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arXiv:1305.4834

On the high energy spin excitations in the high temperature superconductors: an RVB theory

Jiquan Pei, Haijun Liao, Tao Li

Published May 21, 2013• 1 citation
arXivHTMLPDF

Abstract

The high energy spin excitation in the high T$_{c}$ cuprates is studied in the single mode approximation for the $t-t'-J$ model. An exact form for the mode dispersion is derived. When the Gutzwiller projected BCS state is used as the variational ground state, a spin-wave-like dispersion of about 2.2$J$ is uncovered along the $Γ=(0,0)$ to $\mathrm{M}=(π,0)$ line. Both the mode energy and the integrated intensity of the spin fluctuation spectrum are found to be almost doping independent in large doping range, which agrees very well with the observations of recent RIXS measurements. Together with previous studies on the quasiparticle properties of the Gutzwiiler projected BCS state, our results indicate that such a Fermionic RVB theory can provide a consistent description of both the itinerant and the local aspect of electronic excitations in the high T$_{c}$ cuprates.

DOI
10.48550/arxiv.1305.4834

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The high energy spin excitation in the high Tc_{c}c​ cuprates is studied in the single mode approximation for the t−t′−Jt-t'-Jt−t′−J model. An exact form for the mode dispersion is derived. When the Gutzwiller projected BCS state is used as the variational ground state, a spin-wave-like dispersion of about 2.2JJJ is uncovered along the Γ=(0,0)Γ=(0,0)Γ=(0,0) to M=(π,0)\mathrm{M}=(π,0)M=(π,0) line. Both the mode energy and the integrated intensity of the spin fluctuation spectrum are found to be almost doping independent in large doping range, which agrees very well with the observations of recent RIXS measurements. Together with previous studies on the quasiparticle properties of the Gutzwiiler projected BCS state, our results indicate that such a Fermionic RVB theory can provide a consistent description of both the itinerant and the local aspect of electronic excitations in the high Tc_{c}c​ cuprates.
Low-lying one-particle anomalous excitations are studied for Gutzwiller-projected strongly correlated BCS states. It is found that the one-particle anomalous excitations are highly coherent, and the numerically calculated spectrum can be reproduced quantitatively by a renormalized BCS theory, thus strongly indicating that the nature of low-lying excitations described by the projected BCS states is essentially understood within a renormalized Bogoliubov quasiparticle picture. This finding resembles the well-known fact that a Gutzwiller-projected Fermi gas is a Fermi liquid. The present results are consistent with numerically exact calculations of the two-dimensional $t\text{\ensuremath{-}}J$ model as well as recent photoemission experiments on high-TC{T}_{\mathrm{C}}TC​ cuprate superconductors.
We provide a unified interpretation of both paramagnon and plasmon modes in high-Tc{T}_{c}Tc​ copper-oxides, and verify it quantitatively against available resonant inelastic xxx-ray scattering (RIXS) data across the hole-doped phase diagram. The three-dimensional extended Hubbard model, with included long-range Coulomb interactions and doping-independent microscopic parameters for both classes of quantum fluctuations, is used. Collective modes are studied using VWF+1/Nf\mathrm{VWF}+1/{\mathcal{N}}_{f}VWF+1/Nf​ approach which extends variational wave function (VWF) scheme by means of an expansion in inverse number of fermionic flavors (1/Nf)(1/{\mathcal{N}}_{f})(1/Nf​). We show that intense paramagnons persist along the antinodal line from the underdoped to the overdoped regime and undergo rapid overdamping in the nodal direction. Plasmons exhibit a three-dimensional character, with minimal energy corresponding to antiphase oscillations on neighboring CuO2{\mathrm{CuO}}_{2}CuO2​ planes. The theoretical spin- and charge excitation energies reproduce semiquantitatively RIXS data for ${(\mathrm{Bi},\mathrm{Pb})}_{2}{(\mathrm{Sr},\mathrm{La})}_{2}{\mathrm{CuO}}_{6+\ensuremath{\delta}}$. The present VWF+1/Nf\mathrm{VWF}+1/{\mathcal{N}}_{f}VWF+1/Nf​ analysis of dynamics and former VWF results for static quantities combine into a consistent description of the principal properties of hole-doped high-Tc{T}_{c}Tc​ cuprates as strongly correlated systems.
A d-wave superconducting ground state for a doped Mott insulator is obtained. It is distinguished from a Gutzwiller-projected Bardeen–Cooper–Schrieffer (BCS) superconductor by an explicit separation of Cooper pairing and resonating valence bond (RVB) pairing. Such a state satisfies the precise sign structure of the t–J model, just as a BCS state satisfies the Fermi–Dirac statistics. This new class of wavefunctions can be intrinsically characterized and effectively manipulated by electron fractionalization with neutral spinons and 'backflow' spinons forming a two-component RVB structure. While the former spinon is bosonic, originating from the superexchange correlation, the latter spinon is found to be fermionic, accompanying the hopping of bosonic holons. The low-lying emergent gauge fields associated with such a specific fractionalization are of mutual Chern–Simons type. Corresponding to this superconducting ground state, three types of elementary excitations are identified. Among them a Bogoliubov nodal quasiparticle is conventional, while the other two are neutral excitations of non-BCS type that play crucial roles in higher-energy/temperature regimes. Their unique experimental implications for the cuprates are briefly discussed.
The principal purpose of this topical review is to single out some of the universal features of high-temperature (high-Tc) and related strongly-correlated systems, which can be compared with experiment in a quantitative manner. The description starts with the concept of exchange-interaction-mediated (real-space) pairing, combined with strong correlations among narrow band electrons, for which the reference state is that of the Mott–Hubbard insulator. The physical discussion of concrete properties relies on variational approach, starting from generalized renormalized mean-field theory (RMFT) in the form of statistically-consistent Gutzwiller approximation (SGA), and its subsequent generalization, i.e., a systematic Diagrammatic Expansion of the Variational (Gutzwiller-type) Wave Function (DE-GWF). The solution leads to the two energy scales, one involving unconventional quasiparticles close to the Fermi energy, and the other reflecting the fully correlated state, involving electrons deeper below the Fermi surface. Those two regimes are separated by a kink in the dispersion relation, which is observed in photoemission. As a result, one obtains both the doping dependent properties in the correlated state, and effective renormalized quasiparticles. The reviewed ground-state characteristics for high-Tc systems encompass high-Tc superconductivity, nematicity, charge- (and pair-) density-wave effects, as well as non-BCS kinetic energy gain in the paired state. The calculated dynamic properties are: the universal Fermi velocity, the Fermi wave-vector, the effective mass enhancement, the pseudogap; and the d-wave gap magnitude. We discuss that, within the variational approach, the minimal realistic model is represented by the so-called t-J-U Hamiltonian. Inadequacy of the t-J and Hubbard models, particularly of their RMFT versions, is discussed explicitly. For heavy fermion systems, modeled by the Anderson lattice model and with the DE-GWF approach, we discuss the phase diagram, encompassing superconducting, Kondo insulating, ferro- and anti-ferromagnetic states. The superconducting state is then a two-d-wave gap system. If the orbital degeneracy of f-electrons is included, the coexistent ferromagnetic- (spin–triplet) superconducting phases appear and match those observed for UGe2 in a semiquantitative manner. Finally, in the second part, we generalize our approach to the collective spin and charge fluctuations in high-Tc systems, starting from variational approach, defining the saddle-point state, and combining it with 1/N expansion. The present scheme differs essentially from that starting from the saddle-point Hartree–Fock approximation, and incorporating the fluctuations in the random phase approximation (RPA). The spectrum of collective spin and charge excitations is determined for the Hubbard and t-J-U models, and subsequently compared quantitatively with recent experiments. The Appendices provide formal details to make this review self-contained.
The generic phase diagram of lightly hole doped high-Tc{T}_{c}Tc​ cuprates hosts an antiferromagnetic insulating phase with well-defined spin-wave excitations. Contrary to the weak-coupling prediction, these modes persist up to the overdoped metallic regime as intense and dispersive paramagnons. Here we report on our study of the low-energy magnetic and charge excitations within the extended Hubbard model at strong coupling, using a modified 1/N1/N1/N expansion method with a variational state serving as the saddle point solution. Despite clear separation of magnetic and Hubbard-UUU energy scales, we find that incipient Mottness affects qualitatively dispersions and widths of magnetic modes throughout the entire phase diagram. The obtained magnetic and charge dynamical structure factors agree semiquantitatively with recent resonant x-ray and neutron scattering data for ${\mathrm{La}}_{2\ensuremath{-}\mathit{x}}{\mathrm{Sr}}_{\mathit{x}}{\mathrm{CuO}}_{4}$ and ${(\mathrm{Bi},\mathrm{Pb})}_{2}{(\mathrm{Sr},\mathrm{La})}_{2}{\mathrm{CuO}}_{6+\ensuremath{\delta}}$ at all available doping levels. The weak-coupling random-phase approximation fails already for underdoped samples, pointing to the nontrivial intertwining of distinct energy scales in cuprate superconductors. The existence of a discrete charge mode which splits off the electron-hole continuum is also predicted.
We study the electronic structure of a strongly correlated d-wave superconducting state. Combining a renormalized mean field theory with direct calculation of matrix elements, we obtain explicit analytical results for the nodal Fermi velocity upsilon(F), the Fermi wave vector k(F), and the momentum distribution n(k) as a function of hole doping in a Gutzwiller projected d-wave superconductor. We calculate the energy dispersion E(k) and spectral weight of the Gutzwiller-Bogoliubov quasiparticles and find that the spectral weight associated with the quasiparticle excitation at the antinodal point shows a nonmonotonic behavior as a function of doping. Results are compared to angle resolved photoemission spectroscopy of the high-temperature superconductors.