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arXiv:1301.6036 · Physical Review B

Itinerant ferromagnetism with finite-ranged interactions

Curt W. von Keyserlingk, G. J. Conduit

Published May 20, 2013• 15 citations
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Abstract

Quantum fluctuations are of central importance in itinerant ferromagnets; when modeled by a homogeneous electron gas with contact interactions, fluctuations deliver a rich phase diagram featuring a first order ferromagnetic transition preempted by a spin spiral and a paired density wave. In this work we develop the formalism to analyze the effects of fluctuations with a realistic screened Coulomb potential. The finite-ranged interaction suppresses the tricritical point temperature of the first order ferromagnetic transition, bringing theory into line with experiment, while retaining the exotic spin spiral and paired density wave. In an ultracold atomic gas a finite-ranged interaction damps the competing molecular instability, permitting the observation of ferromagnetic correlations.

DOI
10.1103/physrevb.87.184424

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Quantum fluctuations are of central importance in itinerant ferromagnets; when modeled by a homogeneous electron gas with contact interactions, fluctuations deliver a rich phase diagram featuring a first order ferromagnetic transition preempted by a spin spiral and a paired density wave. In this work we develop the formalism to analyze the effects of fluctuations with a realistic screened Coulomb potential. The finite-ranged interaction suppresses the tricritical point temperature of the first order ferromagnetic transition, bringing theory into line with experiment, while retaining the exotic spin spiral and paired density wave. In an ultracold atomic gas a finite-ranged interaction damps the competing molecular instability, permitting the observation of ferromagnetic correlations.
In the 1930s, two main paradigms for the theoretical description of ferromagnetism were developed: Heisenberg ferromagnetism of localized fermions (e.g., in a lattice), and Bloch or Stoner ferromagnetism of nonlocalized fermions (i.e., in a gas), also called itinerant ferromagnetism. Despite many theoretical predictions, itinerant ferromagnetism has remained elusive in experiments. This ferromagnetic state is predicted to occur for strong repulsive interactions, corresponding to a regime that is very challenging to describe theoretically because there are multiple competing physical effects, including superfluid pairing. In this paper, we point out that the problem of itinerant ferromagnetism for atomic Fermi gases is different from that of electron gases in metals due to the short-range nature of the interatomic interactions. We also show that the standard saddle point used to describe itinerant ferromagnetism of the electron gas in metals does not apply, because in the short-range limit of this approximation the Pauli exclusion principle is violated. As a remedy, we introduce a modified interaction pseudopotential for ultracold gases which includes both local (Hartree) and nonlocal (Fock) terms while preserving the Pauli exclusion principle in the short-range regime. Furthermore, we demonstrate the usefulness of this method to study the existence and stability of itinerant ferromagnetism in ultracold atomic gases. Lastly, we obtain the critical temperature for the ferromagnetic transition as a function of the opposite-spin interaction strength and find a rather good agreement with recent experimental results.
Abstract At temperatures well below the Fermi temperature T F , the coupling of magnetic fluctuations to particle-hole excitations in a two-component Fermi gas leads to non-analytic corrections in the renormalized free energy and makes the transition to itinerant ferromagnetism first order. On the other hand, despite that larger symmetry often introduces larger degeneracies in the low-lying states, here we show that for a Fermi gas with SU(N > 2)-symmetry in three space dimensions the ferromagnetic phase transition is first order in agreement with the predictions of Landau’s mean-field theory in its minimal formulation, which contains a cubic term in the free-energy (Cazalilla et al 2009 New J. Phys. 11 103033). By performing unrestricted Hartree–Fock calculations for an SU(N > 2)-symmetric Fermi gas with short range interactions, we find the order parameter undergoes a finite jump across the transition. In addition, for SU(N > 2) we do not observe any tri-critical point up to temperatures T ≃ 0.5 T F , for which the thermal smearing of the Fermi surface and thermal fluctuations are substantial. Going beyond mean-field theory, we find that the coupling of magnetic fluctuations to particle-hole excitations makes the transition more abrupt and further enhances the tendency of the gas to become fully polarized for smaller values of N and the gas parameter k F a s . In our study, we also clarify the role of time reversal symmetry in the microscopic Hamiltonian and obtain the temperature dependence of Tan’s contact. For the latter, the presence of the tri-critical point for N = 2 leads to a more pronounced temperature dependence around the transition than for SU(N > 2)-symmetric gases. Although the results are obtained for a microscopic model relevant to ultracold atomic gases, they may also apply to models of solid state systems with SU(N > 2) symmetry provided Coulomb interactions are sufficiently well screened.
We study finite-temperature properties of a Hubbard model including sites of a particle bath, which was proposed as a microscopic model to show itinerant ferromagnetism at finite electron density. We use direct numerical methods, such as exact diagonalization and random vector methods. The temperature dependence of quantities is surveyed in the full range of the temperature. We find that the specific heat has several peaks, which correspond to ordering processes in different energy scales. In particular, magnetic correlations develop at very low temperature. The system exhibits an itinerant ferromagnetic state or an antiferromagnetic state of the Mott insulator depending on the chemical potential of the particle bath and the Coulomb interaction. From a microscopic viewpoint, the competition between these two types of magnetic states causes a peculiar ordering process of local spin correlations. Some local ferromagnetic correlations are found to be robust, which indicates that the ferromagnetic correlation originates from the motion of itinerant electrons in a short-range cluster.
Itinerant ferromagnetism is one of the most-studied quantum phase transitions, the transition point and the nature of this phase transition being widely discussed. In dilute Fermi liquids, this analysis has been carried out up to second order in the gas parameter, where the results for any spin degeneracy are universal in terms of only the s -wave scattering length a 0 . We extend this analysis to third order, where energies depend not only on a 0 , but also on the s -wave effective range r 0 and the p -wave scattering length a 1 . The introduction in the theory of these new parameters changes the transition point, with respect to the second-order estimation, and also can modify the nature of the phase transition itself. We analyze these interaction effects on the phase transition for different spin values. The emerging phase diagram shows that the type of ferromagnetic transition changes dramatically as a function of r 0 and a 1 and, importantly, that this classification is not solely determined by the spin value, as happens at second order.
Itinerant ferromagnetism in cold Fermi gases with repulsive interactions is studied applying the Jastrow-Slater approximation generalized to finite polarization and temperature. For two components at zero temperature, a second-order transition is found at ${\mathit{ak}}_{F}\ensuremath{\simeq}0.90$ compatible with results of quantum-Monte-Carlo (QMC) calculations. Thermodynamic functions and observables, such as the compressibility and spin susceptibility and the resulting fluctuations in number and spin, are calculated. For trapped gases, the resulting cloud radii and kinetic energies are calculated and compared to recent experiments. Spin-polarized systems are recommended for effective separation of large ferromagnetic domains. Collective modes are predicted and tricritical points are calculated for multicomponent systems.
A recent experiment has provided tentative evidence for itinerant ferromagnetism in an ultracold atomic gas. However, the interpretation of the results is complicated by significant atom losses. We argue that during the loss process the system gradually heats up but remains in local equilibrium.To quantify the consequences of atom loss on the putative ferromagnetic transition we adopt an extended Hertz-Millis theory. The losses damp quantum fluctuations, thus increasing the critical interaction strength needed to induce ferromagnetism and revert the transition from being first order to second order. This effect may resolve a discrepancy between the experiment and previous theoretical predictions. We further illuminate the impact of loss by studying the collective spin excitations in the ferromagnet. Even in the fully polarized state, where loss is completely suppressed, spin waves acquire a decay rate proportional to the three-body loss coefficient.