We show that fermionic high-spin systems with spin-changing collisions allow one to monitor superexchange processes in optical superlattices with large amplitudes and strong spin fluctuations. By investigating the non-equilibrium dynamics, we find a superexchange dominated regime at weak interactions. The underlying mechanism is driven by an emerging tunneling-energy gap in shallow few-well potentials. As a consequence, the interaction-energy gap that is expected to occur only for strong interactions in deep lattices is re-established. By tuning the optical lattice depth, a crossover between two regimes with negligible particle number fluctuations is found: firstly, the common regime with vanishing spin-fluctuations in deep lattices and, secondly, a novel regime with strong spin fluctuations in shallow lattices. We discuss the possible experimental realization with ultracold 40 K atoms and observable quantities in double wells and two-dimensional plaquettes.
We show that fermionic high-spin systems with spin-changing collisions allow one to monitor superexchange processes in optical superlattices with large amplitudes and strong spin fluctuations. By investigating the non-equilibrium dynamics, we find a superexchange dominated regime at weak interactions. The underlying mechanism is driven by an emerging tunneling-energy gap in shallow few-well potentials. As a consequence, the interaction-energy gap that is expected to occur only for strong interactions in deep lattices is re-established. By tuning the optical lattice depth, a crossover between two regimes with negligible particle number fluctuations is found: firstly, the common regime with vanishing spin-fluctuations in deep lattices and, secondly, a novel regime with strong spin fluctuations in shallow lattices. We discuss the possible experimental realization with ultracold 40 K atoms and observable quantities in double wells and two-dimensional plaquettes.
We investigate the spin dynamics, starting from the initial band-insulating state, of fermionic high-spin atoms in optical superlattices. Through numerical simulations and analytical calculations, we determine the time evolution behavior of the system. When the spin-changing strength and tunneling strength are comparable, the spin dynamics feature a spin-changing oscillation with the amplitude modulated by the superexchange interaction. When the double-well potential is very shallow, the spin dynamics feature a simple harmonic oscillation with the oscillation frequencies related only to the spin-changing strength, which can be properly explained with the perturbation model.
Ultracold atoms in optical lattices provide a versatile platform for studying many-body physics in a defect-free system with tunable parameters. For the analog quantum simulation of the Fermi-Hubbard model, fermionic atoms take on the role of the valence electrons and optical lattices provide the periodic potential in place of the solid-state crystal. The dynamics in the system are described by the tunneling amplitude t between neighboring lattice sites and the interaction energy U of two particles occupying the same lattice site. With the depth of the optical lattices and an external magnetic field, both parameters can be tuned to access a wide range of regimes. Two superimposed lattices with different lattice periods form an optical superlattice, where the most common configuration is a bichromatic superlattice with lattice periods different by a factor of two. Depending on the lattice depths and the relative phase of the lattices, the bichromatic superlattice potential ranges from an array of weakly-coupled double wells to a continuous lattice potential with a staggered energy offset. We developed a calibration technique for measuring the depth of an optical lattice with local resolution. The band structure of the optical lattice is probed by modulating the lattice depth and exciting the atoms to higher bands. However, compared to resolving the band occupations in a time-of-flight measurement, we further excite the atoms to an untrapped band to deplete the optical lattice along equipotential lines where the modulation frequency is resonant with the local band transitions. From the profile of the lattice depth, we obtain the calibration factor for the power regulation, the waist of the underlying lattice beams and the position of the lattice axis. This technique combines several calibration measurements, thereby reducing the measurement time and enabling an automation of the lattice alignment. For the bichromatic superlattice we realized an active stabilization of the superlattice phase that enables long-term measurements with a precise control over the superlattice phase. The instability of the superlattice phase is a result of the different refractive indices for the two lattices in air and the optical elements along the optical path. Using environmental sensors, we monitor the temperature, the pressure, and the relative humidity to apply the expected correction to the superlattice phase. The stabilized superlattice phase enabled the investigation of Floquet-driven double wells by modulating the energy offset through the superlattice phase. We used a near-resonant driving frequency with respect to the interaction energy to enhance the pair-tunneling amplitude in doubly-occupied double wells compared to static double wells and compared to the tunneling amplitude in singly-occupied double wells.
This dissertation summarizes my recent work regarding systems of strongly interacting fermionic atoms in optical lattices. This work addresses the combination of two experimental techniques that have been the subject of much recent research in ultracold atom physics. One is the use of optical lattices, which provide a means to realize diverse interaction configurations within a clean, controllable system. The other is the use of magnetically tunable Feshbach resonances to control the strength of the interatomic interaction. Together, these techniques offer the possibility of an experimental realization of many important model Hamiltonians of condensed matter physics, and may also lead to the discovery of new physics. Recent study of this system has shown that strong interactions near Feshbach resonance will lead to the population of multiple lattice bands, and that collisions between atoms on neighboring sites cannot be neglected. These effects lead to a complicated Hamiltonian, but one which can be simplified to an effective single-band model equivalent to the generalized Hubbard model (GHM), which is an extension of the Hubbard model that includes correlated hopping terms. My main results concern the study of this model. The strong correlations between the particles make it difficult to definitively determine the many body physics of the GHM. As a first approach to understanding the GHM in optical lattices, I focus mainly on cases where the problem is greatly simplified by allowing interactions among only small groups of lattice sites. This restriction can be implemented in experiments using an optical superlattice potential. Our results include a proposed scheme (based on double-well superlattices) to empirically verify that the GHM describes this system and to directly measure the various parameters of this model. Other results include exact solutions on four-site square plaquettes, which demonstrate that d-wave excitations can occur in the low-energy states. By using a superlattice to give an array of weakly coupled plaquettes, one can thus produce a d-wave superfluid state. This is of relevance to the study of high-Tc superconductors, although I note certain key differences between the sort of d-wave superfluid described here and that of the superconductors.
This thesis presents quantum simulation of strongly-correlated systems beyond standard Hubbard models, using ultracold fermionic potassium atoms in both static and periodically-driven optical superlattices. For this study, we utilize a three-dimensional optical lattice setup, controlling particle interactions via magnetic Feshbach resonances and tunneling between lattice sites through optical lattice intensity. High-resolution absorption imaging combined with radio-frequency spectroscopy distinguishes between singly and doubly occupied sites. To enhance our systems capabilities beyond the standard Hubbard model, we extend the apparatus with an in-plane optical superlattice, creating a bi-chromatic structure by superposition of two optical lattices with commensurate lattice spacings. Using a phase locked loop with an environmental feed forward, we create an excellent phase stability of the superlattice exceeding 3 mrad. This precision allows us to explore both static and periodically-driven one-dimensional tight-binding models with strong interactions. We characterize the static superlattice through radio-frequency spectroscopy and Rabi oscillations, and validate the experimental data against theoretical calculations. In a tilted superlattice configuration, we successfully prepare and detect repulsively bound atom pairs, representing a highly excited eigenstate of the system. Furthermore, we demonstrate control over pair tunneling dynamics in a double-well potential using Floquet engineering, employing a low-noise periodic modulation of the optical superlattice tilt. Using an adiabatic band mapping technique, we directly observe the tunneling dynamics in the driven superlattice. We realize dynamic localization in quarter-filled wells and density-assisted tunneling up to the third harmonic order in half-filled wells. We observe a crossover from density-assited tunneling to dominant pair tunneling by tuning the effective interactions. Remarkably, the pair tunneling is not only enhanced relative to the suppressed single-particle tunneling but also exceeds the superexchange rate of a static double-well by more than a factor of two. This opens the possibility to study many-body systems with dominant pair tunneling, that extend beyond the standard Hubbard model.
Superexchange and inter-orbital spin-exchange interactions are key ingredients for understanding (orbital) quantum magnetism in strongly correlated systems and have been realized in ultracold atomic gases. Here we study the spin dynamics of ultracold alkaline-earth atoms in an optical lattice when the two exchange interactions coexist. In the superexchange interaction dominating regime, we find that the time-resolved spin imbalance shows a remarkable modulated oscillation, which can be attributed to the interplay between local and nonlocal quantum mechanical exchange mechanisms. Moreover, the filling of the long-lived excited atoms affects the collapse and revival of the magnetization dynamics. These observations can be realized in state-dependent optical lattices combined with the state-of-the-art advances in optical lattice clock spectroscopy.
The interplay of magnetic exchange interactions and tunneling underlies many complex quantum phenomena observed in real materials. We study nonequilibrium magnetization dynamics in an extended two-dimensional (2D) system by loading effective spin-1/2 bosons into a spin-dependent optical lattice and use the lattice to separately control the resonance conditions for tunneling and superexchange. After preparing a nonequilibrium antiferromagnetically ordered state, we observe relaxation dynamics governed by two well-separated rates, which scale with the parameters associated with superexchange and tunneling. With tunneling off-resonantly suppressed, we observe superexchange-dominated dynamics over two orders of magnitude in magnetic coupling strength. Our experiment will serve as a benchmark for future theoretical work as the detailed dynamics of this 2D, strongly correlated, and far-from-equilibrium quantum system remain out of reach of current computational techniques.