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arXiv:1305.1516 · Journal of Physics B Atomic Molecular and Optical Physics

Coherent internal state transfer by a three-photon STIRAP-like scheme for many-atom samples

Marius Romuald Kamsap, Thierry Blanchard Ekogo, J. Pedregosa-Gutierrez, G. Hagel, M. Houssin, Olivier Morizot, Martina Knoop, C. Champenois

Published Jun 21, 2013• 11 citations
arXivHTMLPDF

Abstract

A STIRAP-like scheme is proposed to exploit a three-photon resonance taking place in alkaline-earth-metal ions. This scheme is designed for state transfer between the two fine structure components of the metastable D-state which are two excited states that can serve as optical or THz qu-bit. The advantage of a coherent three-photon process compared to two-photon STIRAP lies in the possibility of exact cancellation of the first order Doppler shift which opens the way for an application to a sample composed of many ions. The transfer efficiency and its dependence with experimental parameters are analyzed by numerical simulations. This efficiency is shown to reach a fidelity as high as $(1-8.10^{-5})$ with realistic parameters. The scheme is also extended to the synthesis of a linear combination of three stable or metastable states.

DOI
10.1088/0953-4075/46/14/145502

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A STIRAP-like scheme is proposed to exploit a three-photon resonance taking place in alkaline-earth-metal ions. This scheme is designed for state transfer between the two fine structure components of the metastable D-state which are two excited states that can serve as optical or THz qu-bit. The advantage of a coherent three-photon process compared to two-photon STIRAP lies in the possibility of exact cancellation of the first order Doppler shift which opens the way for an application to a sample composed of many ions. The transfer efficiency and its dependence with experimental parameters are analyzed by numerical simulations. This efficiency is shown to reach a fidelity as high as (1−8.10−5)(1-8.10^{-5})(1−8.10−5) with realistic parameters. The scheme is also extended to the synthesis of a linear combination of three stable or metastable states.
We demonstrate coherent three-photon excitation of the strontium clock transition with a contrast of 51(12)% using a Bose-Einstein condensate. We follow it up with a demonstration of three-photon STIRAP-like transfer, overcoming the typical limitations of this technique to odd-level numbers. We also measure the two-body loss coefficient of Sr 84 clock-state atoms. Our work constitutes an essential step towards outcoupling a continuous atom laser beam and provides a fast excitation mechanism for quantum simulation using bosonic alkaline-earth-like atoms.
Abstract STIRAP (stimulated Raman adiabatic passage) is a powerful laser-based method, usually involving two photons, for efficient and selective transfer of populations between quantum states. A particularly interesting feature is the fact that the coupling between the initial and the final quantum states is via an intermediate state, even though the lifetime of the latter can be much shorter than the interaction time with the laser radiation. Nevertheless, spontaneous emission from the intermediate state is prevented by quantum interference. Maintaining the coherence between the initial and final state throughout the transfer process is crucial. STIRAP was initially developed with applications in chemical dynamics in mind. That is why the original paper of 1990 was published in The Journal of Chemical Physics . However, from about the year 2000, the unique capabilities of STIRAP and its robustness with respect to small variations in some experimental parameters stimulated many researchers to apply the scheme to a variety of other fields of physics. The successes of these efforts are documented in this collection of articles. In Part A the experimental success of STIRAP in manipulating or controlling molecules, photons, ions or even quantum systems in a solid-state environment is documented. After a brief introduction to the basic physics of STIRAP, the central role of the method in the formation of ultracold molecules is discussed, followed by a presentation of how precision experiments (measurement of the upper limit of the electric dipole moment of the electron or detecting the consequences of parity violation in chiral molecules) or chemical dynamics studies at ultralow temperatures benefit from STIRAP. Next comes the STIRAP-based control of photons in cavities followed by a group of three contributions which highlight the potential of the STIRAP concept in classical physics by presenting data on the transfer of waves (photonic, magnonic and phononic) between respective waveguides. The works on ions or ion strings discuss options for applications, e.g. in quantum information. Finally, the success of STIRAP in the controlled manipulation of quantum states in solid-state systems, which are usually hostile towards coherent processes, is presented, dealing with data storage in rare-earth ion doped crystals and in nitrogen vacancy (NV) centers or even in superconducting quantum circuits. The works on ions and those involving solid-state systems emphasize the relevance of the results for quantum information protocols. Part B deals with theoretical work, including further concepts relevant to quantum information or invoking STIRAP for the manipulation of matter waves. The subsequent articles discuss the experiments underway to demonstrate the potential of STIRAP for populating otherwise inaccessible high-lying Rydberg states of molecules, or controlling and cooling the translational motion of particles in a molecular beam or the polarization of angular-momentum states. The series of articles concludes with a more speculative application of STIRAP in nuclear physics, which, if suitable radiation fields become available, could lead to spectacular results.
We demonstrate experimentally how the process of stimulated Raman adiabatic passage (STIRAP) can be utilized for efficient coherent internal state transfer in single trapped and laser-cooled 40 Ca + ions. The transfer from the D 3/2 to the D 5/2 state, is detected by a fluorescence measurement revealing the population not transferred to the D 5/2 state. A coherent population transfer efficiency at the level of 95% in a set-up allowing for the internal state detection of individual ions in a string has been obtained.
The field of quantum computation and communication has prospered over the last few decades because of multiple advances in our understanding of trapping and controlling physical quantum systems like neutral atoms, superconducting qubits, trapped ions, quantum dots etc. using light. A lot of research has gone into development of techniques which facilitate trapping and manipulation of ensembles of neutral atoms by studying how the atomic properties of the system respond to properties of light used to control them. In this dissertation we shall explore some applications of light-matter interactions in ensembles of lambda three level neutral atoms for the purpose of entanglement generation and distribution. The first part of this dissertation focuses on the study of a protocol that can be used to generate multi-particle entangled quantum states called the Greenberger-Horne-Zeilinger (GHZ) states in an ensemble of N neutral atoms. Schemes for creation of N particle entangled Greenberger-Horne-Zeilinger (GHZ) states are important for understanding multi-particle non-classical correlations. A theoretical protocol for creation of a multi-particle GHZ state implemented on a target ensemble of N, three-level Rydberg atoms and a single Rydberg atom as a control using Stimulated Raman Adiabatic Passage (STIRAP) is presented. We work in the Rydberg blockade regime for the ensemble atoms induced due to excitation of the control atom to a high lying Rydberg level. It is shown that using STIRAP, atoms from one ground state of the ensemble can be adiabatically transferred with high fidelity to the other multi-particle ground state, depending on the state of the control atom. Measurement of the control atom in a specific basis after this conditional transfer facilitates one-step creation of a N particle GHZ state. A thorough analysis of adiabatic conditions associated with STIRAP for this scheme and the influence of radiative decay from the excited Rydberg levels is presented. The most important and novel feature of this scheme is that it is immune to the decay rate of the excited level in ensemble atoms and provides a robust way of creating GHZ states. In the second part of this dissertation, we study atomic ensemble based quantum interfaces used in quantum repeater protocols for entanglement distribution. Quantum interfaces provide a platform where in the flying photonic qubits used for information and entanglement transfer can interact with a physical system which stores, processes and releases this information back as photons. The Duan-Lukin-Cirac-Zoller (DLCZ) quantum repeater protocol, which was proposed to realize long distance quantum communication, requires usage of quantum memories or quantum interfaces. Atomic ensembles interacting with optical beams based on off-resonant Raman scattering serve as convenient on-demand quantum memories. Here a complete, free space, three-dimensional theory of the associated read and write process for this quantum memory is worked out with the aim of understanding intrinsic retrieval efficiency. We develop a formalism to calculate the transverse mode structure for the signal and the idler photons and use the formalism to study the intrinsic retrieval efficiency under various configurations. The effects of atomic density fluctuations and atomic motion are incorporated by numerically simulating this system for a range of realistic experimental parameters. Results describe the variation in the intrinsic retrieval efficiency as a function of the memory storage time for skewed beam configuration at a finite temperature, which provides valuable information for optimization of the retrieval efficiency in experiments.
Ongoing work aimed at developing highly efficient methods of populating a chosen sublevel of an energy level highlights the need to understand off-resonant effects in coherent excitation. This motivated us to re-examine some aspects of the theory of coherent excitation in a three-state system with a view to obtaining algebraic expressions for off-resonant eigenvalues and eigenvectors. Earlier work gives simple closed-form expressions for the eigenvalues this system, expressions applying even when the system is not on two-photon resonance. We present here expressions of similar simplicity for the components of the normalised eigenvectors. The analytic properties of these components explain the observed sensitivity of the stimulated-Raman-adiabatic-passage process (STIRAP) to the condition of two-photon resonance. None of the eigenstates is ‘trapped’ or ‘dark’ unless the system is on two-photon resonance; off resonance, all states have nonzero projections on the unperturbed intermediate state. A simple argument shows that no dressed state can be adiabatically connected to both the unperturbed initial and final states when the system is off two-photon resonance. That is, adiabatic transfer from initial to final state requires that these be degenerate before and after the STIRAP pulse sequence, and this implies zero two-photon detuning. However, substantial transfer probabilities are observed experimentally for very small two-photon detunings. We show that such systems are characterised by very sharp avoided crossings of two eigenvalues, and that the observed population transfer can be understood as an effect of non adiabatic transitions occurring at the avoided crossings.