We control quantum fluctuations to create the ground state magnetic phases of a classical Ising model with a tunable longitudinal magnetic field using a system of 6 to 10 atomic ion spins. Because of the long-range Ising interactions, the various ground state spin configurations are separated by multiple first-order phase transitions, which in our zero temperature system cannot be driven by thermal fluctuations. We instead use a transverse magnetic field as a quantum catalyst to observe the first steps of the complete fractal devil's staircase, which emerges in the thermodynamic limit and can be mapped to a large number of many-body and energy-optimization problems.
We control quantum fluctuations to create the ground state magnetic phases of a classical Ising model with a tunable longitudinal magnetic field using a system of 6 to 10 atomic ion spins. Because of the long-range Ising interactions, the various ground state spin configurations are separated by multiple first-order phase transitions, which in our zero temperature system cannot be driven by thermal fluctuations. We instead use a transverse magnetic field as a quantum catalyst to observe the first steps of the complete fractal devil's staircase, which emerges in the thermodynamic limit and can be mapped to a large number of many-body and energy-optimization problems.
We perform a quantum simulation of the Ising model with a transverse field using a collection of three trapped atomic ion spins. By adiabatically manipulating the Hamiltonian, we directly probe the ground state for a wide range of fields and form of the Ising couplings, leading to a phase diagram of magnetic order in this microscopic system. The technique is scalable to much larger numbers of trapped ion spins, where phase transitions approaching the thermodynamic limit can be studied in cases where theory becomes intractable.
For a system at absolute zero temperature, all thermal fluctuations are frozen out, while quantum fluctuations prevail.These microscopic quantum fluctuations can induce a quantum phase transition (QPT) in the ground state of a many-body system when the relative strength of two competing energy terms is varied across a critical value.This paper presents a detailed and quantitative study of the magnetic properties of Ising two-spin system at zero temperature in the presence of longitudinal, transverse and mixed fields, and also at finite temperatures.At the critical longitudinal magnetic field, the system is found to undergo a QPT to a ferromagnetic state.For this system, an infinitesimal departure from zero transverse field is found to trigger off QPT and also remove the degeneracies that persisted even in the presence of longitudinal field.These quantum fluctuations, leading to QPT are more evident in the mixed field than the separate effect of longitudinal and transverse fields.The observed quantum effects at zero temperature for this system are found to be completely wiped out at finite temperatures due to thermal fluctuations.A temperature increase favours antiferromagnetic alignment of spins, while a decrease in temperature favours ferromagnetic alignment.
The Ising model in transverse magnetic field is perhaps the simplest quantum spin model, yet the elements of site disorder, random magnetic fields, and tunable quantum fluctuations permit a rich array of ground states, and the rare ability to emphasize their classical or quantum character. We briefly review in this chapter experimental results from chains to crystals of spins, with magnetic, glassy, and spin liquid ground states. Singlet Ground State Magnets In a crystalline lattice, the crystal fields often take a form such that the ground states of magnetic ions are singlets separated from the higher lying spin multiplets. Sufficiently strong magnetic dipolar or exchange couplings between different sites can mix the singlets with the multiplets enough so as to induce non-zero expectation values for the magnetic dipoles at individual sites. Examples of this phenomenon are generally found among metals and insulators based on rare earths. Such metals were a subject of extensive research in the 1960's and 1970's, and the book by MacKintosh and Jensen [408] gives an excellent account of both the data as well as mean field approaches. With respect to insulating materials, LiTbF 4 emerged as a model system in the 1970's. It is an example of an ideal Ising dipolar coupled ferromagnet; here the long-range nature of the dipolar interactions leads to an upper critical dimension [149] (at which mean field theory with logarithmic corrections calculable using RG methods becomes an exact description of thermal phase transitions) of three rather than four. LiTbF 4 belongs to the LiREF 4 isostructural series of ionic salts. Li and F carry valences +1 and −1 respectively, leaving RE, which can be any rare earth atom or the nonmagnetic element Y, with a valence of +3. Figure 14.1 shows the body-centered tetragonal crystal structure for the family.
The quantum Ising model is perhaps the simplest possible model of a quantum magnetic material. Despite its simplicity, its versatility and wide range of applications, from quantum computation, to combinatorial optimization, to biophysics, make it one of the most important models of modern physics. In this thesis, we develop a general framework for studying quantum Ising systems with an arbitrary single ion Hamiltonian, with emphasis on the effects of quantum fluctuations, and the quantum phase transition between paramagnetic and ferromagnetic states that occurs when a magnetic field is applied transverse to the easy axis of the system. The magnetic insulating crystal LiHoF₄ is a physical realization of the quantum Ising model, with the additional features that the dominant coupling between spins is the long range dipolar interaction, and each electronic spin is strongly coupled to a nuclear degree of freedom. These nuclear degrees of freedom constitute a spin bath environment acting on the system. In this thesis, we present an effective low temperature Hamiltonian for LiHoF₄ that incorporates both these features, and we analyze the effects of the nuclear spin bath on the system. We find the lowest energy crystal field excitation in the system is gapped at the quantum critical point by the presence of the nuclear spins, with spectral weight being transferred down to a lower energy electronuclear mode that fully softens to zero at the quantum critical point. Furthermore, we present a toy model, the spin half spin half model, that illustrates the effects of an anisotropic hyperfine interaction on a quantum Ising system. We find the critical transverse field is increased when the longitudinal hyperfine coupling is dominant, as well as an enhancement of both the longitudinal electronic susceptibility and an applied longitudinal field. In addition, we present a field theoretic formalism for incorporating the effects of fluctuations beyond the random phase approximation in general quantum Ising systems. We find that any regular on site interaction, such as a nuclear spin bath, does not fundamentally alter the critical properties of a quantum Ising system. This formalism is used to calculate corrections to the magnetization of LiHoF₄.
In a proof-of-principle experiment, we simulate the dynamics of a quantum spin system in an ion trap. Following a theoretical proposal by D. Porras and I. Cirac, we use a system of ground state cooled trapped ions to simulate and study the dynamics of a quantum-mechanical system, or more precisely, the dynamics of a quantum spin Hamiltonian. We implement the smallest non-trivial quantum spin Hamiltonian, the quantum Ising model for two spins. Each spin is represented by two hyperfine ground levels of trapped 25Mg+ ions. The interaction with an external magnetic field is simulated by coherently coupling these hyperfine levels via laser and radiofrequency radiation. The spin-spin interaction is simulated via optical dipole forces, where the effective interaction is mediated by the phonons of the linear ion chain. We demonstrate the adiabatic evolution from a paramagnetically ordered system to ferromagnetic order. The final state of this adiabatic transition is a superposition state of the two degenerate spin configurations of ferromagnetic order Psi_final = 1/sqrt(2) (|up up> + |down down>) with a quantum magnetisation of 98%. We also show the transition from paramagnetic to antiferromagnetic order with the final state Psi_final = 1/sqrt(2) (|up down> + |down up>). Moreover, we prove that this transition which is to become a quantum phase transition in the thermodynamic limit of infinitely many spins, is driven by quantum fluctuations which dominate the dynamics of such systems at the absolute zero-point of temperature rather than thermal fluctuations which are absent at 0 K. This is verified by the fact that the final state of our adiabatic evolution is entangled, close to a Bell state at a fidelity exceeding 88%. The set of tools presented in this thesis might serve as a basis for larger scale quantum simulations which might help in gaining insight into many-particle effects that are intractable on classical computers such as spin frustration in triangular lattices or high-Tc superconductivity.
A collection of trapped atomic ions represents one of the most attractive platforms for the quantum simulation of interacting spin networks and quantum magnetism. Spin-dependent optical dipole forces applied to an ion crystal create long-range eective spin-spin interactions and allow the simulation of spin Hamiltonians that possess nontrivial phases and dynamics. We trap linear chains of 171Yb+ ions in a Paul trap, and constrain the occupation of energy levels to the ground hyperne clock-states, creating a qubit or pseudo-spin 1/2 system. We proceed to implement spin-spin couplings between two ions using the far detuned Mlmer-Srenson scheme and perform adiabatic quantum simulations of Ising Hamiltonians with long-range couplings. We then demonstrate our ability to control the sign and relative strength of the interaction between three ions. Using this control, we simulate a frustrated triangular lattice, and for the first time establish an experimental connection between frustration and quantum entanglement. We then scale up our simulation to show phase transitions from paramagnetism to ferromagnetism for nine ions, and to anti-ferromagnetism for sixteen ions. The experimental work culminates with our most complicated Hamiltonian - a long range anti-ferromagnetic Ising interaction between 10 ions with a biasing axial field. Theoretical work presented in this thesis shows how the approach to quantum simulation utilized in this thesis can be further extended and improved. It is shown how appropriate design of laser elds can provide for arbitrary multidimensional spin-spin interaction graphs even for the case of a linear spatial array of ions. This scheme uses currently existing trap technology and is scalable to levels where classical methods of simulation are intractable.