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arXiv:1305.2488 · Physical Review A

QED with a parabolic mirror

G. Alber, József Zsolt Bernád, Magdalena Stobińska, Luis Lorenzo Sánchez-Soto, Gerd Leuchs

Published Aug 14, 2013• 29 citations
arXivHTMLPDF

Abstract

We investigate the quantum electrodynamics of a single two-level atom located at the focus of a parabolic cavity. We first work out the modifications of the spontaneous emission induced by the presence of this boundary in the optical regime, where the dipole and the rotating-wave approximations apply. Furthermore, the single-photon state that leaves the cavity asymptotically is determined. The corresponding time-reversed single-photon quantum state is capable of exciting the atom in this extreme multimode scenario with near-unit probability. Using semiclassical methods, we derive a photon-path representation for the relevant transition amplitudes and show that it constitutes a satisfactory approximation for a wide range of wavelengths.

DOI
10.1103/physreva.88.023825

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We investigate the quantum electrodynamics of a single two-level atom located at the focus of a parabolic cavity. We first work out the modifications of the spontaneous emission induced by the presence of this boundary in the optical regime, where the dipole and the rotating-wave approximations apply. Furthermore, the single-photon state that leaves the cavity asymptotically is determined. The corresponding time-reversed single-photon quantum state is capable of exciting the atom in this extreme multimode scenario with near-unit probability. Using semiclassical methods, we derive a photon-path representation for the relevant transition amplitudes and show that it constitutes a satisfactory approximation for a wide range of wavelengths.
We investigate spontaneous photon emission processes of two-level atoms in parabolic and ellipsoidal cavities thereby taking into account the full multimode scenario. In particular, we calculate the excitation probabilities of the atoms and the energy density of the resulting few-photon electromagnetic radiation field by using semiclassical methods for the description of the multimode scenario. Based on this approach photon path representations are developed for relevant transition probability amplitudes which are valid in the optical frequency regime where the dipole and the rotating-wave approximations apply. Comparisons with numerical results demonstrate the quality of these semiclassical results even in cases in which the wave length of a spontaneously emitted photon becomes comparable or even larger than characteristic length scales of the cavity. This is the dynamical regime in which diffraction effects become important so that geometric optical considerations are typically not applicable.
The spectral properties of a photon spontaneously emitted by a material two-level system, modelling an atom or ion, in a parabolic cavity are investigated.In particular, we concentrate on the special case of a motionless two-level system positioned exactly at the focus of a parabolic cavity with a dipole moment oriented along the symmetry axis of this cavity.Treating the corresponding atom-field coupling in the dipoleand rotating wave approximation, it is demonstrated that inside the parabolic cavity the position and frequency dependence of the spectrum of the spontaneously emitted photon exhibits interesting interference patterns.These patterns are explored in detail with the help of a photon path representation of the first-order electric field correlation function.In the radiation, zone the spatial behavior of the spectrum reveals strong interference in particular at distances from the two-level system of the order of the focal length of the parabola.With increasing distances, these interference patterns decay except for an undepleted component surrounding the symmetry axis at an almost constant radius.Furthermore, the maximum of the frequency dependence of the spectrum exhibits a position-dependent frequency shift with respect to the atomic resonance frequency.
A single two-level emitter coupled to a single mode of an electromagnetic resonator constitutes the most fundamental instance of light--matter interaction. Realizations of this type of system are investigated in the field of cavity quantum electrodynamics (cavity QED). Particularly important are schemes in which the coupling is strong enough to exceed the spontaneous emission rate as well as cavity damping. In this case, the coherent exchange of excitation between source and photon is the dominating process, providing the unique possibility to deterministically control the quantum evolution of the system. Great progress has recently been accomplished, technologically as well as conceptually, and the focus section in this issue of Journal of Optics B: Quantum and Semiclassical Optics features five articles highlighting important recent developments in the field. Strong coupling between single atoms and the electromagnetic cavity field have been achieved in two distinct regimes, the optical and the microwave region. The latter is represented by the micromaser, a high-Q microwave cavity pumped by a beam of highly excited Rydberg atoms. It has proved to be an almost ideal system for the generation of non-classical field states. A constraint in these experiments is the fact that the field inside the cavity can only be examined indirectly, by analysing the occupation of atoms leaving the cavity. While only two atomic states were previously identified for this purpose, V A Reshetov shows in his article (pages 119--126) that more information on the field may be extracted by taking advantage of the Zeeman substructure of the atomic levels. In the optical domain of cavity QED, by contrast, the state of the resonator field may be probed directly by measuring the light leaking from the cavity using photodetectors. In order to minimize damping, high-quality cavities must be employed. In most optical experiments these are Fabry--Perot resonators with ultra-high reflectivity mirrors, with losses as low as a few parts per million being state of the art. At the same time, the coupling of atoms and photons is enhanced by reducing the length of the cavity, so that strong coupling conditions are reached. A very attractive application of this type of cavity QED setup is the possibility of exerting control over the quantum dynamics of the system. An impressive example is the implementation of quantum feedback, reported in the paper by W P Smith and L A Orozco (pages 127--134). Using information gained from detecting a single photon escaping from the cavity, active feedback is applied to halt the dynamical evolution of the system. This is the first time active feedback has been used to modify the quantum evolution of a system at the single-photon level. The authors discuss how detunings between the subsystems affect the quantum feedback, an issue particularly relevant for ensembles of atoms with a spread in detuning. Perfect quantum feedback in this case requires the use of additional parameters to control the system. The majority of optical cavity QED experiments performed so far have used as a medium atoms traversing the cavity on random trajectories, such as, for example, thermal atomic beams. In this case, the observation of quantum effects is degraded in two ways. The Doppler effect and the finite transit time lead to line broadening, while the spatial structure of the cavity mode results in atoms in different locations experiencing different coupling with the photonic field. J E Reiner et al (pages 135--142) investigate the impact of these effects on quantum fluctuations in their cavity QED system. In order to overcome line broadening, they have developed a continuous cold atomic beam, extracted from a magneto-optical trap. An even better control of broadening effects and fluctuating coupling strength is provided by trapping the atoms inside the cavity and cooling them to temperatures at which their position spread is smaller than the optical wavelength. Much recent activity has been devoted to developing such an ultimate cavity QED system. A Vukics et al (pages 143--153) present a theoretical proposal for dynamically trapping and cooling atoms inside a cavity. By driving the atoms with a standing wave injected from the side of the cavity and by weakly exciting the cavity field itself, they predict three-dimensional trapping of the atom for periods around 1 second, an extremely long time on the typical scale of cavity QED dynamics. The essential component of their scheme is the interference between the two driving fields, determining the temperature of the particle and the stable trapping positions. In the quest for better confinement of radiation, lately, an appealing alternative to the Fabry--Perot cavity has been investigated -- the optical microsphere resonator. A sphere with a diameter of a few tens of microns, it supports so-called whispering gallery modes near its circumference, for which quality factors up to 10 10 have been measured. In order to exploit the correspondingly low field damping rates for cavity QED, a method must be found to couple atomic or solid state emitters to these modes. S Göotzinger et al (pages 154--158) report the coupling of single nanocrystals on the surface of a microsphere through the evanescent field of the mode. Selective excitation of a single nano-emitter was accomplished with a scanning confocal microscope. The system is a promising candidate for cavity QED with single-quantum emitters. The ability to fully control the quantum dynamics of atoms and light is beginning to spawn early applications. The most notable example is quantum information processing. This requires the coherent manipulation of single-quantum systems, which is ideally provided by cavity QED interaction in the strong-coupling limit. The development of practical devices will be among the principal future tasks for research in the field. This will include physical systems, which have not been covered in this issue, such as semiconductors, quantum dots as emitters, or photonic crystals as resonator structures. Cavity QED is therefore guaranteed to remain a vigorous field in the years to come.
Rapid advances in quantum technology have made possible the control of quantum states of elementary material quantum systems, such as atoms or molecules, and of the electromagnetic radiation field resulting from spontaneous photon emission of their unstable excited states to such a level of precision that subtle quantum electrodynamical phenomena have become observable experimentally. Recent developments in the area of quantum information processing demonstrate that characteristic quantum electrodynamical effects can even be exploited for practical purposes provided the relevant electromagnetic field modes are controlled by appropriate cavities. A central problem in this context is the realization of an ideal transfer of quantum information between a state of a material quantum system and a quantum state of the electromagnetic radiation field which contains a small number or even a single photon only. Despite much recent work in cavity quantum electrodynamics, which has explored this problem successfully in cases in which the number of accessible electromagnetic field modes is strongly restricted by a cavity, currently still much less is known about ideal quantum state transfer between matter and few-photon quantum states of the electromagnetic field in the extreme opposite case of free space. In this contribution we review recent work which explores characteristic quantum electrodynamical phenomena governing the interaction of a material quantum system with the electromagnetic field in extreme many-mode cases which are close to cavity-free situations. For this purpose the simplest possible quantum electrodynamical situation, namely the interaction of a single material two-level system with the wave packet of a single optical photon, is investigated in free space and in situations in which a large cavity modifies the mode structure of the electromagnetic field modes. It is demonstrated that perfect excitation of an atom by a properly shaped single-photon wave packet is possible even in free space. In particular, it is demonstrated that perfect excitation of an atom can be achieved by a single optical photon which is prepared initially in an appropriate superposition of plane-wave modes, provided this photon is focused subsequently onto the absorbing atom by a parabolic cavity.
The problem of a single two level atom in its excited state, placed in a cavity in which no photons are present initially, and interacting with N modes of the electromagnetic field is solved exactly in the electric dipole, rotating wave approximation. Expressions for the energy eigenvalues and eigenvectors are derived, and an exact representation for the time dependent wavefunction of the system is given. These quantities are evaluated analytically for N=1,2 and 3, and the time dependent properties of the system for these values of N are investigated and discussed.
The efficient interaction between single photons and single matter objects in free space is of key importance for quantum technologies. An experimental setup for testing this possibility involves single two-level ion trapped at the focus of a parabolic metallic mirror. We study the conditions for the setup, under which the assumption about the free-space mode structure of the radiation field in the vicinity of the atom is justified. In our analysis we apply vectorial properties of light by including the polarization degree of freedom. We look for possible changes in the spontaneous emission rate of the atom resulting from the presence of the parabolic boundary conditions.