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arXiv:1305.1177 · New Journal of Physics

Interaction-induced chiral px ± ipy superfluid order of bosons in an optical lattice

Matthias Ölschläger, T. Kock, Georg Wirth, A Ewerbeck, C. Morais Smith, Andreas Hemmerich

Published Aug 22, 2013• 52 citations
arXivHTMLPDF

Abstract

The study of superconductivity with unconventional order is complicated in condensed matter systems by their extensive complexity. Optical lattices with their exceptional precision and control allow one to emulate superfluidity avoiding many of the complications of condensed matter. A promising approach to realize unconventional superfluid order is to employ orbital degrees of freedom in higher Bloch bands. In recent work, indications were found that bosons condensed in the second band of an optical chequerboard lattice might exhibit p x ± i p y order. Here we present experiments, which provide strong evidence for the emergence of p x ± i p y order driven by the interaction in the local p-orbitals. We compare our observations with a multi-band Hubbard model and find excellent quantitative agreement.

DOI
10.1088/1367-2630/15/8/083041

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The study of superconductivity with unconventional order is complicated in condensed matter systems by their extensive complexity. Optical lattices with their exceptional precision and control allow one to emulate superfluidity avoiding many of the complications of condensed matter. A promising approach to realize unconventional superfluid order is to employ orbital degrees of freedom in higher Bloch bands. In recent work, indications were found that bosons condensed in the second band of an optical chequerboard lattice might exhibit p x ± i p y order. Here we present experiments, which provide strong evidence for the emergence of p x ± i p y order driven by the interaction in the local p-orbitals. We compare our observations with a multi-band Hubbard model and find excellent quantitative agreement.
The breaking of time-reversal symmetry via the spontaneous formation of chiral order is ubiquitous in nature. Here, we present an unambiguous demonstration of this phenomenon for atoms Bose-Einstein condensed in the second Bloch band of an optical lattice. As a key tool, we use a matter-wave interference technique, which lets us directly observe the phase properties of the superfluid order parameter and allows us to reconstruct the spatial geometry of certain low-energy excitations, associated with the formation of domains of different chirality. Our work marks a new era of optical lattices where orbital degrees of freedom play an essential role for the formation of exotic quantum matter, similarly as in electronic systems.
Abstract Topological superfluidity is an important concept in electronic materials as well as ultracold atomic gases1. However, although progress has been made by hybridizing superconductors with topological substrates, the search for a material—natural or artificial—that intrinsically exhibits topological superfluidity has been ongoing since the discovery of the superfluid 3He-A phase2. Here we report evidence for a globally chiral atomic superfluid, induced by interaction-driven time-reversal symmetry breaking in the second Bloch band of an optical lattice with hexagonal boron nitride geometry. This realizes a long-lived Bose–Einstein condensate of 87Rb atoms beyond present limits to orbitally featureless scenarios in the lowest Bloch band. Time-of-flight and band mapping measurements reveal that the local phases and orbital rotations of atoms are spontaneously ordered into a vortex array, showing evidence of the emergence of global angular momentum across the entire lattice. A phenomenological effective model is used to capture the dynamics of Bogoliubov quasi-particle excitations above the ground state, which are shown to exhibit a topological band structure. The observed bosonic phase is expected to exhibit phenomena that are conceptually distinct from, but related to, the quantum anomalous Hall effect3–7 in electronic condensed matter.
Ultracold atoms loaded into higher Bloch bands provide an elegant setting for realizing many-body quantum states that spontaneously break time-reversal symmetry through the formation of chiral orbital order. The applicability of this strategy remains nonetheless limited due to the finite lifetime of atoms in high-energy bands. Here we introduce an alternative framework, suitable for bosonic gases, which builds on assembling square plaquettes pierced by a $\ensuremath{\pi}$ flux (half a magnetic-flux quantum). This setting is shown to be formally equivalent to an interacting bosonic gas loaded into ppp orbitals, and we explore the consequences of the resulting chiral orbital order, both for weak and strong on-site interactions. We demonstrate the emergence of a chiral superfluid vortex lattice, exhibiting a long-lived gapped collective mode that is characterized by local chiral currents. This chiral superfluid phase is shown to undergo a phase transition to a chiral Mott insulator for sufficiently strong interactions. Our work establishes coupled $\ensuremath{\pi}$-flux plaquettes as a practical route for the emergence of orbital order and chiral phases of matter.
We study a model of interacting bosons that occupy the first excited ppp-band states of a two-dimensional optical lattice. In contrast to the much studied single band Bose-Hubbard Hamiltonian, this more complex model allows for nontrivial superfluid phases associated with condensation at nonzero momentum and staggered order of the orbital angular momentum in addition to the superfluid-Mott insulator transition. More specifically, we observe staggered orbital angular momentum order in the Mott phase at commensurate filling and superfluidity at all densities. We also observe a transition between the staggered angular momentum superfluid phase and a striped superfluid, with an alternation of the phase of the superfluid along one direction. The transition between these two phases was observed in a recent experiment, which is then qualitatively well described by our model.
We study two models realized by two-component Fermi gases loaded in optical lattices. We clarify that multiband effects inevitably caused by the optical lattices generate a rich structure, when the systems crossover from the region of weakly bound molecular bosons to the region of strongly bound atomic bosons. Here the crossover can be controlled by attractive fermion interaction. One of the present models is a case with attractive fermion interaction, where an insulator-superfluid transition takes place. The transition is characterized as the transition between a band insulator and a Bose-Einstein condensate superfluid state. Differing from the conventional Bardeen-Cooper-Schrieffer (BCS) superfluid transition, this transition shows unconventional properties. In contrast to the one-particle excitation gap scaled by the superfluid order parameter in the conventional BCS transition, because of the multiband effects, a large gap of one-particle density of states is retained all through the transition, although the superfluid order grows continuously from zero. A re-entrant transition with lowering temperature is another unconventionality. The other model is the case with coexisting attractive and repulsive interactions. Within a mean-field treatment, we find a new insulating state, an orbital ordered insulator. This insulator is one candidate for the Mott insulator of molecular bosons and is the first example that the orbital internal degrees of freedom of molecular bosons appears explicitly. Besides the emergence of a new phase, a coexisting phase also appears where superfluidity and an orbital order coexist just by doping holes or particles. The insulating and superfluid particles show differentiation in momentum space as in the high-Tc{T}_{\text{c}}Tc​ cuprate superconductors.
Abstract This article provides a synopsis of our recent experimental work exploring Bose–Einstein condensation in metastable higher Bloch bands of optical lattices. Bipartite lattice geometries have allowed us to implement appropriate band structures, which meet three basic requirements: the existence of metastable excited states sufficiently protected from collisional band relaxation, a mechanism to excite the atoms initially prepared in the lowest band with moderate entropy increase, and the possibility of cross-dimensional tunneling dynamics, necessary to establish coherence along all lattice axes. A variety of bands can be selectively populated and a subsequent thermalization process leads to the formation of a condensate in the lowest energy state of the chosen band. As examples the 2nd, 4th and 7th bands in a bipartite square lattice are discussed. The geometry of the 2nd and 7th bands can be tuned such that two inequivalent energetically degenerate energy minima arise at the X ± -points at the edge of the 1st Brillouin zone. In this case even a small interaction energy is sufficient to lock the phase between the two condensation points such that a complex-valued chiral superfluid order parameter can emerge, which breaks time reversal symmetry. In the 4th band a condensate can be formed at the Γ-point in the center of the 1st Brillouin zone, which can be used to explore topologically protected band touching points. The new techniques to access orbital degrees of freedom in higher bands greatly extend the class of many-body scenarios that can be explored with bosons in optical lattices.