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arXiv:1302.4891 · The Journal of Chemical Physics

Quantum critical point of spin-boson model and infrared catastrophe in bosonic bath

Hang Zheng, Zhiguo Lü

Published May 7, 2013• 15 citations
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Abstract

An analytic ground state is proposed for the unbiased spin-boson Hamiltonian, which is non-Gaussian and beyond the Silbey-Harris ground state with lower ground state energy. The infrared catastrophe in Ohmic and sub-Ohmic bosonic bath plays an important role in determining the degeneracy of the ground state. We show that the infrared divergence associated with the displacement of the nonadiabatic modes in bath may be removed from the proposed ground state for the coupling α < αc. Then αc is the quantum critical point of a transition from non-degenerate to degenerate ground state and our calculated αc agrees with previous numerical results.

DOI
10.1063/1.4803661

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An analytic ground state is proposed for the unbiased spin-boson Hamiltonian, which is non-Gaussian and beyond the Silbey-Harris ground state with lower ground state energy. The infrared catastrophe in Ohmic and sub-Ohmic bosonic bath plays an important role in determining the degeneracy of the ground state. We show that the infrared divergence associated with the displacement of the nonadiabatic modes in bath may be removed from the proposed ground state for the coupling α < αc. Then αc is the quantum critical point of a transition from non-degenerate to degenerate ground state and our calculated αc agrees with previous numerical results.
The spin-boson model is analytically studied using displaced Fock states (DFS) without discretization of the continuum bath. In the orthogonal displaced Fock basis, the ground-state wavefunction can be systematically improved in a controllable way. Interestingly, the zeroth-order DFS reproduces exactly the well known Silbey-Harris results. In the framework of the second-order DFS, the magnetization and the entanglement entropy are exactly calculated. It is found that the magnetic critical exponent βββ is converged to 0.50.50.5 in the whole sub-Ohmic bath regime $0
We explore the spin-boson model in a special case, i.e., with zero local field. In contrast to previous studies, we find no possibility for quantum phase transition (QPT) happening between the localized and delocalized phases, and the behavior of the model can be fully characterized by the even or odd parity as well as the parity breaking, instead of the QPT, owned by the ground state of the system. The parity breaking mentioned in our case is completely different from the spontaneously broken symmetry relevant to the conventionally defined QPT in previous studies. Our analytical treatment about the eigensolution of the ground state of the model presents for the first time a rigorous proof of no-degeneracy for the ground state of the model, which is independent of the bath type, the degrees of freedom of the bath and the calculation precision. We argue that the QPT mentioned previously appears due to incorrect employment of the ground state of the model and/or unreasonable treatment of the infrared divergence existing in the spectral functions for Ohmic and sub-Ohmic dissipations.
By means of a unitary transformation, we study quantum phase transitions in the ground state of a two-qubit system interacting with a dissipative reservoir. First, the ground state phase diagram is analyzed in the presence of the Ohmic and sub-Ohmic bath using an analytic ground state wave function which takes into account the competition between intrasite tunneling and intersite correlation. The quantum critical point is determined as the transition point from non-degenerate to degenerate ground state and our calculated critical coupling strength αc\alpha_cαc​ agrees with that from the numerical renormalization group method. Moreover, by computing the entanglement entropy between the qubits and the bath in the ground state, we explore the nature of the quantum phase transition between the delocalized and localized states.
Unitary transformation with a double polaronic generator is proposed for the unbiased spin-boson Hamiltonian, which leads to a new ground state with lower ground state energy, as well as an effective Hamiltonian without the counter-rotating coupling. The infrared divergence associated with the nonadiabatic modes in Ohmic bath plays an important role in determining the quantum critical point αc of the ground state, which separates the non-degenerate ground state for α<αc from the degenerate one for α>αc and leads to logarithmic divergence of the bosonic numbers. The thermodynamic properties, the dynamical evolution, and time correlation of the SBM model are studied by the effective Hamiltonian obtained from the unitary transformation, which can be solved easily and transparently by the perturbation theory. As a check of our theoretical treatment and numerical results, we have calculated the Wilson ratio and shown that the spectral sum rule and Shiba's relation are exactly fulfilled.
The influence of dissipation on quantum tunneling in the spin-boson model with a sub-Ohmic bath is studied by a variational calculation. By examining the evolution of solutions of the variational equation with the coupling strength near the phase boundary, we are able to present a scenario of discontinuous transition in sub-Ohmic dissipation case in accord with Ginzburg-Landau theory. Based on the constructed picture, it is shown that the critical point found in the general way is not thermodynamically the critical point, but the point where the second energy minimum begins to develop. The true cross-over point is calculated and the obtained phase diagram is in agreement with the result of numerical renormalization group calculation.
The sub-Ohmic spin-boson model possesses a quantum phase transition at zero temperature between a localized and a delocalized phase, whose properties have so far only been extracted by numerical approaches. Here we present an extension of the Silbey-Harris variational polaron ansatz which allows us to develop an analytical theory which correctly describes a continuous transition with mean-field exponents for 0<s<0.5. The critical properties, couplings, and observables we obtain show excellent agreement with existing numerical results, and we give an intuitive microscopic description of the changing correlations between the system and bath which suppress the spin coherence and drive the transition.