We study the ground state of frustrated spin-
S chains in a strong magnetic field in the immediate vicinity of saturation. In strongly frustrated chains, the magnon dispersion has two degenerate minima at inequivalent momenta $\ifmmode\pm\else\textpm\fi{}Q$, and just below the saturation field the system can be effectively represented as a dilute one-dimensional lattice gas of two species of bosons that correspond to magnons with momenta around $\ifmmode\pm\else\textpm\fi{}Q$. We present a theory of effective interactions in such a dilute magnon gas that allows us to make quantitative predictions for arbitrary values of the spin. With the help of this method, we are able to establish the magnetic phase diagram of frustrated chains close to saturation and study phase transitions between several nontrivial states, including a two-component Luttinger liquid, a vector chiral phase, and phases with bound magnons. We study those phase transitions numerically and find a good agreement with our analytical predictions.
We study the ground-state phase diagram of a frustrated spin-1/2 four-leg tube. Using a variety of complementary techniques, namely, density matrix renormalization group, exact diagonalization, Schwinger boson mean-field theory, quantum Monte Carlo, and series expansion, we explore the parameter space of this model in the regime of all-antiferromagnetic exchange. In contrast to unfrustrated four-leg tubes, we uncover a rich phase diagram. Apart from the Luttinger liquid fixed point in the limit of decoupled legs, this comprises several gapped ground states, namely, a plaquette, an incommensurate, and an antiferromagnetic quasispin-2 chain phase. The transitions between these phases are analyzed in terms of total energy and static structure factor calculations and are found to be of (weak) first order. Despite the absence of long-range order in the quantum case, remarkable similarities to the classical phase diagram are uncovered, with the exception of the icommensurate regime, which is strongly renormalized by quantum fluctuations. In the limit of large leg exchange, the tube exhibits a deconfinement crossover from gapped magnon-like excitations to spinons.
We explore the ground-state phase diagram of the
S=1/2 two-leg ladder with different leg interactions. The
xy and
z components of the leg interactions between nearest-neighbor spins in the
a (
b) leg are respectively denoted by
Jl,a and
ΔlJl,a (
Jl,b and
ΔlJl,b). On the other hand, the
xy and
z components of the uniform rung interactions are respectively denoted by
ΓrJr and
Jr. In the above,
Δl and
Γr are the
XXZ-type anisotropy parameters for the leg and rung interactions, respectively. This system has a frustration when
Jl,aJl,b<0 irrespective of the sign of
Jr. The phase diagram on the
Δl (
∣Δl∣≤1.0) versus
Jl,b (
−2.0≤Jl,b≤3.0) plane in the case where
Jl,a=0.2,
Jr=−1.0, and
Γr=0.5 is determined numerically. We employ the physical consideration, and the level spectroscopy and phenomenological renormalization-group analyses of the numerical date obtained by the exact diagonalization method. The resultant phase diagram contains the ferromagnetic, Haldane, N{é}el, nematic Tomonaga-Luttinger liquid (TLL), partial ferrimagnetic, and
XY1 phases. Interestingly enough, the nematic TLL phase appears in the strong-rung unfrustrated region as well as in the strong-rung frustrated one. We perform the first-order perturbational calculations from the strong rung coupling limit to elucidate the characteristic features of the phase diagram. Furthermore, we make the density-matrix renormalization-group calculations for some physical quantities such as the energy gaps, the local magnetization, and the spin correlation functions to supplement the reliability of the phase diagram.
We derive and investigate the microscopic model of the quantum magnet
BiCu2PO6 using band-structure calculations, magnetic susceptibility and high-field magnetization measurements, as well as exact diagonalization (ED) and density-matrix renormalization group (DMRG) techniques. The resulting quasi-one-dimensional spin model is a two-leg antiferromagnetic ladder with frustrating next-nearest-neighbor couplings along the legs. The individual couplings are estimated from band-structure calculations and by fitting the magnetic susceptibility with theoretical predictions, obtained using full diagonalizations. The nearest-neighbor leg coupling
J1, the rung coupling
J4, and one of the next-nearest-neighbor couplings
J2 amount to 120--150 K while the second next-nearest-neighbor coupling is ${J}_{2}^{\ensuremath{'}}\ensuremath{\simeq}{J}_{2}/2$. The spin ladders do not match the structural chains, and although the next-nearest-neighbor interactions
J2 and ${J}_{2}^{\ensuremath{'}}$ have very similar superexchange pathways, they differ substantially in magnitude due to a tiny difference in the O-O distances and in the arrangement of nonmagnetic
PO4 tetrahedra. An extensive ED study of the proposed model provides the low-energy excitation spectrum and shows that the system is in the strong rung coupling regime. The strong frustration by the next-nearest-neighbor couplings leads to a triplon branch with an incommensurate minimum. This is further corroborated by a strong-coupling expansion up to second order in the inter-rung coupling. Based on high-field magnetization measurements, we estimate the spin gap of $\ensuremath{\Delta}\ensuremath{\simeq}32\text{ }\text{K}$ and suggest the likely presence of antisymmetric Dzyaloshinskii-Moriya anisotropy and interladder coupling
J3. We also provide a tentative description of the physics of
BiCu2PO6 in magnetic field, in the light of the low-energy excitation spectra and numerical calculations based on ED and DMRG. In particular, we raise the possibility for a rich interplay between one- and two-component Luttinger liquid phases and a magnetization plateau at 1/2 of the saturation value.
We study the ground state phase diagram of a frustrated spin-1/2 four-leg tube in an external magnetic field. We explore the parameter space of this model in the regime of all-antiferromagnetic exchange couplings by means of three different approaches: density matrix renormalization group (DMRG), a low-energy effective Hamiltonian (LEH) and a Hartree variational approach (HVA). We find that in the limit of weakly interacting plaquettes, singlet and triplet states play an important role in the formation of magnetization plateaux. We study the transition regions numerically and analytically, and find that they are described, at first order in a strong- coupling expansion, by an XXZ spin-1/2 chain in a magnetic field. These results are consistent with the DMRG and HVA calculations.
We study the ground state phase diagram of a frustrated spin-1/2 four-leg spin tube in an external magnetic field. We explore the parameter space of this model in the regime of all-antiferromagnetic exchange couplings by means of three different approaches: analysis of low-energy effective Hamiltonian, a Hartree variational approach, and density matrix renormalization group for finite clusters. We find that in the limit of weakly interacting plaquettes, low-energy singlet, triplet, and quintuplet states play an important role in the formation of fractional magnetization plateaus. We study the transition regions numerically and analytically, and find that they are described, at first order in a strong-coupling expansion, by an
XXZ spin-1/2 chain in a magnetic field; the second-order terms give corrections to the
XXZ model. All techniques provide consistent results which allow us to predict the existence of fractional plateaus in an important region in the space of parameters of the model.