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arXiv:1211.4463 · Physical Review Letters

Single Molecule Detection of Nanomechanical Motion

Vadim Puller, Brahim Lounis, F. Pistolesi

Published Mar 19, 2013• 59 citations
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Abstract

We investigate theoretically how single molecule spectroscopy techniques can be used to perform fast and high resolution displacement detection and manipulation of nanomechanical oscillators, such as singly clamped carbon nanotubes. We analyze the possibility of real time displacement detection by the luminescence signal and of displacement fluctuations by the degree of second order coherence. Estimates of the electromechanical coupling constant indicate that intriguing regimes of strong backaction between the two-level system of a molecule and the oscillator can be realized.

DOI
10.1103/physrevlett.110.125501

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We investigate theoretically how single molecule spectroscopy techniques can be used to perform fast and high resolution displacement detection and manipulation of nanomechanical oscillators, such as singly clamped carbon nanotubes. We analyze the possibility of real time displacement detection by the luminescence signal and of displacement fluctuations by the degree of second order coherence. Estimates of the electromechanical coupling constant indicate that intriguing regimes of strong backaction between the two-level system of a molecule and the oscillator can be realized.
It has been recently proposed that single molecule spectroscopy could be employed to detect the motion of nanomechanical resonators. Estimates of the coupling constant (ggg) between the molecular two-level system and the oscillator indicate that it can reach values much larger than the mechanical resonating pulsation (${\ensuremath{\omega}}_{m}$) and the two-level system linewidth ($\mathrm{\ensuremath{\Gamma}}$). Other experimental realizations of the same system are also approaching this strong-coupling regime. In this paper we investigate the behavior of the system in the limit for slow mechanical oscillator ${\ensuremath{\omega}}_{m}\ensuremath{\ll}\mathrm{\ensuremath{\Gamma}}$. We find that, for sufficiently large coupling, the system undergoes a bistability reminiscent of that observed in optical cavities coupled to mechanical resonators.
We propose and analyze an all-mechanical route to coherent control and quantum-state reconstruction of the fundamental flexural mode of a suspended carbon nanotube (CNT) operated in the anharmonic (Duffing/Kerr). A nearby atomic force microscope (AFM) provides a single, localized actuator that applies calibrated, time-dependent forces to the CNT. In the presence of mechanical anharmonicity this enables spectrally selective control of the lowest vibrational transition and thus supports effective two-level protocols such as Rabi oscillations and Ramsey interferometry. The same actuator also implements phase-space displacements required for Wigner function tomography via displaced-parity sampling, thereby unifying control and tomography without optical heating and without dedicated on-chip microwave drive lines at the CNT resonator. We develop explicit pulse sequences and a master equation framework that connect experimentally accessible signals to energy relaxation and phase coherence times and to parity-based quantum signatures, including negative regions of the Wigner function. The approach is compatible with multiple readout modalities, including direct AFM-based detection and dispersive coupling to superconducting circuitry such as Cooper-pair box, and/or a microwave cavity. Together, these techniques provide complete access to populations, coherence, and parity within a single device architecture. This minimal scheme provides a practical route to all-mechanical quantum control and state-resolved characterization of decoherence in mesoscopic mechanical systems.
The quantum behaviour of mechanical resonators is a new and emerging field driven by recent experiments reaching the quantum ground state. The high frequency, small mass, and large quality-factor of carbon nanotube resonators make them attractive for quantum nanomechanical applications. A common element in experiments achieving the resonator ground state is a second quantum system, such as coherent photons or a superconducting device, coupled to the resonators motion. For nanotubes, however, this is a challenge due to their small size. Here, we couple a carbon nanoelectromechanical (NEMS) device to a superconducting circuit. Suspended carbon nanotubes act as both superconducting junctions and moving elements in a Superconducting Quantum Interference Device (SQUID). We observe a strong modulation of the flux through the SQUID from displacements of the nanotube. Incorporating this SQUID into superconducting resonators and qubits should enable the detection and manipulation of nanotube mechanical quantum states at the single-phonon level.
We investigate the coupling of a nanomechanical oscillator in the quantum regime with molecular (electric) dipoles. We find theoretically that the cantilever can produce single-mode squeezing of the center-of-mass motion of an isolated trapped molecule and two-mode squeezing of the phonons of an array of molecules. This work opens up the possibility of manipulating dipolar crystals, which have been recently proposed as quantum memory, and more generally, is indicative of the promise of nanoscale cantilevers for the quantum detection and control of atomic and molecular systems.
Among the various nanoscale systems operating in the quantum limit, nanomechanical oscillators have emerged as particularly powerful platforms. They constitute highly sensitive sensors and can mediate interactions between light and localized quantum systems, playing a central role in various quantum information processing architectures. Due to their relatively large mass, they also serve as ideal platforms for investigating the transition between classical and quantum behavior. This thesis examines the dynamics of a nanomechanical oscillator coupled to a driven two-level system. The analysis focuses on the resolved sideband limit, where the twolevel system’s damping rate Γ is much smaller than the mechanical frequency ωm, and explores both the strong coupling (ωm ≫ g0 ≫ Γ) and ultra-strong coupling (g0 ∼ ωm ≫ Γ) regimes, where g0 denotes the coupling strength. These regimes enable coherent manipulation of the mechanical state while preserving its quantum coherence. Under blue-detuned driving of the two-level system and assuming low mechanical damping, the system exhibits a dynamical instability marked by the emergence of limit cycles in the mechanical oscillator. The onset of this regime is accompanied by pronounced fluctuations in the photon emission from the two-level system, indicated by a large deviation from Poissonian statistics. The phonon statistics display a similar behavior, offering an additional experimental signature. As the coupling strength approaches ωm, the mechanical oscillator reaches a steady state with non-classical feature. The phonon number distribution in this regime resembles that of Fock states, and the corresponding quasi-probability distribution in phase space displays negative regions, a signature of nonclassicality. A method is proposed to detect this non-classicality experimentally through measurements of the emitted light, from which the full quantum state of the coupled system can be reconstructed. The robustness of this approach is analyzed in the presence of realistic noise sources. The thesis further investigates the response of the system under two-tone driving. A tailored model is developed to describe this regime at strong coupling. When the driving frequencies are tuned to the first blue and red sidebands, the mechanical oscillator reaches a steady state exhibiting quadrature squeezing. In the case where both driving frequencies are red-detuned, the oscillator evolves into a superposition of coherent states, analogous to the behavior of a parametrically driven resonator. In both configurations, non-classical features become prominent when g0 approaches ωm. These results provide new insights into the generation and stabilization of non-classical and squeezed mechanical states. We outline feasible strategies for their detection, offering potential applications in hybrid quantum systems and foundational tests of quantum mechanics.
Nonlinearity at the scale of zero-point motion opens new possibilities for the control and readout of nanomechanical systems, but achieving this remains a formidable challenge. Here we demonstrate that ultrastrong coupling (USC) between a nanotube mechanical oscillator and a double-quantum-dot electronic two-level system enables a mechanical Kerr (Duffing) nonlinearity at the zero-point motion scale. In the dispersive regime, this large coupling yields a mechanical anharmonicity of α=1.4%α= 1.4\%α=1.4% - three orders of magnitude larger than in previous work - while preserving the predominantly mechanical nature of the lowest energy states. We further demonstrate a purely quadratic cavity-based continuous readout of the mechanical motion. This continuous nonlinear optomechanical readout is enforced by a double-quantum dot symmetry, which can be broken by gate tuning to introduce a large linear transduction. These results establish a tunable USC platform that enables strong mechanical anharmonicity and nonlinear continuous readout at the zero-point motion scale.