We present an extensive quantum Monte Carlo study of the Néel to valence-bond solid (VBS) phase transition on rectangular- and honeycomb-lattice SU(N) antiferromagnets in sign-problem-free models. We find that in contrast to the honeycomb lattice and previously studied square-lattice systems, on the rectangular lattice for small N, a first-order Néel-VBS transition is realized. On increasing N≥4, we observe that the transition becomes continuous and with the same universal exponents as found on the honeycomb and square lattices (studied here for N=5, 7, 10), providing strong support for a deconfined quantum critical point. Combining our new results with previous numerical and analytical studies, we present a general phase diagram of the stability of CPN-1 fixed points with q monopoles.
I will give an overview of unbiased numerical work on the Neelvalence bond solid (VBS) phase transition in d = 2 antiferromagnets. This progress has been possible due to the discovery of a new class of Hamiltonians of SU(N) spins that are free of the sign problem of quantum Monte Carlo. I will show through extensive numerical studies of the quantum phase transition on a variety of bipartite systems: square, rectangular, honeycomb and square bilayer, for a number of values of N (2 ≤ N ≤ 10), that a close to complete picture of an unusual “deconfined critical point” has emerged. Significantly, no direct evidence for first order behavior has been found on the largest simulations with 256 × 256 spins, the crucial role of Berry phases at the critical point has been verified, strong evidence for non-compact CPN−1 universality is evident for a range of N values, the inferred “dangerous” (ir)relevance of lattice anisotropy at the critical point is consistent with various limiting analytic calculations on the CPN−1 field theory and close to the critical point dramatic signatures of the emergent photon excitation have been detected in VBS correlation functions. I will conclude with some open theoretical issues that remain to be resolved and possible experimental realizations.
We study a spin-1/2 SU(2) model on the honeycomb lattice with nearest-neighbor antiferromagnetic exchange J that favors Néel order and competing six-spin interactions Q that favor a valence-bond-solid (VBS) state in which the bond energies order at the "columnar" wave vector K=(2π/3,-2π/3). We present quantum Monte Carlo evidence for a direct continuous quantum phase transition between Néel and VBS states, with exponents and logarithmic violations of scaling consistent with those at analogous deconfined critical points on the square lattice. Although this strongly suggests a description in terms of deconfined criticality, the measured threefold anisotropy of the phase of the VBS order parameter shows unusual near-marginal behavior at the critical point.
We study the N\'eel to fourfold columnar valence bond solid (cVBS) quantum phase transition in a sign-free
S=1 square-lattice model. This is the same kind of transition that for
S=1/2 has been argued to realize the prototypical deconfined critical point. Extensive numerical simulations of the square-lattice
S=1/2 N\'eel-VBS transition have found consistency with the deconfined critical point scenario with no direct evidence for first-order behavior. In contrast to the
S=1/2 case, in our quantum Monte Carlo simulations for the
S=1 model, we present unambiguous evidence for a direct conventional first-order quantum phase transition. Classic signs of a first-order transition demonstrating coexistence including double-peaked histograms and switching behavior are observed. The sharp contrast from the
S=1/2 case is remarkable; we hypothesize that this is a striking demonstration of the role of the size of the quantum spin in the phase diagram of two-dimensional lattice models.
We generalize the SU(N=2) S=1/2 square-lattice quantum magnet with nearest-neighbor antiferromagnetic coupling (J(1)) and next-nearest-neighbor ferromagnetic coupling (J(2)) to arbitrary N. For all N>4, the ground state has valence-bond-solid order for J(2)=0 and Néel order for J(2)/J(1)≫1, allowing us access to the transition between these types of states for large N. Using quantum Monte Carlo simulations, we show that both order parameters vanish at a single quantum-critical point, whose universal exponents for large enough N (here up to N=12) approach the values obtained in a 1/N expansion of the noncompact CP(N-1) field theory. These results lend strong support to the deconfined quantum-criticality theory of the Néel-valence-bond-solid transition.
To examine the validity of the scenario of the deconfined critical phenomena, we carry out a quantum Monte Carlo simulation for the SU(
N) generalization of the Heisenberg model with four-body and six-body interactions. The quantum phase transition between the SU(
N) N\'eel and valence-bond solid phases is characterized for
N=2, 3, and 4 on the square and honeycomb lattices. While finite-size scaling analysis works well up to the maximum lattice size (
L=256) and indicates the continuous nature of the phase transition, a clear systematic change towards the first-order transition is observed in the estimates of the critical exponent $y\ensuremath{\equiv}1/\ensuremath{\nu}$ as the system size increases. We also confirm the relevance of a squared valence-bond solid field ${\ensuremath{\Psi}}^{2}$ for the SU(3) model.
We use quantum Monte Carlo methods to study the ground-state phase diagram of a
S=1/2 honeycomb lattice magnet in which a nearest-neighbor antiferromagnetic exchange
J (favoring N\'eel order) competes with two different multispin interaction terms: a six-spin interaction
Q3 that favors columnar valence-bond solid (VBS) order, and a four-spin interaction
Q2 that favors staggered VBS order. For ${Q}_{3}\ensuremath{\sim}{Q}_{2}\ensuremath{\gg}J$, we establish that the competition between the two different VBS orders stabilizes N\'eel order in a large swath of the phase diagram even when
J is the smallest energy scale in the Hamiltonian. When ${Q}_{3}\ensuremath{\gg}({Q}_{2},J)$ $\mathrm{[}{Q}_{2}\ensuremath{\gg}({Q}_{3},J)\text{]}$, this model exhibits at zero temperature phase transition from the N\'eel state to a columnar (staggered) VBS state. We establish that the N\'eel-columnar VBS transition is continuous for all values of
Q2, and that critical properties along the entire phase boundary are well characterized by critical exponents and amplitudes of the noncompact
CP1 (NCCP1) theory of deconfined criticality, similar to what is observed on a square lattice. However, a surprising threefold anisotropy of the phase of the VBS order parameter at criticality, whose presence was recently noted at the
Q2=0 deconfined critical point, is seen to persist all along this phase boundary. We use a classical analogy to explore this by studying the critical point of a three-dimensional
XY model with a fourfold anisotropy field which is known to be weakly irrelevant at the three-dimensional
XY critical point. In this case, we again find that the critical anisotropy appears to saturate to a nonzero value over the range of sizes accessible to our simulations.