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arXiv:1212.6291 · Science

A Quantum Many-Body Spin System in an Optical Lattice Clock

Michael J. Martin, Michael Bishof, Matthew D. Swallows, Xiaogang Zhang, Craig Benko, Javier von Stecher, Alexey Vyacheslavovich Gorshkov, Ana María Rey, Jun Ye

Published Aug 8, 2013• 194 citations
arXivHTMLPDF

Abstract

Strongly interacting quantum many-body systems arise in many areas of physics, but their complexity generally precludes exact solutions to their dynamics. We explored a strongly interacting two-level system formed by the clock states in (87)Sr as a laboratory for the study of quantum many-body effects. Our collective spin measurements reveal signatures of the development of many-body correlations during the dynamical evolution. We derived a many-body Hamiltonian that describes the experimental observation of atomic spin coherence decay, density-dependent frequency shifts, severely distorted lineshapes, and correlated spin noise. These investigations open the door to further explorations of quantum many-body effects and entanglement through use of highly coherent and precisely controlled optical lattice clocks.

DOI
10.1126/science.1236929

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Strongly interacting quantum many-body systems arise in many areas of physics, but their complexity generally precludes exact solutions to their dynamics. We explored a strongly interacting two-level system formed by the clock states in (87)Sr as a laboratory for the study of quantum many-body effects. Our collective spin measurements reveal signatures of the development of many-body correlations during the dynamical evolution. We derived a many-body Hamiltonian that describes the experimental observation of atomic spin coherence decay, density-dependent frequency shifts, severely distorted lineshapes, and correlated spin noise. These investigations open the door to further explorations of quantum many-body effects and entanglement through use of highly coherent and precisely controlled optical lattice clocks.
Strontium optical lattice clocks at JILA recently demonstrated record-high accuracy and stability. These advances were enabled by an ultrastable laser with fractional frequency stability of 1x10-16 at 1 second. This laser allows us to study systematic shifts of the 1S0 to 3P0 clock transition with unprecedented precision. Density-dependent frequency shifts represent an unavoidable perturbation for clocks based on many atoms. Our studies of atomic interactions in an optical lattice clock system uncover the nature of these interactions and reveal important many-body atomic correlation effects in this open quantum system. By extending our measurements to all ten nuclear-spin sublevels of the clock states, we observe the first direct evidence of SU(N) symmetric interactions in alkaline earth(-like) atoms. Using the techniques we developed in these studies, we also demonstrate a novel technique for measuring the frequency noise spectrum of an ultrastable laser. We discuss designs for the future direction of our experiment which will place 87Sr atoms within a high finesse cavity that is resonant on the 1S0 to 3P1 transition. We will use this system to study collective effects in cavity quantum electrodynamics. Most notably, strong atom-cavity coupling can enhance the spectroscopic sensitivity of our clock by creating spin-squeezed states via quantum non-demolition measurements. As a precursor to future work studying cavity-mediated collective behavior, we use the unique atomic structure of 88Sr to investigate free-space retarded dipolar coupling in an optically thick sample of atoms.
Advances in ultra-stable lasers now permit sub-Hz resolution of optical atomic transitions. At this level, weak interactions by any ordinary scale can in fact dominate the dynamics of the interrogated atoms, even for spin polarized fermions at ultralow temperatures. Contrary to results obtained in radio frequency spectroscopy of alkali fermionic atoms, optical spectroscopy of 87 Sr and 171 Yb has revealed density dependent frequency shifts of the 1 S0 - 3 P 0 “clock” transition. Understanding interactions in these systems is necessary to improve their accuracy and stability. Moreover, such an understanding will enable optical lattice clock systems to serve as quantum simulators for open, driven, strongly-interacting quantum systems at the mesoscopic scale. In this talk we presented our progress towards a comprehensive evaluation and understanding of the interactions present during spectroscopy of the 87 Sr clock transition under various operating conditions. Our studies indicate that a mean-field solution of a master equation is sufficient to capture the many-body dynamics of alkaline earth atom clocks. Entering the regime in which a treatment beyond mean-field is required for a proper description of the clock dynamics is under immediate experimental reach.
We report precise measurements of inter-level interactions in a bosonic optical lattice clock based on 88^{88}88Sr atoms. We observe a nonlinear density dependence of the clock shift, even without reaching quantum degeneracy. In a 2D lattice, the Rabi line shape exhibits an interaction sideband consistent with a collective spin model, while in a 1D lattice the shift is modified by density-induced dephasing. These findings, combined with a careful choice of interrogation detuning and atomic density, can enable operation at a net-zero systematic density shift in 88^{88}88Sr lattice clocks. We discuss the implications of these findings in many-body physics, quantum simulation, and precision isotope shift measurements, which provide a powerful probe for new physics beyond the Standard Model.
Neutral atom optical standards require the highest levels of laser precision to operate near the limit set by quantum fluctuations. We develop state-of-the-art ultra-stable laser systems to achieve a factor of 10 enhancement in clock measurement precision and additionally demonstrate optical linewidths below 50 mHz. The most stable of these lasers reaches its thermal noise floor of 1 × 10-16 fractional frequency instability, allowing the attainment of near quantum-noise-limited clock operation with single-clock instabilities of 3×10-16 at 1 s. We utilize this high level of spectral resolution to operate a 87Sr optical lattice clock in a regime in which quantum collisions play a dominant role in the dynamics, enabling the study of quantum many-body physics. With a fractional level of precision of near 1 × 10-16 at 1 s, we clearly resolve the signatures of many-body interactions. We find that the complicated interplay between the p wave-dominated elastic and inelastic interaction processes between lattice-trapped atoms leads to severe lineshape distortion, shifts, and loss of Ramsey fringe contrast. We additionally explore the theoretical prediction that these many-body interactions will modify the quantum fluctuations of the system and we find that in certain parameter regimes the quantum noise distribution exhibits a quadrature dependence. We further present technological advancements that will permit ultra-stable lasers to operate with reduced thermal noise, leading to a potential gain of an additional factor of 10 in stability. This indicates that laser fractional frequency instabilities of 1 × 10-17 are within experimental reach, as is a fully-quantum-limited regime of optical clock operation.
In this work we study the effect of interactions in an optical lattice clock based on fermionic Sr atoms. In current one-dimensional lattice clocks nuclear spin-polarized atoms are known to have contact interactions of p-wave character and collective in nature. Here we focus on interactions that will influence the design of future optical lattice clocks. We study the case where atoms are no longer confined to a single nuclear spin state. By using samples of atoms with different distributions among the ten nuclear spin states of Sr we show that these interactions are SU(N) symmetric up to a 3% uncertainty in our measurements. Through these measurements we are also able to determine all the s-wave and p-wave scattering lengths.\nWe also study the case of nuclear spin-polarized interacting atoms that are allowed to tunnel between different lattice sites where the electronic spin and the motion of these atoms become coupled. We observe spectroscopically the precession of the collective magnetization and evolution of spin locking effects arising from the interplay between p-wave interactions and interactions induced by the spin-orbit coupling. The many-body dynamics are captured by a spin model that describes a broad class of condensed matter systems ranging from superconductors to quantum magnets.\nBy loading a dense sample of atoms into a magneto-optical trap we are able to observe long-range dipole-dipole interactions between our Sr atoms. These interactions will be important for atomic clocks based on a three dimensional lattice, such as the one recently demonstrated in our lab. In these clocks it is possible to remove the contact interactions between the atoms by loading only one atom per lattice site. In this case the dominant interactions will be from the long-range dipole-dipole interactions that will take place between the atoms.
Scaling up the performance of atomic clocks requires understanding complex many-body Hamiltonians to ensure meaningful gains for metrological applications. Here we use a degenerate Fermi gas loaded into a three-dimensional optical lattice to study the effect of a tunable Fermi-Hubbard Hamiltonian. The clock laser introduces a spin-orbit coupling spiral phase and breaks the isotropy of superexchange interactions, leading to XXZ-type spin anisotropy. By tuning the lattice confinement and applying imaging spectroscopy, we map out favorable atomic coherence regimes. We transition through various interaction regimes and observe coherent superexchange, tunable through on-site interaction and site-to-site energy shift, affecting the Ramsey fringe contrast over timescales >1 second. This study lays the groundwork for using a three-dimensional optical lattice clock to probe quantum magnetism and spin entanglement.