Abstract We report on measurements of the lifetime of the state in single ions confined in a radiofrequency quadrupole trap. Experimental parameters that affect hyperfine state preparation and detection efficiency are characterized and optimized. A set of wait times for optimal sampling of the lifetime is chosen and used to measure that lifetime with high statistical sensitivity. A systematic variation in this lifetime seems to be apparent. The source of the variation was not identified, but ion number and cooling rate appear to be ruled out. A net determination is made of ms which is significantly longer than other measurements of the same quantity with four times better statistical precision than the most recent measurement. An alternate shelving scheme is proposed that would provide S – D state discrimination for Yb + even isotopes as well as improved sensitivity for D state hyperfine discrimination in odd isotopes.
A generalized probe sequence typical of trapped ion experiments using shelving is studied. Detection efficiency is analyzed for finite shelved state lifetimes and using multi-modal count distributions. Multi-modal distributions are more appropriate for measurements that use a small number of ions than the simple Poisson counting statistics usually considered and have a larger variance that may be significant in determining uncertainties and in making weighted fits. Optimal probe times and the resulting state detection efficiency and sensitivity are determined for arbitrary cooling rates, initial states and shelved state lifetimes, in terms of a probe coherence time τp. A universal optimal probe time of tp ~ 0.43τp is shown to give an almost optimal probe sensitivity for most systems.
Compared to other stable isotopes of
Yb+,
173Yb+ has a richer hyperfine structure, which leads to more favorable clock transitions, spectroscopic techniques for probing new physics, and more sophisticated quantum computing architectures. However, to date, its electronic spectrum remains poorly characterized. Here, we report on efficient laser cooling, state preparation, and detection of a single trapped
173Yb+ ion. The previously unobserved
2S1/2→2D3/2 electric quadrupole transition at 436 nm is coherently excited, and the isotope shift between
171Yb+ and
173Yb+ on this transition is determined with an uncertainty of 1.4 Hz. Using microwave spectroscopy, we resolve the hyperfine structure (HFS) of the
2D3/2 state with a relative uncertainty below
10−8. From the HFS measurement data, we infer for
173Yb a nuclear magnetic octupole moment
Ω=−0.062(8)(b×μN) with uncertainty reduced by more than 2 orders of magnitude compared to previous studies. The data also allow us to determine hyperfine anomalies for the
2S1/2 and
2D3/2 states.
A generalized probe sequence typical of trapped ion experiments using shelving is studied. Detection efficiency is analyzed for finite shelved state lifetimes and using multi-modal count distributions. Multi-modal distributions are more appropriate for measurements that use a small number of ions than the simple Poisson counting statistics usually considered and have a larger variance that may be significant in determining uncertainties and in making weighted fits. Optimal probe times and the resulting state detection efficiency and sensitivity are determined for arbitrary cooling rates, initial states and shelved state lifetimes, in terms of a probe coherence time τp. A universal optimal probe time of tp ~ 0.43τp is shown to give an almost optimal probe sensitivity for most systems.
We present a method to precisely determine the
2D3/2 state lifetime of a single trapped
174Yb+ ion. This method is based on the detection of photons emitted from excited states, where a highly synchronized measurement sequence for laser control and an intensity-alternating sequence for atomic excitation and photon counting are used to minimize systematic errors. This method is easy to implement and is immune to fluctuations of magnetic field, laser intensity, and frequency detuning. Combined with the real-time approach of background photon correction, the radiative lifetime of the
2D3/2 state is determined to be $54.83\ifmmode\pm\else\textpm\fi{}0.18$ ms, which represents an order of magnitude improvement in measurement precision. The accurately determined lifetime sets a benchmark for many-body atomic theories and is particularly useful to determine the coherence time limit of the optical clock.
Qubits encoded in hyperfine states of trapped ions are ideal for quantum computation given their long lifetimes and low sensitivity to magnetic fields, yet they suffer from off-resonant scattering during detection, often limiting their measurement fidelity. In
171Yb+ this is exacerbated by a low fluorescence yield, which leads to a need for complex and expensive hardware, a problematic bottleneck especially when scaling up the number of qubits. We demonstrate a detection routine based on electron shelving to address this issue in
171Yb+ and achieve a $5.6\ifmmode\times\else\texttimes\fi{}$ reduction in single-ion detection error on an avalanche photodiode to $1.8(2)\ifmmode\times\else\texttimes\fi{}{10}^{\ensuremath{-}3}$ in a 100 $\ensuremath{\mu}\mathrm{s}$ detection period and a $4.3\ifmmode\times\else\texttimes\fi{}$ error reduction on an electron multiplying CCD camera with $7.7(2)\ifmmode\times\else\texttimes\fi{}{10}^{\ensuremath{-}3}$ error in 400 $\ensuremath{\mu}\mathrm{s}$. We further improve the characterization of a repump transition at 760 nm to enable a more rapid reset of the auxiliary
2F7/2 states populated after shelving. Finally, we examine the detection fidelity limit using the long-lived
2F7/2 state, achieving further $300\ifmmode\times\else\texttimes\fi{}$ and $12\ifmmode\times\else\texttimes\fi{}$ reductions in error to $6(7)\ifmmode\times\else\texttimes\fi{}{10}^{\ensuremath{-}6}$ and $6.3(3)\ifmmode\times\else\texttimes\fi{}{10}^{\ensuremath{-}4}$ in 1 ms on the respective detectors. While shelving-rate limited in our setup, we suggest various techniques to realize this detection method at speeds compatible with quantum information processing, providing a pathway to ultrahigh-fidelity detection in
171Yb+.