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arXiv:1305.6082 · Nature Communications

Time-resolved magnetic sensing with electronic spins in diamond

A. Cooper, Easwar Magesan, H. Yum, Paola Cappellaro

Published Jan 24, 2014• 73 citations
arXivHTMLPDF
DOI
10.1038/ncomms4141

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Time-resolved magnetic sensing is of great importance from fundamental studies to applications in physical and biological sciences. Recently, the nitrogen-vacancy defect center in diamond has been developed as a promising sensor of magnetic fields under ambient conditions. However, methods to reconstruct time-resolved magnetic fields with high sensitivity are not yet fully developed. Here, we propose and demonstrate a sensing method based on spin echo and Haar wavelet transformation. Our method is exponentially faster in reconstructing time-resolved magnetic fields with comparable sensitivity than existing methods. It is also easier to implement in experiments. Furthermore, the wavelet's unique features enable our method to extract information from the whole signal with only part of the measuring sequences. We then explore this feature for a fast detection of simulated nerve impulses. These results will be useful to time-resolved magnetic sensing with quantum probes at nanoscale.
Many-body dynamics constitutes a promising approach for creating correlations between quantum particles which can be used for applications in sensing and metrology. However, utilizing this potential for substantial gains in practical settings is a challenging task with only a very few applications realized to date. Here, we demonstrate an approach to nanoscale magnetic sensing enabled by strongly interacting electronic spins in a room temperature solid. By coherently controlling collective many-body dynamics of a dipolar ensemble of ∼104\sim 10^4∼104 nitrogen-vacancy (NV) centres in diamond with pulsed magnetic field gradients, we demonstrate practical metrological gain up to 7.9(2) dB7.9(2)\,\mathrm{dB}7.9(2)dB for magnetic signal detection and 8.8(3) dB8.8(3)\,\mathrm{dB}8.8(3)dB for magnetic noise sensing, fully accounting for experimental overheads. Finally, we combine these methods to demonstrate a momentum-space-resolved sensing modality that enables detection of spatially correlated magnetic noise at continuously tunable length scales down to 50 nanometers. These observations open the door toward practical applications of interaction-enhanced quantum sensors for nanoscale biological imaging and material characterization.
Quantum-enhanced sensing with spin-bearing defects in solids is important for measuring magnetic fields at the atomic scale, but progress is impeded by the difficulty of accessing ensembles of strongly coupled spins that can be entangled deterministically. This study exploits an optically dark electronic-nuclear spin defect near a single nitrogen-vacancy center in diamond to create an entangled state of two electronic spins, and measure the amplitude of time-varying magnetic fields with superior performance. With their stability under optical illumination, dark electronic spins can be repeatedly measured through the N-VVV center to further improve the signal-to-noise ratio.