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arXiv:1305.1714 · Physical Review A

Microscopic characterization of Lévy flights of light in atomic vapors

Nicolas Mercadier, Martine Chevrollier, William Guerin, Robin Kaiser

Published Jun 24, 2013• 20 citations
arXivHTMLPDF

Abstract

We investigate multiple scattering of near-resonant light in a Doppler-broadened atomic vapor. We experimentally characterize the length distribution of the steps between successive scattering events. The obtained power law is characteristic of a superdiffusive behavior, where rare but very long steps (L\'evy flights) dominate the transport properties.

DOI
10.1103/physreva.87.063837

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We investigate multiple scattering of near-resonant light in a Doppler-broadened atomic vapor. We experimentally characterize the length distribution of the steps between successive scattering events. The obtained power law is characteristic of a superdiffusive behavior, where rare but very long steps (L'evy flights) dominate the transport properties.
Multiple scattering of light by resonant vapor is characterized by Lévy-type superdiffusion with a single-step size distribution p(x)∝1/x^{1+α}. We investigate Lévy flight of light in a hot rubidium vapor collisional-broadened by 50 torr of He gas. The frequent collisions produce Lorentzian absorptive and emissive profiles with α<1 and a corresponding divergent mean step size. We extract the Lévy parameter α≈0.5 in a multiple-scattering regime from radial profile of the transmission and from violation of the Ohm's law. The measured radial transmission profile and the total diffusive transmission curves are well reproduced by numerical simulations for Lorentzian line shapes.
The propagation of light in a resonant atomic vapor can a priori be thought of as a multiple scattering process, in which each scattering event redistributes both the direction and the frequency of the photons. Particularly, the frequency redistribution may result in L\'evy flights of photons, directly affecting the transport properties of light in a resonant atomic vapor and turning this propagation into a superdiffusion process. Here, we report on a Monte Carlo simulation developed to study the evolution of the spectrum of the light in a resonant thermal vapor. We observe the gradual change of the spectrum and its convergence towards a regime of complete frequency redistribution as the number of scattering events increases. We also analyze the probability density function of the step length of photons between emissions and reabsorptions in the vapor, which governs the statistics of the light diffusion. We observe two different regimes in the light transport: superdiffusion when the vapor is excited near the line center and normal diffusion for excitation far from the line center. The regime of complete frequency redistribution is not reached for excitation far from resonance even after many absorption and reemission cycles due to correlations between emitted and absorbed frequencies.
We experimentally investigate the transmission of light by dense atomic vapor. The light propagating in dense atomic vapor can be modeled as a Lévy flight random walk. For such system, the step-length distribution can be modeled as P(ℓ)∼ℓ−1−α(ℓ)P(\ell)\sim \ell^{-1-α(\ell)}P(ℓ)∼ℓ−1−α(ℓ), with the Lévy index α(ℓ)α(\ell)α(ℓ) varying smoothly with the step length. Moreover, the walkers alternate between two distinct distributions depending on the occurrence of collisions between atoms in the light scattering. We obtain the Lévy index from transmission measurements for different system sizes and atomic densities. The measured Lévy index is determined by the system size α=α(ℓ=L)α=α(\ell=L)α=α(ℓ=L). Simulations are made for walkers alternating between two Lévy like step-length
Lévy flight superdiffusion consists of random walks characterized by very long jumps that dominate the transport. However, the finite size of real samples introduces truncation of long jumps and modifies the transport properties. We measure typical Levy flight parameters for photon diffusion in atomic vapor characterized by a Voigt absorption profile. We observe the change of Lévy parameter as a function of truncation length. We associate this variation with size-dependent contributions from different spectral regions of the emission profile with the Doppler core dominating the transport for thin samples and Lorentz wings for thick samples. Monte Carlo simulations are implemented to support the interpretation of results.
Multiple scattering is a process in which a particle is repeatedly deflected by other particles. In an overwhelming majority of cases, the ensuing random walk can successfully be described through Gaussian, or normal, statistics. However, like a (growing) number of other apparently inoffensive systems, diffusion of light in dilute atomic vapours eludes this familiar interpretation, exhibiting a superdiffusive behaviour. As opposed to normal diffusion, whereby the particle executes steps in random directions but with lengths slightly varying around an average value (like a drunkard whose next move is unpredictable but certain to within a few tens of centimetres), superdiffusion is characterised by sudden abnormally long steps (Lévy flights) interrupting sequences of apparently regular jumps which, although very rare, determine the whole dynamics of the system. The formal statistics tools to describe superdiffusion already exist and rely on stable, well understood distributions. As scientists become aware of, and more familiar with, this non-orthodox possibility of interpretation of random phenomena, new systems are discovered or re-interpreted as following Lévy statistics. Propagation of light in resonant atomic vapours is one of these systems which have been studied for decades and have only recently been shown to be the scene of Lévy flights.