity of photons as functions of temperature are obtained. Finally, we demonstrate that the energy of light can be accumulated in the BEC state.

DOI
10.1103/physreva.89.033862

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The paper considers Bose-Einstein condensation (BEC) of light in a cavity with a medium. In the framework of a two-level model we show the effect of gaseous medium on the critical temperature of light condensation in the system. Transition of the system to the state with released light condensate is illustrated in consequent stages. Analytical expressions for a typical spatial extent of the condensed cloud of photons, as well for spectral characteristics of the condensate peak are derived. Energy and heat capacity of photons as functions of temperature are obtained. Finally, we demonstrate that the energy of light can be accumulated in the BEC state.
Bose-Einstein condensation, the macroscopic ground state occupation of a system of bosonic particles below a critical temperature, has been observed in cold atomic gases and solid-state physics quasiparticles. In contrast, photons do not show this phase transition usually, because in Planck's blackbody radiation the particle number is not conserved and at low temperature the photons disappear in the walls of the system. Here we report on the realization of a photon Bose-Einstein condensate in a dye-filled optical microcavity, which acts as a "white-wall" photon box. The cavity mirrors provide a trapping potential and a non-vanishing effective photon mass, making the system formally equivalent to a two-dimensional gas of trapped massive bosons. Thermalization of the photon gas is reached in a number conserving way by multiple scattering off the dye molecules. Signatures for a BEC upon increased photon density are: a spectral distribution that shows Bose-Einstein distributed photon energies with a macroscopically populated peak on top of a broad thermal wing, the observed threshold of the phase transition showing the predicted absolute value and scaling with resonator geometry, and condensation appearing at the trap centre even for a spatially displaced pump spot.
Bose-Einstein condensation (BEC) is the transition to a macroscopic occupation of the ground state of a system of bosonic particles. In 1995 the first experimental realization of BEC was achieved by condensing a dilute atomic gas [1,2]. It was long thought only massive particles could undergo BEC. However, in 2010 it was shown that photon BEC was achieved in an optical dye-filled microcavity [3]. In 2015, we became the second group to successfully repeat these experiments.\n\nBEC is a phase transition and thus it occurs at thermal equilibrium. To achieve a thermal photon gas the cavity is filled with a fluorescent dye solution. The dye molecules thermalize the photons by means of repeated absorption-emission cycles. We optically pump the cavity. With the pump we determine the number of photons absorbed by the dye, consequently defining a nonvanishing chemical potential. This ensures a conserved photon number. The photons are trapped by the harmonic potential induced by the concave cavity mirrors. Due to the cutoff energy determined by the cavity length, the trapped photons have a dispersion similar to that of a massive particle in a quantum harmonic oscillator. The cavity length is tuned such that the free spectral range is larger than the bandwidth of the dye. Therefore, only one longitudinal mode fits inside the cavity, making the photon gas effectively two-dimensional. We end up with a thermalized two-dimensional photon gas that has the eigenenergies of a quantum harmonic oscillator. The Bose-Einstein distribution function predicts a critical photon number. Pumping the thermal photon gas beyond this critical number will lead to photon BEC.\n\nWe measure the spectral- and spatial distributions of our two-dimensional photon gas. In both distributions we observe photon BEC. Results show the characteristics of a phase transition: the appearance of a sharp peak on top of the thermal cloud that coincides with a converging chemical potential to zero. Both the spectral- and spatial distribution are in agreement with the theoretical distribution of photons with an effective mass in a quantum harmonic oscillator. Expansion of the condensate has been measured. This could indicate nonlinear optical effects such as thermal lensing or repulsive photon-photon interactions.
We review recent experiments on the Bose-Einstein condensation of photons in a dye-filled optical microresonator. The most well-known example of a photon gas, photons in blackbody radiation, does not show Bose-Einstein condensation. Instead of massively populating the cavity ground mode, photons vanish in the cavity walls when they are cooled down. The situation is different in an ultrashort optical cavity imprinting a low-frequency cutoff on the photon energy spectrum that is well above the thermal energy. The latter allows for a thermalization process in which both temperature and photon number can be tuned independently of each other or, correspondingly, for a nonvanishing photon chemical potential. We here describe experiments demonstrating the fluorescence-induced thermalization and Bose-Einstein condensation of a two-dimensional photon gas in the dye microcavity. Moreover, recent measurements on the photon statistics of the condensate, showing Bose-Einstein condensation in the grand-canonical ensemble limit, will be reviewed. Introduction Quantum statistical effects become relevant when a gas of particles is cooled, or its density is increased, to the point where the associated de Broglie wavepackets spatially overlap. For particles with integer spin (bosons), the phenomenon of Bose-Einstein condensation (BEC) then leads to macroscopic occupation of a single quantum state at finite temperatures [1]. Bose-Einstein condensation in the gaseous case was first achieved in 1995 by laser and subsequent evaporative cooling of a dilute cloud of alkali atoms [2, 3, 4], as detailed in Chapter 3 of this volume. The condensate atoms can be described by a macroscopic singleparticle wavefunction, similar to the case of liquid helium [1]. Bose-Einstein condensation has also been observed for exciton-polaritons, which are hybrid states of matter and light [5, 6, 7] (see Chapter 4), magnons [8] (see Chapter 25), and other physical systems. Other than material particles, photons usually do not show Bose-Einstein condensation [9]. In blackbody radiation, the most common Bose gas, photons at low temperature disappear, instead of condensing to a macroscopically occupied ground-state mode. In this system, photons have a vanishing chemical potential, meaning that the number of photons is determined by the available thermal energy and cannot be tuned independently from temperature.
We have studied conditions of photon Bose-Einstein condensate formation that is in thermodynamic equilibrium with ideal gas of two-level Bose atoms below the degeneracy temperature.Equations describing thermodynamic equilibrium in the system were formulated; critical temperatures and densities of photonic and atomic gas subsystems were obtained analytically.Coexistence conditions of these photonic and atomic Bose-Einstein condensates were found.There was predicted the possibility of an abrupt type of photon condensation in the presence of Bose condensate of ground-state atoms: it was shown that the slightest decrease of the temperature could cause a significant gathering of photons in the condensate.This case could be treated as a simple model of the situation known as "stopped light" in cold atomic gas.We also showed how population inversion of atomic levels can be created by lowering the temperature.The latter situation looks promising for light accumulation in atomic vapor at very low temperatures.
A Bose-Einstein condensate (BEC) is a quantum phase of matter achieved at low temperatures. Photons, one of the most prominent species of bosons, do not typically condense due to the lack of a particle number conservation. We recently described a photon thermalization mechanism which gives rise to a grand canonical ensemble of light with effective photon number conservation between a subsystem and a particle reservoir. This mechanism occurs during Doppler laser cooling of atoms where the atoms serve as a temperature reservoir while the cooling laser photons serve as a particle reservoir. In contrast to typical discussions of BEC, our system is better treated with a controlled chemical potential rather than a controlled particle number, and is subject to energy-dependent loss. Here, we address the question of the possibility of a BEC of photons in this laser cooling photon thermalization scenario and theoretically demonstrate that a Bose condensation of photons can be realized by cooling an ensemble of two-level atoms (realizable with alkaline-earth atoms) inside a Fabry-Pérot cavity.
We study peculiarities of Bose-Einstein condensation of photons that are in thermodynamic equilibrium with atoms of noninteracting gases. General equations of the thermodynamic equilibrium of the system under study are obtained. We examine solutions of these equations in the case of high temperatures, when the atomic components of the system can be considered as nondegenerated ideal gases of atoms, and the photonic component can form a state with the Bose condensate. Transcendental equation for transition temperature and expression for the density of condensed photons in the considered system are derived. We also obtain analytical solutions of the equation for the critical temperature in a number of particular cases. The existence of two regimes of Bose condensation of photons, which differ significantly in nature of transition temperature dependence on the total density of photons pumped into the system, is revealed. In one case, this dependence is a traditional fractional-power law, and in another one it is the logarithmic law. Applying numerical methods, we determine boundaries of existence and implementation conditions for different regimes of condensation depending on the physical parameters of the system under study. We also show that for a large range of physical systems that are in equilibrium with photons (from ultracold gases of alkali metals to certain types of ideal plasma), the condensation of photons should occur according to the logarithmic regime.