Quantum coherence is one of the primary non-classical features of quantum systems. While protocols such as the Leggett-Garg inequality (LGI) and quantum tomography can be used to test for the existence of quantum coherence and dynamics in a given system, unambiguously detecting inherent "quantumness" still faces serious obstacles in terms of experimental feasibility and efficiency, particularly in complex systems. Here we introduce two "quantum witnesses" to efficiently verify quantum coherence and dynamics in the time domain, without the expense and burden of non-invasive measurements or full tomographic processes. Using several physical examples, including quantum transport in solid-state nanostructures and in biological organisms, we show that these quantum witnesses are robust and have a much finer resolution in their detection window than the LGI has. These robust quantum indicators may assist in reducing the experimental overhead in unambiguously verifying quantum coherence in complex systems.
Quantum coherence is one of the primary non-classical features of quantum systems. While protocols such as the Leggett-Garg inequality (LGI) and quantum tomography can be used to test for the existence of quantum coherence and dynamics in a given system, unambiguously detecting inherent "quantumness" still faces serious obstacles in terms of experimental feasibility and efficiency, particularly in complex systems. Here we introduce two "quantum witnesses" to efficiently verify quantum coherence and dynamics in the time domain, without the expense and burden of non-invasive measurements or full tomographic processes. Using several physical examples, including quantum transport in solid-state nanostructures and in biological organisms, we show that these quantum witnesses are robust and have a much finer resolution in their detection window than the LGI has. These robust quantum indicators may assist in reducing the experimental overhead in unambiguously verifying quantum coherence in complex systems.
Quantum coherence, present whenever a quantum system exists in a superposition of multiple classically distinct states, marks one of the fundamental departures from classical physics. Quantum coherence has recently been investigated rigorously within a resource-theoretic formalism. However, the finer-grained notion of multilevel coherence, which explicitly takes into account the number of superposed classical states, has remained relatively unexplored. A comprehensive analysis of multi-level coherence, which acts as the single-party analogue to multi-partite entanglement, is essential for understanding natural quantum processes as well as for gauging the performance of quantum technologies. Here we develop the theoretical and experimental groundwork for characterizing and quantifying multilevel coherence. We prove that non-trivial levels of purity are required for multilevel coherence, as there is a ball of states around the maximally mixed state that do not exhibit multilevel coherence in any basis. We provide a simple necessary and sufficient analytical criterion to verify multilevel coherence, which leads to a complete classification for three-level systems. We present the robustness of multilevel coherence, a bona fide quantifier which we show to be numerically computable via semidefinite programming and experimentally accessible via multilevel coherence witnesses. We further verify and lower-bound the robustness of multilevel coherence by performing a semi-device-independent phase discrimination task, implemented experimentally with four-level probes in a photonic setup. Our results contribute to understanding the operational relevance of genuine multilevel coherence, also by demonstrating the key role it plays in enhanced phase discrimination---a primitive for quantum communication and metrology---and suggest new ways to reliably test the quantum behaviour of physical systems.
Abstract Quantum coherence is one of the most basic characteristics of quantum mechanics. Here we give some methods to detect and measure quantum coherence. Firstly, we propose a coherence criterion without full quantum state tomography based on partial transposition. Moreover, we present a coherent nonlinear detection strategy from witnesses, in which we find that for some coherent states, normal witness detection fails but our nonlinear detection succeeds. In addition, we prove that when the nonlinear detection on the two copies of the coherent state fails, the nonlinear detection on the three copies may be successful. Finally, due to the difficulty in calculating robustness of coherence for general states, we introduce a lower bound for coherent robustness based on the witness operator, and after comparing our lower bound with the currently known lower bound, one show that our lower bound is better. Coherence is believed to play a crucial role in quantum information tasks, making the detection and quantization of coherence particularly significant. Therefore, these results help to open up new avenues for advancement in quantum theory.
In this paper, we investigate the violation of the quantum witness, the entropic Leggett-Garg inequality (LGI) and the no-coherence-generating-and-detecting (NCGD) dynamics, under projective and coarsening measurements. We consider a qubit in the three scenarios: coherent dynamics, in the presence of dissipation, and in the presence of dephasing. For the pure qubit, we find that in the case of the projective measurement, the non-violation conditions of the quantum witness and the NCGD are the same; while the non-violation conditions of the entropic LGI and the quantum witness do not contain each other, i.e., a suitable conjunction of the quantum witness and the entropic LGI may be better for testing macrorealism. Also, for the pure qubit with coarsening measurement similar results can be obtained. For the dissipative qubit with projective measurement, the quantum witness and the NCGD can be both violated for a wider parameter regime than the entropic LGI. For the dissipative qubit with coarsening measurement, the violation of the NCGD is the most robust compared to the quantum witness and the entropic LGI. For the dephasing qubit with projective and coarsening measurements, the relationship among the quantum witness, the entropic LGI and the NCGD is similar to that of the pure qubit. In addition, we find that for pure, dissipative and dephasing qubits, the robustness of the coarsening measurement in final resolution is more vulnerable than that of the coarsening measurement in reference for the entropic LGI.
Abstract Leggett-Garg (LG) inequalities have been derived to clarify the validity of generalizing quantum mechanics to macroscopic systems for more than thirty years. They have been used as tools to investigate the existence of quantum coherence in macroscopic systems. Here, we show that such inequality violation can also be observed in classical optical systems. Using the linear polarization degree of freedom as the dichotomic observables, in a classical optical experiment, we have observed the violation of LG inequality by implementing the non-invasive measurement. Furthermore, the coherence witness, which is analogous to the quantum witness, has also been observed in the classical optical experiment. Our results not only provide new physical insights into the macroscopic quantum correlation and quantum witness, but also show their potential applications in correlated information processes.
Violations of the Leggett-Garg inequality (LGI) up to its algebraic bound under non-Hermitian dynamics are well established theoretically. Here, we demonstrate that such extreme violations are intrinsically fragile when realistic measurement processes are taken into account. We consider an open two-level system described by a time-local hybrid Liouvillian, with a continuous parameter q∈[0,1], representing detector efficiency, i.e., the fraction of quantum jump trajectories that are retained in the ensemble. This parameter interpolates between trace-preserving Lindblad dynamics (q=1) and non-Hermitian ``no-jump" evolution (q=0). While K3 approaches its algebraic maximum of 3 in the null-efficiency limit, even an infinitesimal increase in detector efficiency induces a rapid, highly nonlinear suppression toward the classical bound. This logarithmic sensitivity reveals that maximal LGI violations are not robust physical features but rather singular limits of idealized measurement conditions. Our results have direct experimental implications: achieving algebraic LGI violations in systems undergoing continuous time evolution requires near-perfect suppression of detected quantum jumps (i.e., effective post-selection), placing stringent constraints on detector performance. In contrast to discrete protocols based on time-non-divisible dynamics, our framework shows that extreme violations arising within continuous, divisible quantum trajectory evolution constitute a fundamentally fragile regime.
Quantum coherence has wide-ranging applications from quantum thermodynamics to quantum metrology, quantum channel discrimination, and even quantum biology. Thus, detecting and quantifying coherence are two fundamental problems in quantum resource theory. Here, we introduce feasible methods to detect and estimate the coherence by constructing coherence witnesses for any finite-dimensional states. Our coherence witnesses detect coherent states by testing whether the expectation value of the witness is negative or not. Two typical coherence witnesses are proposed and discussed based on our witness-constructing method, which are also used to estimate the robustness of coherence, the l1 norm, and the l2 norm of coherence measures. Furthermore, we compare one of our coherence witnesses with a previously introduced witness by proving that our witness is strictly stronger than that previous witness. We also present an application of coherence in a quantum metrology task, in which we estimate an unknown parameter by measuring our coherence witness.