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arXiv:1310.5453 · Physical Review A

Natural correlation between a system and a thermal reservoir

Takashi Mori

Published Apr 2, 2014• 4 citations
arXivHTMLPDF

Abstract

Non-Markovian corrections to the Markovian quantum master equation of an open quantum system are investigated up to the second order of the interaction between the system of interest and a thermal reservoir. The concept of ``natural correlation'' is discussed. When the system is naturally correlated with a thermal reservoir, the time evolution of the reduced density matrix looks Markovian even in a short-time regime. If the total system was initially in an ``unnatural'' state, the natural correlation is established during the time evolution, and after that the time evolution becomes Markovian in a long-time regime. It is also shown that for a certain set of reduced density matrices, the naturally correlated state does not exist. If the initial reduced density matrix has no naturally correlated state, the time evolution is inevitably non-Markovian in a short-time regime.

DOI
10.1103/physreva.89.040101

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Europhysics Letters (EPL)•Jun 1, 2013•14 citations
Non-Markovian corrections to the Markovian quantum master equation of an open quantum system are investigated up to the second order of the interaction between the system of interest and a thermal reservoir. The concept of natural correlation'' is discussed. When the system is naturally correlated with a thermal reservoir, the time evolution of the reduced density matrix looks Markovian even in a short-time regime. If the total system was initially in an unnatural'' state, the natural correlation is established during the time evolution, and after that the time evolution becomes Markovian in a long-time regime. It is also shown that for a certain set of reduced density matrices, the naturally correlated state does not exist. If the initial reduced density matrix has no naturally correlated state, the time evolution is inevitably non-Markovian in a short-time regime.
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Beyond the conventional quantum regression theorem, a general formula for non-Markovian correlation functions of arbitrary system operators both in the time- and frequency-domain is given. Weapproach the problem by transforming the conventional time-non-local master equation into dispersed time-local equations-of-motion. The validity of our approximations is discussed and we find that the non-Markovian terms have to be included for short times. While calculations of the density matrix at short times suffer from the initial value problem, a correlation function has a well defined initial state. The resulting formula for the non-Markovian correlation function has a simple structure and is as convenient in its application as the conventional quantum regression theorem for the Markovian case. For illustrations, we apply our method to investigate the spectrum of the current fluctuations of interacting quantum dots contacted with two electrodes. The corresponding non- Markovian characteristics are demonstrated.
We study the role of correlations with the environment as the source of non-Markovian quantum evolutions. We first focus on the impact that correlations with the environment can have on the dynamical map that evolve the system. We expand the set of initial states of a system and its environment that are known to guarantee completely positive reduced dynamics for the system when the combined state evolves unitarily. We characterize the correlations in the initial state in terms of its quantum discord. The induced maps can be not completely positive when quantum correlations including, but not limited to, entanglement are present. We discuss the implications and limitations of the Markov approximation necessary to derive the Kossakowski-Lindblad master equation. A generalized non-Markovian master equation is derived from the dynamical map of systems correlated with their environment. The physical meaning of not completely positive maps is studied to obtain a consistent theory of non-Markovian quantum dynamics. These are associated to inverse maps necessary to establish correlations and they give rise to a canonical embedding map that is local in time. This master equation goes beyond the Kossakowski-Lindblad master equation. Non-equilibrium quantum thermodynamics can be be studied within this theory. Through out this discussion, the general dynamics of two interacting qubits is used as an example for illustrations.
We study the non-Markovian dynamics of a two-mode bosonic system interacting with two uncorrelated thermal bosonic reservoirs. We present the solution to the exact microscopic Master equation in terms of the quantum characteristic function and study in detail the dynamics of entanglement for bipartite Gaussian states. In particular, we analyze the effects of short-time system-reservoir correlations on the separability thresholds and show that the relevant parameter is the reservoir spectral density. If the frequencies of the involved modes are within the reservoir spectral density, entanglement persists for a longer time than in a Markovian channel. On the other hand, when the reservoir spectrum is out of resonance, short-time correlations lead to a faster decoherence and to the appearance of entanglement oscillations.
In this work we investigate the late-time steady states of open quantum systems coupled to a thermal reservoir in the strong coupling regime. In general such systems do not necessarily relax to a Boltzmann distribution if the coupling to the thermal reservoir is nonvanishing or equivalently if the relaxation time scales are finite. Using a variety of nonequilibrium formalisms valid for non-Markovian processes, we show that starting from a product state of the closed system = system+environment, with the environment in its thermal state, the open system which results from coarse graining the environment will evolve towards an equilibrium state at late times. This state can be expressed as the reduced state of the closed system thermal state at the temperature of the environment. For a linear (harmonic) system and environment, which is exactly solvable, we are able to show in a rigorous way that all multitime correlations of the open system evolve towards those of the closed system thermal state. Multitime correlations are especially relevant in the non-Markovian regime, since they cannot be generated by the dynamics of the single-time correlations. For more general systems, which cannot be exactly solved, we are able to provide a general proof that all single-time correlations of the open system evolve to those of the closed system thermal state, to first order in the relaxation rates. For the special case of a zero-temperature reservoir, we are able to explicitly construct the reduced closed system thermal state in terms of the environmental correlations.
Starting from unitary dynamics we study the evolution in time of a non-relativistic quantum system that exchanges energy with a thermal reservoir of harmonic oscillators. System and reservoir are assumed to be initially decorrelated. Reservoir correlation functions are factorized by means of a Kraus compliant version of Wick's theorem. As a result, the non-Markovian Kraus map for the system density operator can be completely expressed in terms of system potentials and reservoir pair correlation functions. An infinite hierarchy for the evolution operators of the Kraus map is derived. The system density operator is obtained as a time-ordered exponential containing a non-Markovian counterpart of the standard Markovian generator for dissipative dynamics. We specify a condition on this non-Markovian generator for return to thermal equilibrium. We set up a non-Markovian perturbation theory that preserves both trace and positivity of the system density operator.