The interaction of a cavity with an external field is symmetric under time reversal. Thus, coupling to a resonator is most efficient when the incident light is the time reversed version of a free cavity decay, i.e. when it has a rising exponential shape matching the cavity lifetime. For light entering the cavity from only one side, the maximally achievable coupling efficiency is limited by the choice of the cavity mirrors' reflectivities. Such an empty-cavity experiment serves also as a model system for single-photon single-atom absorption dynamics. We present experiments coupling exponentially rising pulses to a cavity system which allows for high coupling efficiencies. The influence of the time constant of the rising exponential is investigated as well as the effect of a finite pulse duration. We demonstrate coupling 94% of the incident TEM 00 mode into the resonator.
The interaction of a cavity with an external field is symmetric under time reversal. Thus, coupling to a resonator is most efficient when the incident light is the time reversed version of a free cavity decay, i.e. when it has a rising exponential shape matching the cavity lifetime. For light entering the cavity from only one side, the maximally achievable coupling efficiency is limited by the choice of the cavity mirrors' reflectivities. Such an empty-cavity experiment serves also as a model system for single-photon single-atom absorption dynamics. We present experiments coupling exponentially rising pulses to a cavity system which allows for high coupling efficiencies. The influence of the time constant of the rising exponential is investigated as well as the effect of a finite pulse duration. We demonstrate coupling 94% of the incident TEM 00 mode into the resonator.
The absorption of a single photon by a single two-level system (TLS) in free space is a fundamental physical process. In this contribution, we present the experimental realization of a model system to simulate the dynamics of such an absorption experiment: Comparing the absorption process of a single photon by a single TLS and the incoupling dynamics of an optical resonator, one finds an analogy between the energy stored inside the resonator and the probability of the photon to be absorbed by the TLS [1]. Both systems, resonators and TLS, respond in an equivalent way to the temporal profile of the incident light pulse. The energy storage in a resonator as well as the absorption of a single photon by a TLS can reach an unit efficiency under idealized conditions. Such an optimized process is achieved by an exponentially rising incident light field with a time constant which matches the lifetime of the system [2]. For such a perfect coupling, the end mirror of the resonator needs to have a reflectivity of unity. This corresponds to the excitation of a TLS from the complete solid angle. For a smaller reflectivity of the end mirror, the cavity simulates the absorption dynamics in the case of excitation from only a part of the solid angle. However, using real mirrors, a good analogy with excitation from a large solid angle can still be obtained by using a strongly asymmetric resonator, i.e. an incoupling mirror which has a significantly lower reflectivity than the end mirror of the cavity.
A single atom in free space can have a strong influence on a light beam and a single photon can have a strong effect on a single atom in free space. Regarding this interaction, two conceptually different questions can be asked: can a single atom fully absorb a single photon and can a single atom fully reflect a light beam. The conditions for achieving the full effect in either case are different. Here we discuss related questions in the context of an optical resonator. When shaping a laser pulse properly it will be fully absorbed by an optical resonator, i.e., no light will be reflected and all the pulse energy will accumulate inside the resonator before it starts leaking out. We show in detail that in this case the temporal pulse shape has to match the time-reversed pulse obtained by the cavity's free decay. On the other hand a resonator, made of highly reflecting mirrors which normally reflect a large portion of any incident light, may fully transmit the light, as long as the light is narrow band and resonant with the cavity. The analogy is the single atom-normally letting most of the light pass-which under special conditions may fully reflect the incident light beam. Using this analogy we are able to study the effects of practical experimental limitations in the atom-photon coupling, such as finite pulses, bandwidths, and solid angle coverage, and to use the optical resonator as a test bed for the implementation of the quantum experiment.
This thesis describes an experiment to optimize the interaction of light and a single ion in free space. The key to efficient coupling consists in mode-matching the incident electromagnetic field to the radiative properties of the ion. For perfect coupling, the incident mode has to match the emission pattern of the ion. In free space, this requires illumination of the ion with an incoming dipole wave. In the present work, such a situation is realized experimentally. To this end, a radially polarized doughnut mode is focused with a deep parabolic mirror while the ion is localized in the focal point of the parabolic mirror by means of a trap of special geometry. This thesis reports first on the implementation of the two basic components of the experiment: the ion trapping in the focal point of the parabolic mirror and the generation of the required doughnut mode. Then, the coupling efficiency of the combined system is analyzed by means of saturation measurements. Characterization of our setup reveals aberrations of the parabolic mirror which prevent perfect coupling. However, the measured coupling efficiency of (7.2 ± 0.2)% is to date among the highest values reported for coupling experiments with a single atom in free space. A special aim of our group is the full excitation of an ion by a single photon. This requires, in addition to the above mentioned spatial mode matching, temporal shaping of the incident light. Perfect excitation can be achieved if the single-photon wavepacket shows an exponentially rising envelope with a time constant matching the lifetime of the excited state of the ion. The present work demonstrates the power of temporal mode matching using a model system: an empty optical cavity. Both, light inside a cavity and atomic excitation, decay exponentially. Thus, there is an analogy between atomic excitation and field energy inside a cavity. The task of exciting an ion translates to the task of coupling a classical light pulse into a cavity. This thesis confirms experimentally that almost the entire energy of a rising exponential pulse can be coupled into a cavity, provided the pulse time constant matches the cavity lifetime.
A single atom in free space can have a strong influence on a light beam and a single photon can have a strong effect on a single atom in free space. Regarding this interaction, two conceptually different questions can be asked: can a single atom fully absorb a single photon and can a single atom fully reflect a light beam. The conditions for achieving the full effect in either case are different. Here we discuss related questions in the context of an optical resonator. When shaping a laser pulse properly it will be fully absorbed by an optical resonator, i.e., no light will be reflected and all the pulse energy will accumulate inside the resonator before it starts leaking out. We show in detail that in this case the temporal pulse shape has to match the time-reversed pulse obtained by the cavity’s free decay. On the other hand a resonator, made of highly reflecting mirrors which normally reflect a large portion of any incident light, may fully transmit the light, as long as the light is narrow band and resonant with the cavity. The analogy is the single atom—normally letting most of the light pass—which under special conditions may fully reflect the incident light beam. Using this analogy we are able to study the effects of practical experimental limitations in the atom-photon coupling, such as finite pulses, bandwidths, and solid angle coverage, and to use the optical resonator as a test bed for the implementation of the quantum experiment.
We describe a method to couple a light pulse into a cavity with arbitrarily high finesse, with an efficiency that in theory can approach 100% even if the pulse duration is much longer than the round-trip time of the cavity. The spectrum of the pulse is compressed into a single narrow mode in an adiabatic and reversible way. The method uses an input coupler with a variable effective reflectivity which is adapted to match the known temporal shape of the pulse. In addition to a theoretical description of the method, we demonstrate the principle experimentally.
We demonstrate that a single photon with an optimal temporal waveform can be efficiently loaded into a cavity. Using heralded narrow-band single photons with exponential growth wave packet shaped by an electro-optical amplitude modulator, whose time constant matches the photon lifetime in the cavity, we demonstrate a loading efficiency of (87±2)% from free space to a single-sided Fabry-Perot cavity. We further demonstrate directly loading heralded single Stokes photons into the cavity with an efficiency of (60±5)% without the electro-optical amplitude modulator and verify the time reversal between the frequency-entangled paired photons. Our result and approach may enable promising applications in realizing large-scale quantum networks based on cavity quantum electrodynamics.