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arXiv:1302.5908 · Physical Review B

Electron spin resonance in a dilute magnon gas as a probe of magnon scattering resonances

Yusuke Nishida

Published Dec 2, 2013• 6 citations
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Abstract

We study the electron spin resonance in a dilute magnon gas that is realized in a ferromagnetic spin system at low temperature. A quantum cluster expansion is developed to show that the frequency shift of the single-magnon peak changes its sign and the linewidth reaches its maximum across a scattering resonance between magnons. Such characteristic behaviors are universal and can be used to experimentally locate the two-magnon resonance when an external parameter such as pressure is varied. Future achievement of the two-magnon resonance may have an impact comparable to the Feshbach resonance in ultracold atoms and will open up a rich variety of strongly correlated physics such as the recently proposed Efimov effect in quantum magnets. We also suggest how the emergence of an Efimov state of three magnons and its binding energy may be observed with the electron spin resonance.

DOI
10.1103/physrevb.88.224402

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Feshbach resonances in cold atomic gases

E. G. M. van Kempen

The research described in this thesis is part of an international effort with the aim of studying ultracold quantum degenerate gas samples like Bose-Einstein condensates and Fermi degenerate systems, consisting of atoms confined in magnetic or optical traps. The behavior of such samples is governed by the inter-atomic interactions and the resulting properties of the atom-atom scattering. At the relevant temperatures of 1nK to 10µK a key property is the atom-atom scattering length a. In chapter 2 a theoretical method is presented which enables one to describe the interaction and scattering of (ultra)cold atoms to unprecedented precision. It is also unparalleled in comprehensiveness: it allows the prediction of a large and varied set of experimental data for all isotopes of the same element. The method relies on the extraction from experiments of a few (phase) parameters which completely summarize the behavior of the atoms in the (ultra)cold regime. In chapter 3 the method is applied to the "workhorses" of cold-atom physics: the atomic species 85Rb and 87Rb. We extract the foregoing parameters to a very high precision from several recent high precision experiments, allowing us to predict e.g. the 87Rb spinor condensate to be ferromagnetic: a prediction for which the scattering length has to be calculated with a precision better than 1%. We also predict Feshbach resonances at experimentally accessible magnetic field strengths; resonances searched for and found by the experimental group of Rempe. In close collaboration with his group we "fine-tune" the interaction parameters found previously, by making use of only one of the observed resonances. We then obtain agreement with 42 out of the observed 43 resonance field strengths and are able to identify bound states inducing the Feshbach resonances at these locations. Chapter 4 describes the results of this research. With a thorough understanding of the rubidium interactions, we then switch to lithium which has a fermionic (6Li) and a bosonic (7Li) isotope. Both are being used in cold-atom experiments. In chapter 5 we evaluate the interaction parameters for lithium allowing us to predict magnetic field strengths for which a sample of fermionic 6Li atoms can be regarded as strongly interacting. Furthermore, a three-level method for measuring mean-field shifts, based on radio-frequency techniques, is introduced. For weak interactions we find proportionality of resonance shifts to interaction strengths. In the strongly interacting regime, however, these shifts become very small reflecting the quantum unitarity limit and many-body effects. Most interesting is the fact that in this regime the shifts are small both for large positive a and for large negative a, likely reflecting the universality of the interaction energy. In chapters 6 and 7 the interactions between lithium atoms are reinvestigated, making use of newly available experimental data and with the updated interaction parameters special attention is paid to locating field strengths at which magnetically tunable Feshbach resonances occur in the scattering of lithium atoms. In chapter 6 scattering events in a gas of (fermionic) 6Li atoms are studied. In chapter 7 we show that a consistent description of the 6Li+6Li system can be given. We discuss theoretical uncertainties for the position of the wide 6Li Feshbach resonance and present an analytic scattering model for this resonance, based on the inclusion of a field-dependent virtual open-channel state. We predict new Feshbach resonances for the 6Li-7Li system, and their importance for different types of crossover superfluidity models is discussed. Molecules created by magnetically sweeping over these resonances will have a fermionic character. One magnetic field strength is predicted at which two different fermionic molecules can be created simultaneously.

•Jan 1, 2006•1 citation
We study the electron spin resonance in a dilute magnon gas that is realized in a ferromagnetic spin system at low temperature. A quantum cluster expansion is developed to show that the frequency shift of the single-magnon peak changes its sign and the linewidth reaches its maximum across a scattering resonance between magnons. Such characteristic behaviors are universal and can be used to experimentally locate the two-magnon resonance when an external parameter such as pressure is varied. Future achievement of the two-magnon resonance may have an impact comparable to the Feshbach resonance in ultracold atoms and will open up a rich variety of strongly correlated physics such as the recently proposed Efimov effect in quantum magnets. We also suggest how the emergence of an Efimov state of three magnons and its binding energy may be observed with the electron spin resonance.
Understanding how quasi-particles interact with impurities is crucial for unveiling novel properties of quantum many-body systems. A prominent example is the enhanced scattering between electrons and magnetic impurities in the low-energy limit, which gives rise to the Kondo effect. In this letter, motivated by recent developments in quantum simulation platforms, we investigate the universal behavior of long-range quantum spin chains with a single local impurity, focusing on systems that conserve the magnon number. Using effective field theory, we show that distinct classes of universal three-magnon states can emerge when the impurity-mediated two-magnon interaction is on resonance. When the long-range coupling decays as 1/rα1/r^α1/rα, we find that (i) for α∈(2,2.89)α\in (2,2.89)α∈(2,2.89), the system exhibits Efimov effects, with the three-body binding energy forming a geometric series ln⁡∣E3-body(n)∣∼−n(α−1)π/s0(α)\ln|E^{(n)}_{\text{3-body}}|\sim-n (α-1) π/s_0(α)ln∣E3-body(n)​∣∼−n(α−1)π/s0​(α), (ii) for α=2α=2α=2, the system shows semi-super Efimov effects with ln⁡∣E3-body(n)∣∼−(nπ−θ)2/8\ln|E^{(n)}_{\text{3-body}}|\sim-(nπ-θ)^2/8ln∣E3-body(n)​∣∼−(nπ−θ)2/8. Our theoretical prediction is validated by the numerical solution of the Skorniakov-Ter-Martirosian equation. Our results could be tested experimentally in the future on quantum simulation platforms.
Quantum few-body systems exhibit a rich variety of phenomena that provide fundamental insights into universality. A paradigmatic example is the Efimov effect, in which an infinite tower of three-body bound states emerges with binding energies forming a geometric sequence. Motivated by advances in trapped-ion systems, recent theoretical work has predicted that the Efimov effect can arise in certain long-range quantum spin chains, where magnons exhibit a general dispersion εk=u∣k∣zε_k=u|k|^zεk​=u∣k∣z with z∈(0.52,0.88)z\in(0.52,0.88)z∈(0.52,0.88) and interact through a contact potential. Nevertheless, whether Efimov universality persists in the presence of experimentally relevant long-range interactions between magnons remains unexplored. In this work, we address this issue by investigating the two- and three-magnon problems with a model interaction potential V(x)=V0/(1+∣x∣β)V(x)=V_0/(1+|x|^β)V(x)=V0​/(1+∣x∣β). Our results demonstrate that few-body universality persists for any β>1β>1β>1: In the two-magnon sector, the low-energy expansion of the scattering matrix near a two-body resonance agrees with the universal form predicted by contact-interaction theory. The three-magnon bound-state spectrum exhibits Efimov scaling, with a scaling factor consistent with the theory. We further highlight the experimental relevance of our model, which can be readily realized in trapped-ion systems. Our results pave the way for quantum simulations of universal few-body physics beyond the traditional paradigm of nonrelativistic particles.
Three interacting particles form a system which is well known for its complex physical behavior. A landmark theoretical result in few-body quantum physics is Efimov's prediction of a universal set of weakly bound trimer states appearing for three identical bosons with a resonant two-body interaction. Surprisingly, these states even exist in the absence of a corresponding two-body bound state and their precise nature is largely independent of the particular type of the two-body interaction potential. Efimov's scenario has attracted great interest in many areas of physics; an experimental test however has not been achieved. We report the observation of an Efimov resonance in an ultracold thermal gas of cesium atoms. The resonance occurs in the range of large negative two-body scattering lengths and arises from the coupling of three free atoms to an Efimov trimer. We observe its signature as a giant three-body recombination loss when the strength of the two-body interaction is varied near a Feshbach resonance. This resonance develops into a continuum resonance at non-zero collision energies, and we observe a shift of the resonance position as a function of temperature. We also report on a minimum in the recombination loss for positive scattering lengths, indicating destructive interference of decay pathways. Our results confirm central theoretical predictions of Efimov physics and represent a starting point from which to explore the universal properties of resonantly interacting few-body systems.
We have used a combination of neutron resonant spin-echo and triple-axis spectroscopies to determine the energy, fine structure, and linewidth of the magnon resonance in the model spin-1/2 ladder antiferromagnet IPA-CuCl(3) at temperatures T≪Δ(0)/k(B), where Δ(0) is the spin gap at T=0. In this low-temperature regime we find that the results deviate substantially from the predictions of the nonlinear sigma model proposed as a description of magnon excitations in one-dimensional quantum magnets and attribute these deviations to real-space and spin-space anisotropies in the spin Hamiltonian as well as scattering of magnon excitations from a dilute density of impurities. These effects are generic to experimental realizations of one-dimensional quantum magnets.
We report on the experimental observation of a strongly interacting gas of ultracold two-electron fermions with an orbital degree of freedom and magnetically tunable interactions. This realization has been enabled by the demonstration of a novel kind of Feshbach resonance occurring in the scattering of two (173)Yb atoms in different nuclear and electronic states. The strongly interacting regime at resonance is evidenced by the observation of anisotropic hydrodynamic expansion of the two-orbital Fermi gas. These results pave the way towards the realization of new quantum states of matter with strongly correlated fermions with an orbital degree of freedom.
The research described in this thesis is part of an international effort with the aim of studying ultracold quantum degenerate gas samples like Bose-Einstein condensates and Fermi degenerate systems, consisting of atoms confined in magnetic or optical traps. The behavior of such samples is governed by the inter-atomic interactions and the resulting properties of the atom-atom scattering. At the relevant temperatures of 1nK to 10µK a key property is the atom-atom scattering length a. In chapter 2 a theoretical method is presented which enables one to describe the interaction and scattering of (ultra)cold atoms to unprecedented precision. It is also unparalleled in comprehensiveness: it allows the prediction of a large and varied set of experimental data for all isotopes of the same element. The method relies on the extraction from experiments of a few (phase) parameters which completely summarize the behavior of the atoms in the (ultra)cold regime. In chapter 3 the method is applied to the "workhorses" of cold-atom physics: the atomic species 85Rb and 87Rb. We extract the foregoing parameters to a very high precision from several recent high precision experiments, allowing us to predict e.g. the 87Rb spinor condensate to be ferromagnetic: a prediction for which the scattering length has to be calculated with a precision better than 1%. We also predict Feshbach resonances at experimentally accessible magnetic field strengths; resonances searched for and found by the experimental group of Rempe. In close collaboration with his group we "fine-tune" the interaction parameters found previously, by making use of only one of the observed resonances. We then obtain agreement with 42 out of the observed 43 resonance field strengths and are able to identify bound states inducing the Feshbach resonances at these locations. Chapter 4 describes the results of this research. With a thorough understanding of the rubidium interactions, we then switch to lithium which has a fermionic (6Li) and a bosonic (7Li) isotope. Both are being used in cold-atom experiments. In chapter 5 we evaluate the interaction parameters for lithium allowing us to predict magnetic field strengths for which a sample of fermionic 6Li atoms can be regarded as strongly interacting. Furthermore, a three-level method for measuring mean-field shifts, based on radio-frequency techniques, is introduced. For weak interactions we find proportionality of resonance shifts to interaction strengths. In the strongly interacting regime, however, these shifts become very small reflecting the quantum unitarity limit and many-body effects. Most interesting is the fact that in this regime the shifts are small both for large positive a and for large negative a, likely reflecting the universality of the interaction energy. In chapters 6 and 7 the interactions between lithium atoms are reinvestigated, making use of newly available experimental data and with the updated interaction parameters special attention is paid to locating field strengths at which magnetically tunable Feshbach resonances occur in the scattering of lithium atoms. In chapter 6 scattering events in a gas of (fermionic) 6Li atoms are studied. In chapter 7 we show that a consistent description of the 6Li+6Li system can be given. We discuss theoretical uncertainties for the position of the wide 6Li Feshbach resonance and present an analytic scattering model for this resonance, based on the inclusion of a field-dependent virtual open-channel state. We predict new Feshbach resonances for the 6Li-7Li system, and their importance for different types of crossover superfluidity models is discussed. Molecules created by magnetically sweeping over these resonances will have a fermionic character. One magnetic field strength is predicted at which two different fermionic molecules can be created simultaneously.