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arXiv:1210.3623 · Physical Review A

Keldysh approach for nonequilibrium phase transitions in quantum optics: Beyond the Dicke model in optical cavities

Emanuele G. Dalla Torre, Sebastian Diehl, Mikhail D. Lukin, Subir Sachdev A, Philipp Strack

Published Feb 21, 2013• 250 citations
arXivHTMLPDF

Abstract

We investigate nonequilibrium phase transitions for driven atomic ensembles interacting with a cavity mode and coupled to a Markovian dissipative bath. In the thermodynamic limit and at low frequencies, we show that the distribution function of the photonic mode is thermal, with an effective temperature set by the atom-photon interaction strength. This behavior characterizes the static and dynamic critical exponents of the associated superradiance transition. Motivated by these considerations, we develop a general Keldysh path-integral approach that allows us to study physically relevant nonlinearities beyond the idealized Dicke model. Using standard diagrammatic techniques, we take into account the leading-order corrections due to the finite number $N$ of atoms. For finite $N$, the photon mode behaves as a damped classical nonlinear oscillator at finite temperature. For the atoms, we propose a Dicke action that can be solved for any $N$ and correctly captures the atoms' depolarization due to dissipative dephasing.

DOI
10.1103/physreva.87.023831

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Acta Physica Sinica•Jan 1, 2015•0 citations
We investigate nonequilibrium phase transitions for driven atomic ensembles interacting with a cavity mode and coupled to a Markovian dissipative bath. In the thermodynamic limit and at low frequencies, we show that the distribution function of the photonic mode is thermal, with an effective temperature set by the atom-photon interaction strength. This behavior characterizes the static and dynamic critical exponents of the associated superradiance transition. Motivated by these considerations, we develop a general Keldysh path-integral approach that allows us to study physically relevant nonlinearities beyond the idealized Dicke model. Using standard diagrammatic techniques, we take into account the leading-order corrections due to the finite number NNN of atoms. For finite NNN, the photon mode behaves as a damped classical nonlinear oscillator at finite temperature. For the atoms, we propose a Dicke action that can be solved for any NNN and correctly captures the atoms' depolarization due to dissipative dephasing.
In the context of ultracold atoms in multimode optical cavities, the appearance of a quantum-critical glass phase of atomic spins has been predicted recently. Due to the long-range nature of the cavity-mediated interactions, but also the presence of a driving laser and dissipative processes such as cavity photon loss, the quantum optical realization of glassy physics has no analog in condensed matter and could evolve into a ``cavity glass microscope'' for frustrated quantum systems out of equilibrium. Here we develop the nonequilibrium theory of the multimode Dicke model with quenched disorder and Markovian dissipation. Using a unified Keldysh path integral approach, we show that the defining features of a low-temperature glass, representing a critical phase of matter with algebraically decaying temporal correlation functions, are seen to be robust against the presence of dissipation due to cavity loss. The universality class, however, is modified due to the Markovian bath. The presence of strong disorder leads to an enhanced equilibration of atomic and photonic degrees of freedom, including the emergence of a common low-frequency effective temperature. The imprint of the atomic spin-glass physics onto the photon subsystem realizes a ``photon glass'' state and makes it possible to detect the glass state by standard experimental techniques of quantum optics. We provide an unambiguous characterization of the superradiant and glassy phases in terms of fluorescence spectroscopy, homodyne detection, and the temporal photon correlation function ${g}^{(2)}(\ensuremath{\tau})$.
The Dicke model famously exhibits a phase transition to a superradiant phase with a macroscopic population of photons and is realized in multiple settings in open quantum systems. In this paper, we study a variant of the Dicke model where the cavity mode is lossy due to the coupling to a Markovian environment while the atomic mode is coupled to a colored bath. We analytically investigate this model by inspecting its low-frequency behavior via the Schwinger-Keldysh field theory and carefully examine the nature of the corresponding superradiant phase transition. Integrating out the fast modes, we can identify a simple effective theory allowing us to derive analytical expressions for various critical exponents including the dynamical exponent. We find excellent agreement with previous numerical results when the non-Markovian bath is at zero temperature; however, contrary to these studies, our low-frequency approach reveals that the same exponents govern the critical behavior when the colored bath is at finite temperature unless the chemical potential is zero. Furthermore, we show that the superradiant phase transition is classical in nature, while it is genuinely nonequilibrium. We derive a fractional Langevin equation and conjecture the associated fractional Fokker-Planck equation that captures the system's long-time memory as well as its nonequilibrium behavior. Finally, we consider finite-size effects at the phase transition and identify the finite-size scaling exponents, unlocking a rich behavior in both statics and dynamics of the photonic and atomic observables.
We mainly investigate Dicke phase transition at finite temperature in an optomechanical-atomic cavity by means of the functional path-integral approach. By the thermodynamic equilibrium equation, the mean photon number, the scaled atomic population, the mean phonon number, the average energy and the rich phase diagram are depicted in the existence of the nonlinear atom–photon interaction, the nonlinear photon–photon coupling strength, the pump–cavity detuning and the finite temperature. Beside Dicke phase transition from the normal phase (NP) to the superraidant phase (SP) at finite temperature, the collapse of the SP and the dynamically unstable state (DUS) are revealed showing the effects of the photon–phonon coupling strength ξ and nonlinear atom–photon interaction U. Meanwhile, a new phase transition occurs from the SP to the dynamically unstable state (DUS) at the turning point gt with the existence of ξ or U. The region of the SP can be completely eliminated by the mechanically and thermally stimulated photon-emission. The entropy and corresponding specific heats are presented to demonstrate the corresponding critical behavior at the phase transition point.
The Dicke model describes the coherent interaction of a laser-driven ensemble of two-level atoms with a quantized light field. It is realized within cavity QED experiments, which in addition to the coherent Dicke dynamics feature dissipation due to, e.g., atomic spontaneous emission and cavity photon loss. Spontaneous emission supports the uncorrelated decay of individual atomic excitations as well as the enhanced collective decay of an excitation that is shared by NNN atoms and whose strength is determined by the cavity geometry. We derive a many-body master equation for the dissipative Dicke model including both spontaneous emission channels and analyze its dynamics on the basis of Heisenberg-Langevin and stochastic Bloch equations. We find that the collective loss channel leads to a region of bistability between the empty and the superradiant state. Transitions between these states are driven by nonthermal Markovian noise. The interplay between dissipative and coherent elements leads to a genuine nonequilibrium dynamics in the bistable regime, which is expressed via a nonconservative force and a multiplicative noise kernel appearing in the stochastic Bloch equations. We present a semiclassical approach, based on stochastic nonlinear optical Bloch equations, which for the infinite-range Dicke model become exact in the large-NNN-limit. The absence of an effective free-energy functional, however, necessitates the inclusion of fluctuation corrections with O(1/N)O(1/N)O(1/N) for finite $N<\ensuremath{\infty}$ to locate the nonthermal first-order phase transition between the superradiant and the empty cavity.
The interplay between many-body interactions and controlled dissipation provides a rich setting for nonequilibrium quantum phases. We explore the superradiant phase transitions in a Rydberg-interacting open Dicke model with cavity loss and local dissipation. We find that the nonlinear feedback from atomic interactions stabilizes the atomic collective excited state and induces resonant collective motion, which can be further converted into robust superradiant oscillations with the inclusion of local dissipation. Beyond the mean-field approximation, we prove this system can support the finite-size local dissipative temporal order, i.e., continuous time crystal, from evidences of the decreasing damping of a finite-frequency Liouvillian mode and the linear-size scaling of quantum fluctuations. The correlation between the atomic colletive dynamics and the cavity photon number makes our findings easy to detect from output optical signal. By bridging interacting atomic matter and driven-dissipative cavity QED, our Rydberg-interacting Dicke model provides a unique spin-1/2 platform for exploring dynamical phase transitions and macroscopic temporal order in open quantum matter.
In this paper, we investigate the finite-temperature properties and phase transition of the Dicke model. Converting the atomic pseudo-spin operator to the two-mode Fermi operators, we obtain the partition function in terms of the imaginary-time path integral. The atomic population and average photon number as analytic functions of the atom-photon coupling strength are found from the thermodynamic equilibrium equation, which leads to the stationary state at a finite temperature and is determined by the variation in an extremum-condition of the Euclidean action with respect to the bosonic field. In particular we study the phase transition from normal to superradiation phase at a fixed low-temperature, in which the phase transition is dominated by quantum fluctuations. The phase transition induced by the variation of the atom-photon coupling strength indeed obeys the Landau continuous phase-transition theory, in which the average photon-number can serve as an order parameter with non-zero value that characterizes the superradiation phase. In the zero temperature limit our results recover exactly all those obtained from the quantum phase transition theory at zero temperature. In addition, we discuss the thermodynamic properties and compare the difference between finite-temperature phase transition and zero-temperature quantum phase transition. It is discovered that the average photon-number and mean energy in the low-temperature stationary state coincide with the corresponding values of zero-temperature in the strong coupling region. The entropy of the superradiation phase decays rapidly to zero with the increase of coupling strength.