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arXiv:1306.4216 · Physical Review Letters

Spectrum of a Magnetized Strong-Leg Quantum Spin Ladder

D. Schmidiger, Pierre Bouillot, T. Guidi, Robert Bewley, Corinna Kollath, Thierry Giamarchi, A. Zheludev

Published Sep 3, 2013• 67 citations
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Abstract

Inelastic neutron scattering is used to measure the spin excitation spectrum of the Heisenberg S=1/2 ladder material (C7H10N)2CuBr4 in its entirety, both in the gapped spin liquid and the magnetic field-induced Tomonaga-Luttinger spin liquid regimes. A fundamental change of the spin dynamics is observed between these two regimes. Density matrix renormalization group calculations quantitatively reproduce and help understand the observed commensurate and incommensurate excitations. The results validate long-standing quantum field-theoretical predictions but also test the limits of that approach.

DOI
10.1103/physrevlett.111.107202

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Inelastic neutron scattering is used to measure the spin excitation spectrum of the Heisenberg S=1/2 ladder material (C7H10N)2CuBr4 in its entirety, both in the gapped spin liquid and the magnetic field-induced Tomonaga-Luttinger spin liquid regimes. A fundamental change of the spin dynamics is observed between these two regimes. Density matrix renormalization group calculations quantitatively reproduce and help understand the observed commensurate and incommensurate excitations. The results validate long-standing quantum field-theoretical predictions but also test the limits of that approach.
We measure by inelastic neutron scattering the spin excitation spectra as a function of applied magnetic field in the quantum spin-ladder material (C5H12N)2CuBr4. Discrete magnon modes at low fields in the quantum disordered phase and at high fields in the saturated phase contrast sharply with a spinon continuum at intermediate fields characteristic of the Luttinger-liquid phase. By tuning the magnetic field, we drive the fractionalization of magnons into spinons and, in this deconfined regime, observe both commensurate and incommensurate continua.
The strong-leg S=1/2 Heisenberg spin ladder system (C(7)H(10)N)(2)CuBr(4) is investigated using density matrix renormalization group calculations, inelastic neutron scattering, and bulk magnetothermodynamic measurements. Measurements showed qualitative differences compared to the strong-rung case. A long-lived two-triplon bound state is confirmed to persist across most of the Brillouin zone in a zero field. In applied fields, in the Tomonaga-Luttinger spin-liquid phase, elementary excitations are attractive, rather than repulsive. In the presence of weak interladder interactions, the strong-leg system is considerably more prone to three-dimensional ordering.
We study the magnetic-field-induced quantum phase transition from a gapped quantum phase that has no magnetic long-range order into a gapless phase in the spin-1/2 ladder compound bis(2,3-dimethylpyridinium) tetrabromocuprate (DIMPY). At temperatures below about 1 K, the specific heat in the gapless phase attains an asymptotic linear temperature dependence, characteristic of a Tomonaga-Luttinger liquid. Inelastic neutron scattering and the specific heat measurements in both phases are in good agreement with theoretical calculations, demonstrating that DIMPY is the first model material for an S=1/2 two-leg spin ladder in the strong-leg regime.
We present NMR measurements of a strong-leg spin-1/2 Heisenberg antiferromagnetic ladder compound (C7H10N)2CuBr4 under magnetic fields up to 15 T in the temperature range from 1.2 K down to 50 mK. From the splitting of NMR lines, we determine the phase boundary and the order parameter of the low-temperature (three-dimensional) long-range-ordered phase. In the Tomonaga-Luttinger regime above the ordered phase, NMR relaxation reflects characteristic power-law decay of spin correlation functions as 1/T1∝T(1/2K-1), which allows us to determine the interaction parameter K as a function of field. We find that field-dependent K varies within the 1<K<2 range, which signifies attractive interaction between the spinless fermions in the Tomonaga-Luttinger liquid.
We study the ground-state spin correlations in the gapless incommensurate regime of a S=1/2S=1/2S=1/2 XXZ\mathrm{XXZ}XXZ chain and a two-leg antiferromagnetic ladder under a magnetic field, in which the gapless excitations form a Tomonaga-Luttinger (TL) liquid. We calculate numerically the two-spin correlation functions and the local magnetization in the two models using the density-matrix renormalization-group method. By fitting the numerical results for an open XXZ\mathrm{XXZ}XXZ chain of 100 spins to correlation functions of a Gaussian model, we determine the TL-liquid parameter K and the amplitudes of the correlation functions. The value of K estimated from the fits is in excellent agreement with the exact value obtained from the Bethe ansatz. We apply the same method to the open ladder consisting of 200 spins and determine the dependence of K on the magnetization M. The $K\ensuremath{-}M$ relation changes drastically depending on the ratio of the coupling constants in the leg and rung directions. We also discuss implications of these results to experiments on the nuclear spin relaxation rate 1/T1{1/T}_{1}1/T1​ and dynamical spin structure factors.
Magnetic excitations in the strong-leg quantum spin ladder compound (C7H10N)2CuBr4{({\mathrm{C}}_{7}{\mathrm{H}}_{10}\mathrm{N})}_{2}{\mathrm{CuBr}}_{4}(C7​H10​N)2​CuBr4​ (known as DIMPY) in the field-induced Tomonaga-Luttinger spin-liquid phase are studied by means of high-field electron spin resonance (ESR) spectroscopy. The presence of a gapped ESR mode with unusual nonlinear frequency-field dependence is revealed experimentally. Using a combination of analytic and exact-diagonalization methods, we compute the dynamical structure factor and identify this mode with longitudinal excitations in the antisymmetric channel. We argue that these excitations constitute a fingerprint of the spin dynamics in a strong-leg spin-1/2 Heisenberg antiferromagnetic ladder and owe their ESR observability to the uniform Dzyaloshinskii-Moriya interaction.