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arXiv:1312.2719 · Physical Review B

Linear response of a one-dimensional conductor coupled to a dynamical impurity with a Fermi edge singularity

Izak Snyman

Published Feb 18, 2014• 1 citation
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Abstract

I study the dynamical correlations that a quantum impurity induces in the Fermi sea to which it is coupled. I consider a quantum transport setup in which the impurity can be realized in a double quantum dot. The same Hamiltonian describes tunneling states in metallic glasses, and can be mapped onto the Ohmic spin-boson model. It exhibits a Fermi edge singularity, i.e., many fermion correlations result in an impurity decay rate with a nontrivial power-law energy dependence. I show that there is a simple relation between temporal impurity correlations on the one hand and the linear response of the Fermi sea to external perturbations on the other. This results in a power-law singularity in the space and time dependence of the nonlocal polarizability of the Fermi sea, which can be detected in transport experiments.

DOI
10.1103/physrevb.89.085118

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I study the dynamical correlations that a quantum impurity induces in the Fermi sea to which it is coupled. I consider a quantum transport setup in which the impurity can be realized in a double quantum dot. The same Hamiltonian describes tunneling states in metallic glasses, and can be mapped onto the Ohmic spin-boson model. It exhibits a Fermi edge singularity, i.e., many fermion correlations result in an impurity decay rate with a nontrivial power-law energy dependence. I show that there is a simple relation between temporal impurity correlations on the one hand and the linear response of the Fermi sea to external perturbations on the other. This results in a power-law singularity in the space and time dependence of the nonlocal polarizability of the Fermi sea, which can be detected in transport experiments.
We study spatial correlations in the ground state of a one-dimensional electron gas coupled to a dynamic quantum impurity. The system displays a nontrivial many-body effect known as the Fermi edge singularity: transitions between discrete internal states of the impurity have a power-law dependence on the internal energies of the impurity states. We present compact formulas for the static current-current correlator and the pair-correlation function. These reveal that spatial correlations induced by the impurity decay slowly (as the third inverse power of distance) and have a power-law energy dependence, characteristic of the Fermi edge singularity.
We consider a fixed impurity immersed in a Fermi gas at arbitrary temperature. We take the impurity to have two internal spin states where the $\ensuremath{\uparrow}$ state is assumed to interact with the medium such that it exhibits the orthogonality catastrophe, whereas the $\ensuremath{\downarrow}$ state is a bare noninteracting particle. Introducing a Rabi coupling between the impurity states, therefore, allows us to investigate the coupling between a discrete spectral peak and the Fermi-edge singularity, i.e., between states with and without a quasiparticle residue. Combining an exact treatment of the uncoupled impurity Green's functions with a variational approach to treat the Rabi driven dynamics, we find that the system features Rabi oscillations whose frequency scales as a nontrivial power of the Rabi drive at low temperatures. This reflects the power law of the Fermi-edge singularity and, importantly, this behavior is qualitatively different from the case of a mobile impurity quasiparticle where the scaling is linear. We, therefore, argue that the scaling law serves as an experimentally implementable probe of the orthogonality catastrophe. We additionally simulate rf spectroscopy beyond linear response, finding a remarkable agreement with an experiment using heavy impurities [Kohstall et al., Nature 485, 615 (2012)], thus, demonstrating the power of our approach.
Effects of long-range Coulomb interactions on the Fermi-edge singularity in optical spectra are investigated theoretically for one-dimensional spin-1/2 fermion systems with the use of the Tomonaga-Luttinger bosonization technique. Low-energy excitation spectrum near the Fermi level shows that dispersion of the charge-density fluctuation remains gapless but is nonlinear when the electron-electron (e-e) Coulomb interaction is of the ${\mathit{x}}^{\mathrm{\ensuremath{-}}1}$ type (i.e., an infinite force range). Temporal behavior of the current-current correlation function is calculated analytically for arbitrary force ranges, ${\ensuremath{\lambda}}_{\mathit{e}}$ and ${\ensuremath{\lambda}}_{\mathit{h}}$, of the e-e and the electron-hole (e-h) Coulomb interactions. (i) When both the e-e and the e-h interactions have large but finite force ranges (${\ensuremath{\lambda}}_{\mathit{e}}$\ensuremath{\infty} and ${\ensuremath{\lambda}}_{\mathit{h}}$\ensuremath{\infty}), the correlation function yields a power-law decay only for a long-time regime, which is determined by the force ranges as t>max[${\ensuremath{\lambda}}_{\mathit{e}}$,${\ensuremath{\lambda}}_{\mathit{h}}$]/vF{\mathit{v}}_{\mathit{F}}vF​. Corresponding optical spectrum near the Fermi edge (within an energy range of \ensuremath{\Elzxh}vF{\mathit{v}}_{\mathit{F}}vF​/max[${\ensuremath{\lambda}}_{\mathit{e}}$,${\ensuremath{\lambda}}_{\mathit{h}}$]) exhibits the power-law divergence or the power-law convergence, which is an ordinary Fermi-edge singularity. (ii) When either the e-e or the e-h interaction is of the ${\mathit{x}}^{\mathrm{\ensuremath{-}}1}$ type (i.e., ${\ensuremath{\lambda}}_{\mathit{e}}$\ensuremath{\rightarrow}\ensuremath{\infty} and/or ${\ensuremath{\lambda}}_{\mathit{h}}$\ensuremath{\rightarrow}\ensuremath{\infty}), an exponent of the correlation function is dependent on time to lead the faster decay than that of any power laws. Then the optical spectra show no power-law dependence and always converge (become zero) at the Fermi edge, which is in striking contrast to the ordinary power-law singularity. Relations between the spectral shape and a measurement time (frequency resolution) are also clarified. \textcopyright{} 1996 The American Physical Society.
A systematic study is performed on time-dependent dynamic transport characteristics of a side-coupled double-quantum-impurity system based on the hierarchical equations of motion. It is found that the transport current behaves like a single quantum dot when the coupling strength is low during tunneling or Coulomb coupling. For the case of only tunneling transition, the dynamic current oscillates due to the temporal coherence of the electron tunneling device. The oscillation frequency of the transport current is related to the step voltage applied by the lead, while temperature T, electron–electron interaction U and the bandwidth W have little influence. The amplitude of the current oscillation exists in positive correlation with W and negative correlation with U. With the increase in coupling t 12 between impurities, the ground state of the system changes from a Kondo singlet of one impurity to a spin singlet of two impurities. Moreover, lowering the temperature could promote the Kondo effect to intensify the oscillation of the dynamic current. When only the Coulomb transition is coupled, it is found that the two split-off Hubbard peaks move upward and have different interference effects on the Kondo peak at the Fermi surface with the increase in U 12, from the dynamics point of view.
This thesis contributes to the understanding of impurity models. It is divided into two main parts, with a general introduction given in Part I and the research related to it presented in Part II, with the second part being subdivided into two main projects. In the first project, the influence of two many-body effects, the Kondo effect and the Fermi edge singularity, on the absorption and emission spectra of self-assembled quantum dots (QDs) is examined. Whereas the Kondo effect so far was always examined with transport experiments, we show that it has been observed with optical methods for the first time, by comparing experimental data for the absorption line shapes of QDs to calculations with the numerical renormalization group. We continue by examining a QD with strong optical coupling of the energy levels. The resulting interplay of Rabi-oscillations and Kondo effect leads to a new many-body state, a secondary, outer Kondo effect, with Kondo-like correlations between the spin-Kondo and the trion state. The last work regarding optics at QDs addresses the Fermi edge singularity. We show that for QDs this phenomenon can be described numerically on a quantitative level. The second project concerns transport properties of impurity models. First, we present a comprehensive study of the Kondo effect for an InAs-nanowire QD, a system for which the Kondo effect was observed only a few years ago. The second study regarding transport concerns the Kondo effect in bulk metals with magnetic impurities. Although nowadays the Kondo effect is often studied with QDs, it was discovered for iron impurities in noble metals like gold and silver. However, it was unknown for a long time which exact realization of Kondo model describes these systems. We identify the model by comparing numerical calculations for the magnetoresistivity and the dephasing rate for different models to experimental results. The third work about transport concerns the phenomenon that for a fixed type of Kondo model quantities like the magnetoresistivity or the conductivity, respectively, can be scaled onto a universal curve for different parameters, when energies are rescaled with the the Kondo temperature TKT_KTK​, since it is the only relevant low energy scale of the problem. For finite bandwidth, however, different definitions of TKT_KTK​ (which coincide in the limit of infinite bandwidth) lead to different TKT_KTK​-values. We show that with a very common definition of TKT_KTK​, finite bandwidth, which is always present at numerical calculations, can deteriorate the universality of rescaled curves, and we offer an alternative definition of TKT_KTK​ which ensures proper scaling. In the last study presented in this thesis we calculate the Fermi-liquid coefficients for fully screened multi-channel Kondo models. For temperatures below TKT_KTK​, these models show Fermi-liquid behavior, and the impurity density of states and certain quantities which depend on it, like resistivity, show quadratic dependencies on parameters like temperature or magnetic field, described by the Fermi-liquid coefficients. We calculate these coefficients both analytically and numerically.
We study transport through a one-dimensional quantum wire of correlated fermions connected to semi-infinite leads. The wire contains either a single impurity or two barriers, the latter allowing for resonant tunneling. In the leads the fermions are assumed to be noninteracting. The wire is described by a microscopic lattice model. Using the functional renormalization group we calculate the linear conductance for wires of mesoscopic length and for all relevant temperature scales. For a single impurity, either strong or weak, we find power-law behavior as a function of temperature. In addition, we can describe the complete crossover from the weak- to the strong-impurity limit. For two barriers, depending on the parameters of the enclosed quantum dot, we find temperature regimes in which the conductance follows power laws with ``universal'' exponents as well as nonuniversal behavior. Our approach leads to a comprehensive picture of resonant tunneling. We compare our results with those of alternative approaches.