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arXiv:1301.0230 · Physical Review B

Probe spectroscopy of quasienergy states

Matti Silveri, Jani Tuorila, Mika Kemppainen, E. V. Thuneberg

Published Apr 8, 2013• 30 citations
arXivHTMLPDF

Abstract

The present qubit technology, in particular, in Josephson qubits, allows an unprecedented control of discrete energy levels. This motivates a new study of the old pump-probe problem, where a discrete quantum system is driven by a strong drive and simultaneously probed by a weaker one. The strong drive is included by the Floquet method and the resulting quasienergy states are then studied with the probe. We study a qubit where the harmonic drive has a significant longitudinal component relative to the static equilibrium state of the qubit. Both analytical and numerical methods are used to solve the problem. We present calculations with realistic parameters and compare the results with recent experimental results. A short introduction to the Floquet method and the probe absorption is given.

DOI
10.1103/physrevb.87.134505

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The present qubit technology, in particular, in Josephson qubits, allows an unprecedented control of discrete energy levels. This motivates a new study of the old pump-probe problem, where a discrete quantum system is driven by a strong drive and simultaneously probed by a weaker one. The strong drive is included by the Floquet method and the resulting quasienergy states are then studied with the probe. We study a qubit where the harmonic drive has a significant longitudinal component relative to the static equilibrium state of the qubit. Both analytical and numerical methods are used to solve the problem. We present calculations with realistic parameters and compare the results with recent experimental results. A short introduction to the Floquet method and the probe absorption is given.
The device for the Josephson flux qubit can be considered as a solid-state artificial atom with multiple energy levels. When a large-amplitude harmonic excitation is applied to the system, transitions at the energy levels avoided crossings produce visible changes in the qubit population over many driven periods that are accompanied by a rich pattern of interference phenomena. We present a Floquet treatment of the periodically time-dependent Schr\"odinger equation of the strongly driven qubit beyond the standard two-level approach. For low amplitudes, the average probability of a given sign of the persistent current qubit exhibits, as a function of the static flux detuning and the driving amplitude, Landau-Zener-St\"uckelberg (LZS) interference patterns that evolve into complex diamondlike patterns for large amplitudes. In the case of highly coherent flux qubits we show that the higher-order diamonds can not be simply described relying on LZS transitions in each avoided crossing considered separately. In addition we propose a spectroscopic method based on starting the system in the first excited state instead of in the ground state, which can give further information on the energy-level spectrum and dynamics in the case of highly coherent flux qubits. We compare our numerical results with recent experiments that perform amplitude spectroscopy to probe the energy spectrum of the artificial atom.
We consider the dynamics of a two-level system (qubit) driven by strong and short resonant pulses in the framework of Floquet theory. First we derive analytical expressions for the quasienergies and Floquet states of the driven system. If the pulse amplitude varies very slowly, the system adiabatically follows the instantaneous Floquet states, which acquire dynamical phases that depend on the evolution of the quasienergies over time. The difference between the phases acquired by the two Floquet states corresponds to a qubit state rotation, generalizing the notion of Rabi oscillations to the case of large driving amplitudes. If the pulse amplitude changes very fast, the evolution is nonadiabatic, with transitions taking place between the Floquet states. We quantify and analyze the nonadiabatic transitions during the pulse by employing adiabatic perturbation theory and exact numerical simulations. We find that, for certain combinations of pulse rise and fall times and maximum driving amplitude, a destructive interference effect leads to a remarkably strong suppression of transitions between the Floquet states. This effect provides the basis of a quantum control protocol, which we name Floquet interference efficient suppression of transitions in the adiabatic basis (FIESTA), that can be used to design ultrafast high-fidelity single-qubit quantum gates.
Strong periodic driving of cavity-quantum electrodynamics (QED) in the ultrastrong-coupling regime creates nonequilibrium states whose dissipation is governed by Floquet quasienergies rather than undriven dressed resonances. However, modeling such a regime is a significant theoretical challenge, including a number of subtle problems such as the need to ensure gauge invariance for truncated matter-cavity systems with time-dependent driving. To fill this theoretical gap, we introduce a nonsecular Floquet generalized master equation framework for strongly driven open cavity-QED systems, formulated in the dressed basis of the quantum Rabi model and applicable to structured reservoirs without rotating-wave approximations. Our theory can thus model Floquet-driven dynamics in open ultrastrong-coupling cavity-QED, and demonstrates a wide range of quantum state control. Using strong optical pumping and parametric mechanical modulation, we compute long-time populations, fluorescence spectra, and the Floquet-Liouville eigenspectra, resolving observable resonances into hybridized quasienergy channels and decay rates. By systematically comparing with conventional time-independent dressed-basis generalized master equations, we show that static approaches only reproduce steady-state populations in restricted excitation regimes, and fail for frequency-resolved observables and break down under appropriate Floquet engineering, surprisingly, even for spectrally flat baths. Structured environments, such as Lorentzian-Ohmic reservoirs, further amplify these discrepancies through sideband-selective decay. Our results demonstrate that dissipation in driven ultrastrong cavity-QED is intrinsically quasienergy resolved and we establish Floquet-dissipative theory as an accurate and powerful framework for predicting spectra, controlling decay pathways, and engineering nonequilibrium quantum states and reservoirs.
We present experiments on the driven dynamics of a two-level superconducting artificial atom. The driving strength reaches 4.78 GHz, significantly exceeding the transition frequency of 2.288 GHz. The observed dynamics is described in terms of quasienergies and quasienergy states, in agreement with Floquet theory. In addition, we observe the role of pulse shaping in the dynamics, as determined by nonadiabatic transitions between Floquet states, and we implement subnanosecond single-qubit operations. These results pave the way to quantum control using strong driving with applications in quantum technologies.
A superconducting qubit was driven in an ultrastrong fashion by an oscillatory microwave field, which was created by coupling via the nonlinear Josephson energy. The observed Stark shifts of the "atomic" levels are so pronounced that corrections even beyond the lowest-order Bloch-Siegert shift are needed to properly explain the measurements. The quasienergies of the dressed two-level system were probed by resonant absorption via a cavity, and the results are in agreement with a calculation based on the Floquet approach.