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arXiv:1308.3049 · Europhysics Letters (EPL)

Reentrant classicality of a damped system

Benjamin Spreng, Gert‐Ludwig Ingold, Ulrich Weiss

Published Sep 1, 2013• 9 citations
arXivHTMLPDF

Abstract

For a free particle, the coupling to its environment can be the relevant mechanism to induce quantum behavior as the temperature is lowered. We study general linear environments with a spectral density proportional to ω^s at low frequencies and consider in particular the specific heat of the free damped particle. For super-Ohmic baths with s>=2, a reentrant classical behavior is found. As the temperature is lowered, the specific heat decreases from the classical value of k_B/2, thereby indicating the appearence of quantum effects. However, the classical value of the specific heat is restored as the temperature approaches zero. This surprising behavior is due to the suppressed density of bath degrees of freedom at low frequencies. For s<2, the specific heat at zero temperature increases linearly with s from -k_B/2 to k_B/2. An Ohmic bath, s=1, is thus very special in the sense that it represents the only case where the specific heat vanishes at zero temperature.

DOI
10.1209/0295-5075/103/60007

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For a free particle, the coupling to its environment can be the relevant mechanism to induce quantum behavior as the temperature is lowered. We study general linear environments with a spectral density proportional to ω^s at low frequencies and consider in particular the specific heat of the free damped particle. For super-Ohmic baths with s>=2, a reentrant classical behavior is found. As the temperature is lowered, the specific heat decreases from the classical value of k_B/2, thereby indicating the appearence of quantum effects. However, the classical value of the specific heat is restored as the temperature approaches zero. This surprising behavior is due to the suppressed density of bath degrees of freedom at low frequencies. For s<2, the specific heat at zero temperature increases linearly with s from -k_B/2 to k_B/2. An Ohmic bath, s=1, is thus very special in the sense that it represents the only case where the specific heat vanishes at zero temperature.
The quantum thermodynamic behavior of small systems is investigated in presence of finite quantum dissipation. We consider the archetype cases of a damped harmonic oscillator and a free quantum Brownian particle. A main finding is that quantum dissipation helps to ensure the validity of the Third Law. For the quantum oscillator, finite damping replaces the zero-coupling result of an exponential suppression of the specific heat at low temperatures by a power-law behavior. Rather intriguing is the behavior of the free quantum Brownian particle. In this case, quantum dissipation is able to restore the Third Law: Instead of being constant down to zero temperature, the specific heat now vanishes proportional to temperature with an amplitude that is inversely proportional to the ohmic dissipation strength. A distinct subtlety of finite quantum dissipation is the result that the various thermodynamic functions of the sub-system do not only depend on the dissipation strength but depend as well on the prescription employed in their definition.
The quantum thermodynamic behavior of small systems is investigated in presence of finite quantum dissipation. We consider the archetype cases of a damped harmonic oscillator and a free quantum Brownian particle. A main finding is that quantum dissipation helps to ensure the validity of the Third Law. For the quantum oscillator, finite damping replaces the zero-coupling result of an exponential suppression of the specific heat at low temperatures by a power-law behavior. Rather intriguing is the behavior of the free quantum Brownian particle. In this case, quantum dissipation is able to restore the Third Law: Instead of being constant down to zero temperature, the specific heat now vanishes proportional to temperature with an amplitude that is inversely proportional to the ohmic dissipation strength. A distinct subtlety of finite quantum dissipation is the result that the various thermodynamic functions of the sub-system do not only depend on the dissipation strength but depend as well on the prescription employed in their definition.
We consider a free particle coupled with finite strength to a bath and investigate the evaluation of its specific heat. A harmonic oscillator bath of Drude type with cutoff frequency ω D is employed to model an ohmic friction force with dissipation strength γ. Two scenarios for obtaining specific heat are presented. The first one uses the measurement of the kinetic energy of the free particle, while the second one is based on the reduced partition function. Both descriptions yield results which are consistent with the Third Law of thermodynamics. Nevertheless, the two methods produce different results that disagree even in their leading quantum corrections at high temperatures. We also consider the regime where the cutoff frequency is smaller than the friction strength, i.e. ω D < γ. There, we encounter puzzling results at low temperatures where the specific heat based on the thermodynamic prescription becomes negative. This anomaly is rooted in an ill-defined density of states of the damped free particle, which assumes unphysical negative values when γ/ω D > 1.
The evaluation of the specific heat of an open damped quantum system is a subtle issue. One possible route is based on the thermodynamic partition function which is the ratio of the partition functions of system plus bath and of the bath alone. For the free damped particle it has been shown, however, that the ensuing specific heat may become negative for appropriately chosen environments. Being an open system this quantity then naturally must be interpreted as the change in the specific heat obtained as the difference between the specific heat of the heat bath coupled to the system degrees of freedom and the specific heat of the bath alone. While this difference may become negative, the involved specific heats themselves are always positive; thus, the known thermodynamic stability criteria are perfectly guaranteed. For a damped quantum harmonic oscillator, instead of negative values, under appropriate conditions one can observe a dip in the difference of specific heats as a function of temperature. Stylized minimal models containing a single oscillator heat bath are employed to elucidate the occurrence of the anomalous temperature dependence of the corresponding specific heat values. Moreover, we comment on the consequences for the interpretation of the density of states based on the thermal partition function.
The definition of the specific heat for a damped quantum system is a subtle issue. A possible approach is based on an effective partition function defined as the ratio of the partition functions of system plus bath and of the bath alone. For the free damped particle it has been shown, however, that the ensuing specific heat may become negative for appropriately chosen environments. We argue that this quantity should be interpreted as the change of the specific heat of the heat bath when the system degrees of freedom are coupled to it. While this difference may become negative, the involved specific heats themselves are always positive and therefore thermodynamic stability is always guaranteed. For a damped harmonic oscillator, instead of negative values, under appropriate conditions one can observe a dip in the difference of specific heats as a function of temperature. Minimal models containing a single oscillator heat bath are employed to elucidate the temperature dependence of the difference of specific heats. Finally, we comment on the consequences for the interpretation of the density of states based on the effective partition function.
In this Letter it is shown that exact decoherence to minimal uncertainty Gaussian pointer states is generic for free quantum particles coupled to a heat bath. More specifically, the Letter is concerned with damped free particles linearly coupled under product initial conditions to a heat bath at arbitrary temperature, with arbitrary coupling strength and spectral densities covering the Ohmic, sub-Ohmic, and supra-Ohmic regime. Then it is true that there exists a time t(c) such that for times t>t(c) the state can always be exactly represented as a mixture (convex combination) of particular minimal uncertainty Gaussian states, regardless of and independent from the initial state. This exact "localization" is hence not a feature specific to high temperature and weak damping limit, but is a generic property of damped free particles.