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arXiv:1311.5110 · Physical Review Letters

Spin Waves and Dielectric Softening of Polar Molecule Condensates

Ryan Wilson, Brandon M. Peden, Charles W. Clark, Seth T. Rittenhouse

Published Apr 1, 2014• 3 citations
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Abstract

We consider an oblate Bose-Einstein condensate of heteronuclear polar molecules in a weak applied electric field. This system supports a rich quasiparticle spectrum that plays a critical role in determining its bulk dielectric properties. In particular, in sufficiently weak fields the system undergoes a polarization wave rotonization, leading to the development of textured electronic structure and a dielectric instability that is characteristic of the onset of a negative static dielectric function.

DOI
10.1103/physrevlett.112.135301

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We consider an oblate Bose-Einstein condensate of heteronuclear polar molecules in a weak applied electric field. This system supports a rich quasiparticle spectrum that plays a critical role in determining its bulk dielectric properties. In particular, in sufficiently weak fields the system undergoes a polarization wave rotonization, leading to the development of textured electronic structure and a dielectric instability that is characteristic of the onset of a negative static dielectric function.
We show that, under achievable experimental conditions, a Bose–Einstein condensate of polar molecules can exhibit dielectric character. In particular, we derive a set of self-consistent mean-field equations that couple the condensate density to its electric dipole field, leading to the emergence of polarization modes that are coupled to the rich quasi-particle spectrum of the condensate. While the usual roton instability is suppressed in this system, the coupling can give rise to a phonon-like instability that is characteristic of a dielectric material with a negative static dielectric function.
We investigate the properties of the ground state and low-lying excitations of an oblate Bose-Einstein condensate composed of rigid rotor molecules in the presence of an external polarizing electric field. We build in a quantum model of molecular polarizability by including the full manifold of rotational states. The interplay between spatial and microscopic degrees of freedom via feedback between the molecular polarizability and inter-molecular dipole-dipole interactions leads to a rich quasi-particle spectrum. Under large applied fields, we reproduce the well-understood density-wave rotonization that appears in a fully polarized dipolar BEC, but under smaller applied fields, we predict the emergence of a spin wave instability and possible new stable ground state phases.
Abstract We consider a BEC of rigid rotor molecules confined to quasi-2D through harmonic trapping. The molecules are subjected to an external electric field which polarizes the gas, and the molecules interact via dipole–dipole interactions. We present a description of the ground state and low-energy excitations of the system including an analysis of the mean-field energy, polarization, and stability. Under large electric fields the gas becomes fully polarized and we reproduce a well known density-wave instability which arises in polar BECs. Under smaller applied electric fields the gas develops an in-plane polarization leading to the emergence of a new global instability as the molecules ‘tilt’. The character of these instabilities is clarified by means of momentum-space density–density structure factors. A peak at zero momentum in the spin–spin structure factor for the in-plane component of the polarization indicates that the tilt instability is a global phonon-like instability.
We present an analytic Bogoliubov description of a Bose-Einstein condensate of polar molecules trapped in a quasi-two-dimensional geometry and interacting via internal state-dependent dipole-dipole interactions. We derive the mean-field ground-state energy functional, and we derive analytic expressions for the dispersion relations, Bogoliubov amplitudes, and static structure factors. This method can be applied to any homogeneous, two-component system with linear coupling and direct, momentum-dependent interactions. The properties of the mean-field ground state, including polarization and stability, are investigated, and we identify three distinct instabilities: a density-wave rotonization that occurs when the gas is fully polarized, a spin-wave rotonization that occurs near zero polarization, and a mixed instability at intermediate fields. The nature of these instabilities is clarified by means of the real-space density-density correlation functions, which characterize the spontaneous fluctuations of the ground state, and the momentum-space structure factors, which characterize the response of the system to external perturbations. We find that the gas is susceptible to both density-wave and spin-wave responses in the polarized limit but only a spin-wave response in the zero-polarization limit. These results are relevant for experiments with rigid rotor molecules such as RbCs, $\mathrm{\ensuremath{\Lambda}}$-doublet molecules such as ThO that have an anomalously small zero-field splitting, and doublet-$\mathrm{\ensuremath{\Sigma}}$ molecules such as SrF where two low-lying opposite-parity states can be tuned to zero splitting by an external magnetic field.
We develop theory for a flattened dipolar Bose–Einstein condensate produced by harmonic confinement along one direction. The role of both short-ranged contact interactions and long-ranged dipole–dipole interactions is considered, and the dipoles are allowed to be polarized along an arbitrary direction. We discuss the symmetry properties of the condensate and the part of the excitation spectrum determining stability, and introduce two effective interaction parameters that allow us to provide a general description of the condensate properties, rotons, and stability. We diagonalize the full theory to obtain benchmark results for the condensate and quasiparticle excitations, and characterize the exact mean field stability of the system. We provide a unified formulation for a number of approximate schemes to describe the condensate and quasiparticles, including the standard quasi-two-dimensional approximation, two kinds of variational ansatz, and a Thomas–Fermi approximation. Some of these schemes have been widely used in the literature despite not being substantiated against the exact theory. We provide this validation and establish the regimes where the various theories perform well.