Quantum spin liquids (QSLs) are phases of interacting spins that do not order even at the absolute zero temperature, making it impossible to characterize them by a local order parameter. In this paper, we review the unique view provided by the quantum entanglement on QSLs. We illustrate the crucial role of topological entanglement entropy in diagnosing the non-local order in QSLs, using specific examples such as the chiral spin liquid. We also demonstrate the detection of anyonic quasi-particles and their braiding statistics using quantum entanglement. In the context of gapless QSLs, we discuss the detection of emergent fermionic spinons in a bosonic wavefunction, by studying the size dependence of entanglement entropy.
Quantum spin liquids (QSLs) are phases of interacting spins that do not order even at the absolute zero temperature, making it impossible to characterize them by a local order parameter. In this paper, we review the unique view provided by the quantum entanglement on QSLs. We illustrate the crucial role of topological entanglement entropy in diagnosing the non-local order in QSLs, using specific examples such as the chiral spin liquid. We also demonstrate the detection of anyonic quasi-particles and their braiding statistics using quantum entanglement. In the context of gapless QSLs, we discuss the detection of emergent fermionic spinons in a bosonic wavefunction, by studying the size dependence of entanglement entropy.
Quantum spin liquids (QSLs) are exotic phases of matter that host fractionalized excitations. It is difficult for local probes to characterize QSL, whereas quantum entanglement can serve as a powerful diagnostic tool due to its nonlocality. The kagome antiferromagnetic Heisenberg model is one of the most studied and experimentally relevant models for QSL, but its solution remains under debate. Here, we perform a numerical Aharonov-Bohm experiment on this model and uncover universal features of the entanglement entropy. By means of the density matrix renormalization group, we reveal the entanglement signatures of emergent Dirac spinons, which are the fractionalized excitations of the QSL. This scheme provides qualitative insights into the nature of kagome QSL and can be used to study other quantum states of matter. As a concrete example, we also benchmark our methods on an interacting quantum critical point between a Dirac semimetal and a charge-ordered phase.
Abstract Quantum spin liquids (QSLs) give rise to exotic emergent particles by weaving intricate entanglement patterns in the underlying electrons. Bipartite measures between subregions can detect the presence of anyons, but little is known about the full entanglement structure of QSLs. Here, we study the multiparty entanglement of QSLs via entanglement microscopy. We find that in contrast to conventional matter, the genuine multiparty entanglement (GME) between spins is absent in the smallest subregions, a phenomenon we call ``entanglement frustration.'' Instead, GME is more collective, and arises solely in loops. By exploiting exact results and large-scale numerics, we confirm these properties in various gapped and gapless QSLs realized in physically motivated Hamiltonians, as well as with string-net wavefunctions hosting abelian or non-abelian anyons. Our results shed new light on the phase diagram of Kitaev’s honeycomb model in a Zeeman field, and the Kagome Heisenberg model under various perturbations. Going beyond QSLs, we provide evidence that entanglement loops are a universal property of quantum gauge theories. This leads to a new understanding of fractionalization, and the means by which gauge bosons encode quantum information.
Entanglement entropy is a powerful tool for characterizing spin liquids and other systems with long-range entanglement. For gapped spin liquids, this problem has been well-studied, finding a universal subleading constant term in the entanglement entropy, known as the topological entanglement entropy. In this paper, the idea of topological entanglement entropy is generalized to the gapless U(1) spin liquid. First, it is shown that the entanglement entropy separates into two pieces, one due to emergent charges of the theory (assumed to be gapped) and one due to the emergent gapless gauge mode. Both give universal subheading contributions to the entanglement entropy, which are logarithmic in the size of the region considered. The photon contribution is due to the local physics of the gapless mode. The particle contribution, on the other hand, is a topological term, generalizing the notion of topological entanglement entropy. A construction is presented which can isolate this topological piece by eliminating the photon contribution and other local terms, such as the area law. This topological term in the entanglement entropy can serve as a powerful diagnostic tool for U(1) spin liquids.
The search for exotic states of matter continues to be a central theme in condensed matter physics. Among these, quantum spin liquids (QSLs) represent a profound challenge and opportunity, characterized by long-range entanglement and fractionalized excitations without conventional magnetic order even at absolute zero temperature. Frustrated quantum magnets are prime candidates for hosting such states, where competing interactions prevent classical ground states. This paper reports the theoretical and experimental signatures that would lead to the discovery of a chiral bosonic liquid (CBL) in a novel frustrated quantum magnet. A CBL is a particularly elusive type of QSL characterized by elementary excitations that behave as bosons and exhibit a distinct chirality, manifesting as a non-zero thermal Hall effect in the absence of a magnetic field. We outline a comprehensive strategy involving advanced material synthesis, precise low-temperature thermodynamic measurements, inelastic neutron scattering, and numerical simulations to identify the unique fingerprints of this novel state. Key indicators include a gapless or nearly gapless excitation spectrum, a specific heat scaling characteristic of bosonic excitations, and, most critically, a quantized or near-quantized thermal Hall conductivity directly reflecting the chiral nature of the bosonic fractional excitations. The implications of this discovery extend to fundamental understanding of quantum entanglement, topological states of matter, and potential applications in robust quantum information processing.
Abstract We use the topological entanglement entropy (TEE) as an efficient tool to fully characterize the Abelian phase of a Z 2 × Z 2 spin liquid emerging as the ground state of topological color code (TCC), which is a class of stabilizer states on the honeycomb lattice. We provide the fusion rules of the quasiparticle (QP) excitations of the model by introducing single- or two-body operators on physical spins for each fusion process which justify the corresponding fusion outcome. Besides this, we extract the TEE from Renyi entanglement entropy (EE) of the TCC, analytically and numerically by finite size exact diagonalization on the disk shape regions with contractible boundaries. We obtain that the EE has a local contribution, which scales linearly with the boundary length in addition to a topological term, i.e. the TEE, arising from the condensation of closed strings in the ground state. We further investigate the ground state dependence of the TEE on regions with non-contractible boundaries, i.e. by cutting the torus to half cylinders, from which we further identify multiple independent minimum entropy states (MES) of the TCC and then extract the U and S modular matrices of the system, which contain the self and mutual statistics of the anyonic QPs and fully characterize the topological phase of the TCC. Eventually, we show that, in spite of the lack of a local order parameter, TEE and other physical quantities obtained from the ground state wave function such as the entanglement spectrum (ES) and ground state fidelity are sensitive probes to study the robustness of a topological phase. We find that the topological order in the presence of a magnetic field persists until the vicinity of the transition point, where the TEE and fidelity drops to zero and the ES splits severely, signaling breakdown of the topological phase of the TCC.
The main question we address is how to probe the fractionalized excitations of a quantum spin liquid (QSL), for example, in the Kitaev honeycomb model. By analyzing the energy spectrum and entanglement entropy, for antiferromagnetic couplings and a field along either [111] or [001], we find a gapless QSL phase sandwiched between the non-Abelian Kitaev QSL and polarized phases. Increasing the field strength towards the polarized limit destroys this intermediate QSL phase, resulting in a considerable reduction in the number of frequency modes and the emergence of a beating pattern in the local dynamical correlations, possibly observable in pump-probe experiments.