The dynamics of an atom-molecule-conversion system subject to dephasing noises is studied in this paper. Using a dephasing master equation and mean-field theory, we derive a Bloch equation for the system, and this equation is compared with the Bloch equation derived by the Bogoliubov-Born-Green-Kirkwood-Yvon (BBGKY) hierarchy truncation approach. Fixed points of the system are calculated by solving both the Bloch equation and the master equation. Comparison between these two calculations suggests that while at short times the mean-field theory (MFT) is a good approximation for the atom-molecule-conversion system, a high-order hierarchy truncation approach is necessary for the system on a long time scale. Although the MFT cannot predict the fixed points correctly, its predictions for the stability of the fixed points are consistent with the BBGKY theory for a wide range of parameters.
The dynamics of an atom-molecule-conversion system subject to dephasing noises is studied in this paper. Using a dephasing master equation and mean-field theory, we derive a Bloch equation for the system, and this equation is compared with the Bloch equation derived by the Bogoliubov-Born-Green-Kirkwood-Yvon (BBGKY) hierarchy truncation approach. Fixed points of the system are calculated by solving both the Bloch equation and the master equation. Comparison between these two calculations suggests that while at short times the mean-field theory (MFT) is a good approximation for the atom-molecule-conversion system, a high-order hierarchy truncation approach is necessary for the system on a long time scale. Although the MFT cannot predict the fixed points correctly, its predictions for the stability of the fixed points are consistent with the BBGKY theory for a wide range of parameters.
Based on the mean-field approximation and the phase-space analysis, we study the dynamics of atom-molecule conversion systems subject to particle losses. Starting from the many-body dynamics described by a master equation, an effective nonlinear Schr\"odinger equation is introduced. The classical phase space is then specified and classified by fixed points. The boundaries, which separate different dynamical regimes, have been established and discussed. The effect of particle loss on the conversion efficiency and the self-trapping is explored. By numerically solving the master equation, we show that the mean-field approximation is a good approach to study the dynamics of this atom-molecule conversion system.
We establish a theoretical framework for the exploration of the quantum dynamics of finite ultracold bosonic ensembles based on the Born-Bogoliubov-Green-Kirkwood-Yvon (BBGKY) hierarchy for equations of motion for few-particle reduced density matrices (RDMs). The theory applies to zero as well as low temperatures and is formulated in a highly efficient way by utilizing dynamically optimized single-particle basis states and representing the RDMs in terms of permanents with respect to those. An energy, RDM compatibility and, if applicable, symmetry conserving closure approximation is developed on the basis of a cluster expansion for these finite systems, using suitably normalized RDMs and symmetrization operators. The underlying cluster expansion is formulated recursively by means of super-operators, which allows for going to large truncation orders. In order to enforce necessary representability conditions, two novel, minimal-invasive and energy-conserving correction algorithms are proposed, involving the dynamical purification of the solution of the truncated BBGKY hierarchy and the correction of the equations of motion themselves, respectively. For gaining conceptual insights, the impact of two-particle correlations on the dynamical quantum depletion is studied analytically. The theoretical framework provided here is extensively applied and evaluated in our immediate follow-up work [1], involving truncation orders as large as twelve.
Abstract Based on the mean-field approximation and the two-mode Bose–Hubbard model, we investigate the dynamical properties of atom-polyatomic molecule conversion systems under dissipation and dephasing. For such a many-body system problem, we partition phase space based on the states of fixed points, study the movement of fixed points and the transition to attractors in an open system. Additionally, for all the atoms that constitute a molecule, depending on whether the species of these atoms are identical or not, we introduce the innovative concepts of unbiased and biased systems. We discover that in biased conversion systems under particle losses, the evolution trajectories are distributed on a three-dimensional Bloch sphere with an internal structure. There exists a significant difference from the two-dimensional Hilbert space of an unbiased system. Finally, we discuss the sweeping rate of the time-varying magnetic field applied externally to the conversion system, and analyze a feasible scheme for the quantum coherent synthesis of triatomic molecules.
We establish a theoretical framework for exploring the quantum dynamics of finite ultracold bosonic ensembles based on the Born-Bogoliubov-Green-Kirkwood-Yvon (BBGKY) hierarchy of equations of motion for few-particle reduced density matrices (RDMs). The theory applies to zero as well as low temperatures and is formulated in a highly efficient way by utilizing dynamically optimized single-particle basis states and representing the RDMs in terms of permanents with respect to those. An energy, RDM compatibility and symmetry conserving closure approximation is developed on the basis of a recursively formulated cluster expansion for these finite systems. In order to enforce necessary representability conditions, two novel, minimal-invasive and energy-conserving correction algorithms are proposed, involving the dynamical purification of the solution of the truncated BBGKY hierarchy and the correction of the equations of motion themselves, respectively. For gaining conceptual insights, the impact of two-particle correlations on the dynamical quantum depletion is studied analytically. We apply this theoretical framework to both a tunneling and an interaction-quench scenario. Due to our efficient formulation of the theory, we can reach truncation orders as large as twelve and thereby systematically study the impact of the truncation order on the results. While the short-time dynamics is found to be excellently described with controllable accuracy, significant deviations occur on a longer time-scale in sufficiently far off-equilibrium situations. Theses deviations are accompanied by exponential-like instabilities leading to unphysical results. The phenomenology of these instabilities is investigated in detail and we show that the minimal-invasive correction algorithm of the equation of motion can indeed stabilize the BBGKY hierarchy truncated at the second order.
A set of nonlinear evolution equations describing the dynamics of atoms, molecules, and photons in the course of stimulated atomic-molecular conversion in a Bose-Einstein condensate is derived and studied in the mean-field approximation. It is shown that conversion can be periodic or aperiodic in time, the rate of the process being determined to a considerable extent by the initial density of particles and by the initial phase difference. Depending on the initial conditions, various conversion modes can be realized. The possibility of stabilization of a special state (of rest) of the system for nonzero initial number densities of particles is predicted. It is pointed out that coherence of a Bose condensate of atoms, molecules, and photons predetermines the possibility of phase control of the conversion process.
A set of nonlinear evolution equations describing the dynamics of atoms, molecules, and photons in the course of stimulated atomic-molecular conversion in a Bose-Einstein condensate is derived and studied in the mean-field approximation. It is shown that conversion can be periodic or aperiodic in time, the rate of the process being determined, to a considerable extent, by the initial density of particles and by the initial phase difference. Depending on initial conditions, various conversion modes can be realized. The possibility of stabilization of a special state (of rest) of the system for nonzero initial number densities of particles is predicted. It is pointed out that coherence of a Bose condensate of atoms, molecules, and photons predetermines the possibility of phase control of the conversion process.