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arXiv:1311.3395 · New Journal of Physics

Low-temperature pseudogap phenomenon: precursor of high-Tcsuperconductivity

Yao Ma, Peng Ye, Zheng-Yu Weng

Published Aug 26, 2014• 22 citations
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Abstract

In this paper, we try to understand the pseudogap phenomenon observed in the cuprate superconductor through a model study. Specifically, we explore the so-called low-temperature pseudogap state by turning off the superconducting (SC) off diagonal long range order in an ansatz state for the t – J model (Weng 2011 New J. Phys. 13 103039 ). Besides strong non-Gaussian SC fluctuations, the resulting state also exhibits a systematic pseudogap behavior in both spin and charge degrees of freedom, manifested in the uniform spin susceptibility, specific heat, non-Drude resistivity, Nernst effect, as well as the quantum oscillation associated with small Fermi pockets emerging in strong magnetic fields, etc. These anomalous 'normal state' properties are found in qualitative consistency with experimental measurements in the cuprates. Such a model study establishes an intrinsic connection between the peculiar pseudogap properties and the non-BCS nature of the SC ground state. A critical comparison with other approaches to the doped Mott insulator is also made.

DOI
10.1088/1367-2630/16/8/083039

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In this paper, we try to understand the pseudogap phenomenon observed in the cuprate superconductor through a model study. Specifically, we explore the so-called low-temperature pseudogap state by turning off the superconducting (SC) off diagonal long range order in an ansatz state for the t – J model (Weng 2011 New J. Phys. 13 103039 ). Besides strong non-Gaussian SC fluctuations, the resulting state also exhibits a systematic pseudogap behavior in both spin and charge degrees of freedom, manifested in the uniform spin susceptibility, specific heat, non-Drude resistivity, Nernst effect, as well as the quantum oscillation associated with small Fermi pockets emerging in strong magnetic fields, etc. These anomalous 'normal state' properties are found in qualitative consistency with experimental measurements in the cuprates. Such a model study establishes an intrinsic connection between the peculiar pseudogap properties and the non-BCS nature of the SC ground state. A critical comparison with other approaches to the doped Mott insulator is also made.
The pseudogap state of cuprate high-temperature superconductors has been often viewed as either a yet unknown competing order or a precursor state to superconductivity. While awaiting the resolution of the pseudogap problem in cuprates, we demonstrate that local pairing fluctuations, vortex liquid dynamics, and other precursor phenomena can emerge quite generally whenever fermionic excitations remain gapped across the superconducting transition, regardless of the gap origin. Our choice of a tractable model is a lattice band insulator with short-range attractive interactions between fermions in the sss-wave channel. An effective crossover between Bardeen-Cooper-Schrieffer (BCS) and Bose-Einstein condensate (BEC) regimes can be identified in any band insulator above two dimensions, while in two dimensions only the BEC regime exists. The superconducting transition is ``unconventional'' (non-pair-breaking) in the BEC regime, identified by either the bosonic mean field or XY\mathit{XY}XY universality class. The insulator adjacent to the superconductor in the BEC regime is a bosonic Mott insulator of Cooper pairs, which may be susceptible to charge density wave ordering. We construct a function of the many-body excitation spectrum whose nonanalytic changes define a sharp distinction between band and Mott insulators. The corresponding ``second-order transition'' can be observed out of equilibrium by driving a Cooper pair laser in the Mott insulator. We explicitly show that the gap for charged bosonic excitations lies below the threshold for Cooper pair breakup in any BEC regime, despite quantum fluctuations. Our discussion ends with a view of possible consequences for cuprates, where antinodal pair dynamics has certain features in common with our simple sss-wave picture.
Despite the intense theoretical and experimental effort, an understanding of the superconducting pairing mechanism of the high-temperature superconductors leading to an unprecedented high transition temperature Tc{T}_{c}Tc​ is still lacking. An additional puzzle is the unknown connection between the superconducting gap and the so-called pseudogap which is a central property of the most unusual normal state. Angle-resolved photoemission spectroscopy (ARPES) measurements have revealed a gaplike behavior on parts of the Fermi surface, leaving a nongapped segment known as Fermi arc around the diagonal of the Brillouin zone. Two main interpretations of the origin of the pseudogap have been proposed: either the pseudogap is a precursor to superconductivity, or it arises from another order competing with superconductivity. Starting from the t-J model, in this paper we present a microscopic approach to investigate physical properties of the pseudogap phase as well as the superconducting phase in the framework of a renormalization scheme called projector-based renormalization method. This approach is based on a stepwise elimination of high-energy transitions using unitary transformations. We arrive at renormalized ``free'' Hamiltonians for correlated electrons for both phases. Our microscopic approach allows us to explain the experimental findings in the underdoped as well as in the optimal hole doping regime. The ARPES spectral function along the Fermi surface turns out to be in good agreement with experiment: For the pseudogap phase we find well-defined excitation peaks around $\ensuremath{\omega}=0$ near the nodal direction, which become strongly suppressed around the antinodal point. The origin of the pseudogap can be traced back to a suppression of spectral weight from incoherent excitations in a small $\ensuremath{\omega}$ range around the Fermi energy. In the superconducting phase, the order parameter turns out to have ddd-wave symmetry with a coherence length of a few lattice constants. In good agreement with experiments, we find no superconducting solutions for very small hole doping.
There are two seemingly unrelated puzzles about the cuprate superconductors. The first puzzle concerns the strong non-BCS behavior around xc{x}_{c}xc​, the end point of the superconducting dome on the overdoped side, where the cuprate is believed to be well described by the Fermi-liquid theory. This is the most evident in the observed ${\ensuremath{\rho}}_{s}(0)\ensuremath{-}{T}_{c}$ scaling and the large amount of uncondensed optical spectral weight at low energy. The second puzzle concerns the remarkable robustness of the ddd-wave pairing against the inevitable disorder effect in such a doped system, which is also totally unexpected from the conventional BCS picture. Here we show that these two puzzles are deeply connected to the origin of a third puzzle about the cuprate superconductors, namely, the mysterious quantum critical behavior observed around x∗{x}^{*}x∗, the so called pseudogap end point. Through a systematic variational Monte Carlo (VMC) study of the disordered 2D $t\ensuremath{-}J$ model from the resonating valence bond (RVB) perspective, we find that the ddd-wave pairing in this model is remarkably more robust against the disorder effect than that in a conventional ddd-wave BCS superconductor. We find that such remarkable robustness can be attributed to the spin-charge separation mechanism in the RVB picture, through which the ddd-wave RVB pairing of the charge-neutral spinons becomes essentially immune to the disorder potential except for the secondary effect related to the modulation of the local doping level by the disorder. We propose that there exists a Mott transition at x∗{x}^{*}x∗, where the RVB pairing in the underdoped regime is transmuted into the increasingly more BCS-like pairing for x>x∗x>{x}^{*}x>x∗, whose increasing fragility against the disorder effect leads to the non-BCS behavior and the ultimate suppression of superconductivity around xc{x}_{c}xc​.
Despite the intense theoretical and experimental effort, an understanding of the superconducting pairing mechanism of the high-temperature superconductors is still lacking. An additional puzzle is the unknown connection between the superconducting gap and the so-called pseudogap which is a central property of the most unusual normal state. Angle-resolved photoemission spectroscopy (ARPES) measurements have revealed a gap-like behavior on parts of the Fermi surface, leaving a non-gapped segment known as Fermi arc around the diagonal of the Brillouin zone. Starting from the ttt-JJJ model, in this paper we present a microscopic approach to investigate physical properties of the pseudogap phase in the framework of a novel renormalization scheme called PRM. This approach is based on a stepwise elimination of high-energy transitions using unitary transformations. We arrive at a renormalized 'free' Hamiltonian for correlated electrons. The ARPES spectral function along the Fermi surface turns out to be in good agreement with experiment: We find well-defined excitation peaks around ω=0ω=0ω=0 near the nodal direction, which become strongly suppressed around the antinodal point. The origin of the pseudogap can be traced back to a suppression of spectral weight from incoherent excitations in a small ωωω-range around the Fermi energy. In a subsequent paper, also the supercunducting phase at moderate hole doping will be discussed within the PRM approach.
The phase diagram of hole-doped high-temperature superconductors remains puzzling. A state of matter with unusual physical properties, dubbed pseudogap, is found below a characteristic temperature T∗T^*T∗ in a doped Mott insulator. Since the superconducting state is born out of the pseudogap over much of the phase diagram, the nature of the pseudogap is a fundamental issue in the field and it is under intense theoretical and experimental scrutiny. In many cases, it is not even clear whether T∗T^*T∗ is a crossover or a phase transition. Here we show, by constructing the normal-state phase diagram of the archetypal model of strongly correlated electron systems, that T∗T^*T∗ is a crossover line above a critical endpoint, while below that point it is a first-order phase transition between two metallic phases, one with a pseudogap and one without. Thus T∗T^*T∗ appears in a new light: it is an unexpected example of a phenomenon observed in fluids, namely a sharp crossover between different dynamical regimes along a line of thermodynamic anomalies that appears above a first-order phase transition, the Widom line. Our findings thus suggest that the critical point of a first-order transition can be the organizing principle for the rich behavior of the normal state of the cuprates.
The origin of the pseudogap behavior, found in many high-TcT_cTc​ superconductors, remains one of the greatest puzzles in condensed matter physics. One possible mechanism is fermionic incoherence, which near a quantum critical point allows pair formation but suppresses superconductivity. Employing quantum Monte Carlo simulations of a model of itinerant fermions coupled to ferromagnetic spin fluctuations, represented by a quantum rotor, we report numerical evidence of pseudogap behavior, emerging from pairing fluctuations in a quantum-critical non-Fermi liquid. Specifically, we observe enhanced pairing fluctuations and a partial gap opening in the fermionic spectrum. However, the system remains non-superconducting until reaching a much lower temperature. In the pseudogap regime the system displays a gap-filling rather than gap-closing behavior, consistent with experimental observations. Our results provide the first unambiguous lattice model realization of a pseudogap state in a strongly correlated system, driven by superconducting fluctuations.